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Using Quasiparticle Poisoning To Detect Photons

P. M. Echternach, Peter K. Day

Published Mar 1, 2006• 0 citations
OpenAlex

Abstract

According to a proposal, a phenomenon associated with excitation of quasiparticles in certain superconducting quantum devices would be exploited as a means of detecting photons with exquisite sensitivity. The phenomenon could also be exploited to perform medium-resolution spectroscopy. The proposal was inspired by the observation that Coulomb blockade devices upon which some quantum logic gates are based are extremely sensitive to quasiparticles excited above the superconducting gaps in their leads. The presence of quasiparticles in the leads can be easily detected via the charge states. If quasiparticles could be generated in the leads by absorption of photons, then the devices could be used as very sensitive detectors of electromagnetic radiation over the spectral range from x-rays to submillimeter waves. The devices in question are single-Cooper-pair boxes (SCBs), which are mesoscopic superconducting devices developed for quantum computing. An SCB consists of a small superconducting island connected to a reservoir via a small tunnel junction and connected to a voltage source through a gate capacitor. An SCB is an artificial two-level quantum system, the Hamiltonian of which can be controlled by the gate voltage. One measures the expected value of the charge of the eigenvectors of this quantum system by use of a radio-frequency single-electron transistor. A plot of this expected value of charge as a function of gate voltage resembles a staircase that, in the ideal case, consists of steps of height 2 e (where e is the charge of one electron). Experiments have shown that depending on the parameters of the device, quasiparticles in the form of "broken" Cooper pairs present in the reservoir can tunnel to the island, giving rise to steps of 1 e. This effect is sometimes called "poisoning." Simulations have shown that an extremely small average number of quasiparticles can generate a 1-e periodic signal. In a device according to the proposal, this poisoning would be turned to advantage. Depending on the wavelength, an antenna or other component would be used to couple radiation into the reservoir, wherein the absorption of photons would break Cooper pairs, thereby creating quasiparticles that, in turn, would tunnel to the island, creating a 1-e signal. On the basis of conservative estimates of device parameters derived from experimental data and computational simulations that fit the data, it has been estimated that the noise equivalent power of a device according to the proposal could be as low as 6 10(exp -22) W/Hz(exp 1/2). It has also been estimated that the spectroscopic resolution (photon energy divided by increment of photon energy) of such a device in visible light would exceed 100.

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We demonstrate the operation of a differential single Cooper-pair box, a charge qubit consisting of two aluminum islands, isolated from ground, coupled by a pair of small-area Josephson junctions, and read out with a superconducting differential radio-frequency single electron transistor. We have tested four devices, all of which show evidence of quasiparticle poisoning. The devices are characterized with microwave spectroscopy and temperature dependence studies, and Coulomb staircases are shown to be e-periodic in all samples. However, coherent control is still possible with non-adiabatic voltage pulses. Coherent oscillation experiments and a relaxation time measurement were performed using a charge derivative readout technique.

