Low-frequency magnetic flux noise remains a persistent performance bottleneck in dc Superconducting Quantum Interference Devices (SQUIDs) and flux-tunable superconducting qubits across dilution refrigerator base temperatures. Traditional models treat surface paramagnetic spins as independent, non-interacting fluctuators, failing to explain strong exchange interactions, sub-Kelvin temperature insensitivity, and the universal Clarke R/W perimeter scaling law. Here, we resolve these empirical anomalies from first principles by embedding surface spins into a continuous inter-site electrostatic and magnetic potential manifold. Applying the Lindeberg-Feller Vector Central Limit Theorem to random surface dipolar fields yields an emergent Gaussian Density of States (GDOS) for spin inversion barriers. Integrating this disordered manifold across the SQUID washer geometry via magnetostatic reciprocity reproduces the universal R/W scaling law and predicts an absolute spectral amplitude of approximately 1.4 to 1.7 micro-Phi-0 per square root of Hz at 100 mK. Furthermore, accounting for non-cancellation phase agitation within the open spin saddles proves that soft-magnon and phonon bremsstrahlung sustain an irreducible millikelvin quantum flux noise floor down to absolute zero. In order to bridge microscopic theory with practical engineering, the manuscript includes a complete, modular MATLAB simulation toolbox (compatible with MATLAB R2016a/b and later) that computes closed-form classical flux noise spectral densities, frequency sweeps, and absolute spectral amplitudes for device optimization.
The quasiparticle density observed in low-temperature superconducting circuits is several orders of magnitude larger than the value expected at thermal equilibrium. The tunneling of this excess of quasiparticles across Josephson junctions is recognized as one of the main loss and decoherence mechanisms in superconducting qubits. Here we present a unified impedance theory that accounts for quasiparticle energy loss in circuit regions both far from and near to (across) junctions. Our theory leverages the recent experimental demonstration that the excess quasiparticles are in quasiequilibrium [Connolly et al., Phys. Rev. Lett. 132, 217001 (2024)] and uses a generalized fluctuation-dissipation theorem to predict the amount of charge and flux noise generated by them. We compute the resulting energy relaxation time
T1 in transmon qubits with and without junction asymmetric gap engineering, and show that quasiparticles residing away from junctions can play a dominant role in the former case. They also may provide an upper limit for resonator quality factors if the density of amorphous two-level systems is reduced. In addition, we show that charge noise from quasiparticles leads to flux noise that is logarithmic in frequency, giving rise to a ``nearly white'' contribution that is comparable to the flux noise observed in flux qubits. This contrasts with amorphous two-level systems, whose associated flux noise is shown to be super-Ohmic. We discuss how this quasiparticle flux noise can limit ${T}_{2}^{\ensuremath{\ast}}$ coherence times in flux-tunable qubits. The final conclusion is that asymmetric gap engineering can greatly reduce noise and increase coherence times in superconducting qubits.
We compute the decoherence caused by
1∕f fluctuations at low frequency
f in the critical current
I0 of Josephson junctions incorporated into flux, phase, charge, and hybrid flux-charge superconducting quantum bits (qubits). The dephasing time ${\ensuremath{\tau}}_{\ensuremath{\phi}}$ scales as ${I}_{0}∕\ensuremath{\Omega}\ensuremath{\Lambda}{S}_{{I}_{0}}^{1∕2}(1\phantom{\rule{0.3em}{0ex}}\mathrm{Hz})$, where $\ensuremath{\Omega}∕2\ensuremath{\pi}$ is the energy-level splitting frequency,
SI0(1Hz) is the spectral density of the critical-current noise at
1Hz, and $\ensuremath{\Lambda}\ensuremath{\equiv}\ensuremath{\mid}{I}_{0}d\ensuremath{\Omega}∕\ensuremath{\Omega}d{I}_{0}\ensuremath{\mid}$ is a parameter computed for given parameters for each type of qubit that specifies the sensitivity of the level splitting to critical-current fluctuations. Computer simulations show that the envelope of the coherent oscillations of any qubit after time
t scales as $\mathrm{exp}(\ensuremath{-}{t}^{2}∕2{\ensuremath{\tau}}_{\ensuremath{\phi}}^{2})$ when the dephasing due to critical-current noise dominates the dephasing from all sources of dissipation. We compile published results for fluctuations in the critical current of Josephson tunnel junctions fabricated with different technologies and a wide range in
I0 and area
A, and show that their values of
SI0(1Hz) scale to within a factor of 3 of $[144{({I}_{0}∕\ensuremath{\mu}\mathrm{A})}^{2}∕(\mathcal{A}∕\ensuremath{\mu}{\mathrm{m}}^{2})]{(\mathrm{pA})}^{2}∕\mathrm{Hz}$ at
4.2K. We empirically extrapolate
SI01∕2(1Hz) to lower temperatures using a scaling
T(K)∕4.2. Using this result, we find that the predicted values of ${\ensuremath{\tau}}_{\ensuremath{\phi}}$ at
100mK range from $0.8\phantom{\rule{0.5em}{0ex}}\text{to}\phantom{\rule{0.5em}{0ex}}12\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{s}$, and are usually substantially longer than values measured experimentally at lower temperatures.
