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Elsevier eBooks

Resonance fluorescence emission from single semiconductor quantum dots coupled to high-quality microcavities

Sven M. Ulrich, Ata Ulhaq, Peter Michler

Published Jan 1, 2012• 0 citations
Publisher
DOI
10.1533/9780857096395.1.1

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Resonant laser spectroscopy is essential for the characterization, operation, and manipulation of single-quantum systems such as semiconductor quantum dots. The separation of the weak resonance fluorescence from the excitation laser is key for high-quality single- and entangled-photon sources. This is often achieved by cross-polarization laser extinction, which is limited by the quality of the optical elements. Recently, it was discovered that Fresnel-reflection birefringence in combination with single-mode filtering counteracting spin-orbit-coupling effects enables a three-order-of-magnitude improvement of polarization extinction [Benelajla et al., Phys. Rev. X 11, 021007 (2021)]. Here, we demonstrate this method for cross-polarization-extinction enhancement in cryogenic confocal microscopy of a resonantly excited semiconductor quantum dot in a birefringent optical microcavity, and observe a $10\ifmmode\times\else\texttimes\fi{}$ improvement of the single-photon contrast.
It is shown that spectrally resolved photon-statistics measurements of the resonance fluorescence from realistic semiconductor quantum-dot systems allow for high contrast identification of the two-photon strong-coupling states. Using a microscopic theory, the second-rung resonance of Jaynes-Cummings ladder is analyzed and optimum excitation conditions are determined. The computed photon-statistics spectrum displays gigantic, experimentally robust resonances at the energetic positions of the second-rung emission.
Applying continuous-wave pure resonant s-shell optical excitation of individual quantum dots in a high-quality micropillar cavity, we demonstrate the generation of post-selected indistinguishable photons in resonance fluorescence. Close to ideal visibility contrast of 90% is verified by polarization-dependent Hong-Ou-Mandel two-photon interference measurements. Furthermore, a strictly resonant continuous-wave excitation together with controlling the spontaneous emission lifetime of the single quantum dots via tunable emitter-mode coupling (Purcell) is proven as a versatile scheme to generate close to Fourier transform-limited (T2/(2T1)=0.91) single photons even at 80% of the emission saturation level.