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In this thesis the single Cooper pair box (SCB) is investigated with a radio frequency single electron transistor (RF-SET). The RF-SET is used as an electrometer to detect the charge of the SCB. The SCB can be regarded as a quantum two-level system and could therefore be a possible qubit. Both the SCB and the RF-SET have been fabricated with e-beam lithography followed by two-angle shadow evaporation of aluminium. The system has been measured in a dilution refrigerator at temperatures of ~30 mK. A charge sensitivity of 2.3 μe/square root of Hz was measured for an optimized RF-SET with a bandwidth of 7 MHz, operated in the superconducting state. In a phase sensitive measurement of the RF-SET reflected signal, the gate dependence of the quantum capacitance, due to avoided level crossing, was detected in a superconducting SET. Coulomb staircases for the SCB were obtained by changing the charge of the SCB by ramping a gate voltage and continuously measuring the charge with the RF-SET. To prevent quasiparticle poisoning of the SCB island, we have used a method of graded gaps. Here we exploit the greater reduction of the superconducting gap for the connecting leads with an external magnetic field applied, resulting in a higher gap for the island. This creates an effective barrier against quasiparticle tunnelling. The charging energy and the Josephson coupling energy of the SCB were measured with microwave spectroscopy. The SCBs were fabricated in a SQUID geometry, which made it possible to tune the Josephson coupling energy of the box. This tuning was verified through microwave spectroscopy. The effect of tuning could also be seen in the pure 2e Coulomb staircase, as a predicted smearing of the staircase, which was in excellent agreement with the independent spectroscopy data. Coherent quantum oscillation of the SCB charge state was measured by applying nonadiabatic DC-pulses to the SCB gate. The measured amplitude of the charge oscillations was higher than 70%. The deviation from 100% can be explained by the initial charge state purity and the finite rise time of the pulses. The longest decoherence time of the charge oscillations was T2 = 9 ns at the charge degeneracy point. It was found to be limited by relaxation. Away from the degeneracy point the decoherence time was limited by pure dephasing, due to low frequency charge fluctuators.

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The single-electron transistor as an ultrasensitive microwave detector

J. M. Hergenrother, Jia Grace Lu, M. Tinkham

We have measured single-electron tunneling transistors with superconducting islands and conclude that they may be used as ultrasensitive detectors of microwave radiation for frequencies /spl ges/80 GHz. These devices contain a small superconducting Al island that is weakly coupled to a bias circuit through two small-capacitance tunnel junctions and a capacitive gate. At low bias voltages and temperatures, a single quasiparticle may only be introduced to the island through photon-assisted tunneling. Once this occurs, the quasiparticle is trapped on the island for /spl sim/1 /spl mu/s because it takes a relatively long time for this specific quasiparticle to tunnel off. While it is trapped, charge is transported through the system two electrons at a time. Since the photon-assisted transition merely switches the detector current on, this device is not limited to one electron tunneled through the system per absorbed photon. Measurements indicate that at least 100 electrons can tunnel for every absorbed photon, which corresponds to a noise-equivalent power of 3/spl times/10/sup -20/ W//spl radic/Hz at 80 GHz if the current is measured with a commercial current amplifier.>