For over three decades, the presence of magnetic flux noise with a power spectral density scaling roughly as
SPhi(f)propto1/falpha, where
alphalesssim1, has been known to limit the low-frequency performance of dc superconducting quantum interference devices (SQUIDs). In recent years, experiments indicate that this same noise persists to frequencies up to 1~GHz and is a dominant source of dephasing in flux-sensitive superconducting quantum bits (qubits). Thus, the reduction of flux noise presents a major hurdle towards the successful realization of scalable quantum computers that are based on flux-based qubits. In this thesis, we present experimental measurements, theoretical analyses, and numerical simulations that support a more detailed understanding of both the microscopic and macroscopic properties of flux noise.Our experimental work begins with flux noise measurements of a large number of SQUIDs in the temperature range from 0.1~K to 4~K. We report on measurements of ten SQUIDs with systematically varied geometries and show that
alpha increases as the temperature is lowered; in so doing, each spectrum pivots about a nearly constant frequency. The mean square flux noise, inferred by integrating the power spectra, grows rapidly with temperature and at a given temperature is approximately independent of the outer dimension of a given SQUID washer. We show that these results are incompatible with a model based on the random reversal of independent, spins that are located at the surface of the SQUID washer.In the course of our flux noise measurements, we became aware of a spurious contribution to low-frequency critical current noise in Josephson junctions---normally attributed to charge trapping in the barrier---arising from temperature instabilities inherent in cryogenic systems. These temperature fluctuations modify the critical current via its temperature dependence. By computing cross-correlations between measured temperature and critical current noise in Al-AlOx-Al junctions, we show that, despite excellent temperature stability, temperature fluctuations induce observable critical current fluctuations. Particularly, because
1/f critical current noise has decreased with improved fabrication techniques in recent years, it is important to understand and eliminate this additional noise source.Next, we introduce a numerical method of calculating the mean square flux noise
Phisq from independently fluctuating spins on the surface of thin-film loops of arbitrary geometry. By reciprocity,
Phisq is proportional to
langleBbf(rbf)2rangle, where
Bbf(rbf) is the magnetic field generated by a circulating current around the loop and
rbf varies over the loop surface. By discretizing the loop nonuniformly, we efficiently and accurately compute the current distribution and resulting magnetic field, which may vary rapidly across the loop. We use this method to compute
Phisq in a number of scenarios in which we systematically vary physical parameters of the loop. We compare our simulations to an earlier analytic result predicting that
PhisqproptoR/W in the limit where the loop radius
R is much greater than the linewidth
W. We further show that the previously neglected contribution of edge spins to
Phisq is significant---even dominant---in narrow-linewidth loops.To calculate theoretical dephasing rates in qubits, we consider flux noise with a spectral density
SPhi(f)=A2/(f/1 hboxHz)alpha, where
A is of the order of 1~
muPhi0,hboxHz−1/2 and
0.6leqalphaleq1.2;
Phi0 is the flux quantum. For a qubit with an energy level splitting linearly coupled to the applied flux, our calculations of the dependence of the pure dephasing time
tauphi of Ramsey and echo pulse sequences on
alpha for fixed
A show that
tauphi decreases rapidly as
alpha is reduced. We find that
tauphi is relatively insensitive to the noise bandwidth,
f1leqfleqf2, for all
alpha provided the ultraviolet cutoff frequency
f2>1/tauphi. We calculate the ratio
tauphi,E/tauphi,R of the echo (
E) and Ramsey (
R) sequences, and the dependence of the decay function on
alpha and
f2. We investigate the case in which
SPhi(f0) is fixed at the ``pivot frequency''
f0neq1~Hz while
alpha is varied, and find that the choice of
f0 can greatly influence the sensitivity of
tauphi,E and
tauphi,R to the value of
alpha.Finally, we conclude with a brief review of our principal results and conclusions. We also comment on promising avenues of future research.