IEEE Transactions on Applied Superconductivity•Jun 1, 1995•7 citations
According to a proposal, a phenomenon associated with excitation of quasiparticles in certain superconducting quantum devices would be exploited as a means of detecting photons with exquisite sensitivity. The phenomenon could also be exploited to perform medium-resolution spectroscopy. The proposal was inspired by the observation that Coulomb blockade devices upon which some quantum logic gates are based are extremely sensitive to quasiparticles excited above the superconducting gaps in their leads. The presence of quasiparticles in the leads can be easily detected via the charge states. If quasiparticles could be generated in the leads by absorption of photons, then the devices could be used as very sensitive detectors of electromagnetic radiation over the spectral range from x-rays to submillimeter waves. The devices in question are single-Cooper-pair boxes (SCBs), which are mesoscopic superconducting devices developed for quantum computing. An SCB consists of a small superconducting island connected to a reservoir via a small tunnel junction and connected to a voltage source through a gate capacitor. An SCB is an artificial two-level quantum system, the Hamiltonian of which can be controlled by the gate voltage. One measures the expected value of the charge of the eigenvectors of this quantum system by use of a radio-frequency single-electron transistor. A plot of this expected value of charge as a function of gate voltage resembles a staircase that, in the ideal case, consists of steps of height 2 e (where e is the charge of one electron). Experiments have shown that depending on the parameters of the device, quasiparticles in the form of "broken" Cooper pairs present in the reservoir can tunnel to the island, giving rise to steps of 1 e. This effect is sometimes called "poisoning." Simulations have shown that an extremely small average number of quasiparticles can generate a 1-e periodic signal. In a device according to the proposal, this poisoning would be turned to advantage. Depending on the wavelength, an antenna or other component would be used to couple radiation into the reservoir, wherein the absorption of photons would break Cooper pairs, thereby creating quasiparticles that, in turn, would tunnel to the island, creating a 1-e signal. On the basis of conservative estimates of device parameters derived from experimental data and computational simulations that fit the data, it has been estimated that the noise equivalent power of a device according to the proposal could be as low as 6 10(exp -22) W/Hz(exp 1/2). It has also been estimated that the spectroscopic resolution (photon energy divided by increment of photon energy) of such a device in visible light would exceed 100.
We demonstrate the operation of a differential single Cooper-pair box, a charge qubit consisting of two aluminum islands, isolated from ground, coupled by a pair of small-area Josephson junctions, and read out with a superconducting differential radio-frequency single electron transistor. We have tested four devices, all of which show evidence of quasiparticle poisoning. The devices are characterized with microwave spectroscopy and temperature dependence studies, and Coulomb staircases are shown to be e-periodic in all samples. However, coherent control is still possible with non-adiabatic voltage pulses. Coherent oscillation experiments and a relaxation time measurement were performed using a charge derivative readout technique.
We propose a sensitive new detector based on Cooper pair breaking in a superconductor. The quantum capacitor detector (QCD) exploits the extraordinary sensitivity of superconducting single-electron devices to the presence of quasiparticles generated by pair-breaking photons. This concept would enable single-photon detection at far-IR and sub-millimeter frequencies with detector sensitivities that exceed that of transition-edge-sensor bolometers (TES), kinetic inductance detectors (KID), and superconducting tunnel junction detectors (STJ). The detectors we propose are based on the single Cooper pair box (SCB), a mesoscopic superconducting device that has been successfully developed at JPL for applications in quantum computing. This concept allows for frequency multiplexing of a large number of pixels using a single RF line, and does not require individual bias of each pixel. The QCD is ideal for the sensitive spectrographs considered for upcoming cold space telescopes, such as BLISS for SPICA in the coming decade, and for the more ambitious instruments for the SAFIR / CALISTO and SPIRIT / SPECS missions envisioned for the 2020 decade. These missions require large detector arrays (> 10,000 elements) which are limited by astrophysical background noise, corresponding to a noise-equivalent power (NEP) as low as 2x10-20 W / Hz1/2. Given its intrinsic response time, the QCD could also be used for energy-resolved visible photon detection, with estimated energy resolution > 100, enabling imaging low-resolution spectroscopy with an array of detectors.