In this thesis, we first demonstrate that a disordered superconductor with high kinetic inductance can realise a microwave low-loss, non-dissipative circuit element with impedance greater than the quantum resistance. This element, known as a superinductor, can suppress the fluctuations of charge in a quantum circuit.For this purpose, we fabricated and characterised 20 nm thick, 40 nm wide niobium-nitride nanowires and determined the impedance to 6.795 kΩ. We demonstrate internal quality factors Qi = 2.5e4 in nanowire resonators at single photon excitation, which is significantly higher than values reported in devices with similar materials and geometries. Moreover, we show that the dominant dissipation in our nanowires is not an intrinsic property of the disordered films, but can instead be fully understood within the framework of two-level systems.To further characterise these losses, we then explore the geometrical scaling, toward nanowire dimensions, of dielectric losses in superconducting microwave resonators fabricated with the same techniques and from the same NbN thin-film as the nanowire superinductors. For this purpose, we perform an experimental and numerical study of dielectric loss at low temperatures. Using 3D finite-element simulation of the Maxwell--London equations, we compute the geometric filling factors of the lossy regions in our resonator structures and fit the experimental data to determine the intrinsic loss tangents of its interfaces and dielectrics. Finally, we study the effect of two-level systems on the performance of various superconducting quantum circuits. For this purpose, we measure coherence-time fluctuations in qubits and frequency fluctuations in resonators. In all devices, through statistical analysis, we identify the signature of individual Lorentzian fluctuators in the noise. We find that fluctuations in qubit relaxation are local to the qubit and are caused by instabilities of near-resonant two-level-systems. Furthermore, when examining the low-frequency noise of three different types of superconducting resonator - one NbN nanowire, one Al coplanar waveguide, and one Al 3D cavity - we observe a similar power-law dependence of the Lorentzian switching time and amplitude on the circulating power in the resonators, suggesting a common noise mechanism in the three different types of devices.
Abstract Superconducting quantum circuits are a leading platform for quantum-information processing, but their development requires expertise spanning device design, microfabrication, cryogenic operation, microwave control, and quantum characterization. In this work, we report the realization of a flux-tunable superconducting transmon platform and present an integrated workflow encompassing design, fabrication, measurement, and numerical modeling. The device consists of an
Al/AlOx/Al transmon coupled to a three-dimensional microwave cavity operating in the circuit quantum electrodynamics (cQED) dispersive regime. Two-tone spectroscopy reveals a fundamental transition frequency of
ω01=5.0122 GHz and an anharmonicity of
α/2π=−202.4 MHz , corresponding to
EJ/EC≈82.9 . Flux spectroscopy yields a cavity-qubit coupling strength of
g/2π=260 MHz , while the cavity linewidth gives a loaded quality factor of
QL=6127 and a Purcell limit of
T1Purcell≈82 μs . Time-domain measurements yield coherence times of
T1=17.4 μs and
T2∗=5.8 μs . To investigate coherence and dissipation in the device, the experimental observations are analyzed within a Lindblad master-equation framework describing cavity photon loss and thermal excitation, qubit energy relaxation, and pure dephasing processes. Using a set of experimentally extracted parameters, the model reproduces the measured spectroscopic and time-domain observables, providing a quantitative description of the open-system dynamics of the transmon-cavity platform. The analysis shows that the measured coherence is primarily limited by pure dephasing and energy-relaxation processes, whereas thermal excitation plays a minor role under the experimental conditions. Inspired by the broader framework of quantum dissipation in macroscopic quantum systems pioneered by Caldeira and collaborators, this approach enables a quantitative analysis of relaxation and dephasing processes in superconducting quantum circuits. Beyond the characterization of a single device, the present work demonstrates the establishment of the expertise, infrastructure, and experimental workflow required for the design, fabrication, measurement, and modeling of superconducting quantum circuits, contributing to the development of quantum technologies in Brazil and related applications.