In this thesis the single Cooper pair box (SCB) is investigated with a radio frequency single electron transistor (RF-SET). The RF-SET is used as an electrometer to detect the charge of the SCB. The SCB can be regarded as a quantum two-level system and could therefore be a possible qubit. Both the SCB and the RF-SET have been fabricated with e-beam lithography followed by two-angle shadow evaporation of aluminium. The system has been measured in a dilution refrigerator at temperatures of ~30 mK. A charge sensitivity of 2.3 μe/square root of Hz was measured for an optimized RF-SET with a bandwidth of 7 MHz, operated in the superconducting state. In a phase sensitive measurement of the RF-SET reflected signal, the gate dependence of the quantum capacitance, due to avoided level crossing, was detected in a superconducting SET. Coulomb staircases for the SCB were obtained by changing the charge of the SCB by ramping a gate voltage and continuously measuring the charge with the RF-SET. To prevent quasiparticle poisoning of the SCB island, we have used a method of graded gaps. Here we exploit the greater reduction of the superconducting gap for the connecting leads with an external magnetic field applied, resulting in a higher gap for the island. This creates an effective barrier against quasiparticle tunnelling. The charging energy and the Josephson coupling energy of the SCB were measured with microwave spectroscopy. The SCBs were fabricated in a SQUID geometry, which made it possible to tune the Josephson coupling energy of the box. This tuning was verified through microwave spectroscopy. The effect of tuning could also be seen in the pure 2e Coulomb staircase, as a predicted smearing of the staircase, which was in excellent agreement with the independent spectroscopy data. Coherent quantum oscillation of the SCB charge state was measured by applying nonadiabatic DC-pulses to the SCB gate. The measured amplitude of the charge oscillations was higher than 70%. The deviation from 100% can be explained by the initial charge state purity and the finite rise time of the pulses. The longest decoherence time of the charge oscillations was T2 = 9 ns at the charge degeneracy point. It was found to be limited by relaxation. Away from the degeneracy point the decoherence time was limited by pure dephasing, due to low frequency charge fluctuators.
The aluminum single Cooper-pair box (SCB) qubit has demonstrated potential as a candidate for quantum computing. Measurements of coherent manipulation of the relevant SCB states have been demonstrated with various charge and quantum capacitance readout methods. We performed studies of quasiparticle dynamics in an SCB that yielded poisoning probabilities and rates of quasiparticle tunneling processes. Attempts to prevent poisoning with a differential SCB isolated from ground and other quasiparticle sources revealed the possibility for quasiparticle generation on superconducting islands of diminutive size. We have gone on to conduct more advanced measurements of coupled qubits as an important step towards the realization of multi-qubit systems and other precursors that are pivotal in the evolution of reliable quantum computing.
We present a series of measurements on nine single Cooper-pair boxes (SCBs), where the charging energy, E C , and the Josephson coupling energy, E J , have been varied. We have investigated both the ground state properties of the SCBs and their quantum coherent properties. The state of the SCBs could be manipulated by an external gate voltage and the charge was measured by coupling it capacitatively to a radio-frequency single-electron-transistor (RF-SET). By ramping the gate voltage and simultaneously measuring the charge of the SCBs using the RF-SET, we could measure the Coulomb staircases of the SCBs. For sufficiently low E C the SCBs showed a fully 2 e periodic Coulomb staircase. For samples with higher E C the staircase showed a short step for odd number of charges indicating quasi-particle 'poisoning'. However, if E C was not too large, the short step could be removed by applying a parallel magnetic field. We attribute this effect to a stronger suppression of the superconducting energy gap in the reservoir than in the box. Using microwave spectroscopy we have determined E C and E J for the SCBs. These values agree well with the shape of the Coulomb staircases which we measure. For a limited range of gate voltage, the SCBs were found to behave as model two-level quantum-mechanical systems. A non-adiabatic change in the induced island charge was used to bring two charge states into resonance. The resulting time evolution showed clear charge oscillations between the ground and excited state, with an amplitude above 70% and a frequency given by the energy level separation divided by Planck's constant. These oscillations had a longest coherence time of T 2 = 9 ns, at a point where the pure charge states are degenerate. The coherence time at this point was found to be limited by the relaxation rate. Away from the charge degeneracy point, the coherence time was limited by the pure dephasing rate. The dependence of T 2 on gate charge suggested that low frequency fluctuators were the main source of dephasing away from the degeneracy point.
We have measured single-electron tunneling transistors with superconducting islands and conclude that they may be used as ultrasensitive detectors of microwave radiation for frequencies /spl ges/80 GHz. These devices contain a small superconducting Al island that is weakly coupled to a bias circuit through two small-capacitance tunnel junctions and a capacitive gate. At low bias voltages and temperatures, a single quasiparticle may only be introduced to the island through photon-assisted tunneling. Once this occurs, the quasiparticle is trapped on the island for /spl sim/1 /spl mu/s because it takes a relatively long time for this specific quasiparticle to tunnel off. While it is trapped, charge is transported through the system two electrons at a time. Since the photon-assisted transition merely switches the detector current on, this device is not limited to one electron tunneled through the system per absorbed photon. Measurements indicate that at least 100 electrons can tunnel for every absorbed photon, which corresponds to a noise-equivalent power of 3/spl times/10/sup -20/ W//spl radic/Hz at 80 GHz if the current is measured with a commercial current amplifier.>