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Nanosystems Physics Chemistry Mathematics

Adiabatic conditions for non-stationary optical phase modulation: a non-degenerate case

Andrei Gaidash, E. E. Memekh, George P. Miroshnichenko, Козубов Антон Владимирович

Published Aug 31, 2026• 0 citations
Publisher

Abstract

This work examines a non-stationary phase-modulation process characterized by a time-dependent interaction coefficient, confined to the non-degenerate case. We derive an exact non-adiabatic solution to the time-dependent Schro¨ dinger equation. We then establish the criterion under which adiabatic considerations become valid-specifically, the condition permitting a stationary-state solution to approximate the non-stationary problem. Our results hold for an arbitrary number of interacting modes and an arbitrary photon number.

DOI
10.17586/2220-8054-2026-17-4-482-490

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This work examines a non-stationary phase-modulation process characterized by a time-dependent interaction coefficient, confined to the non-degenerate case. We derive an exact non-adiabatic solution to the time-dependent Schro¨ dinger equation. We then establish the criterion under which adiabatic considerations become valid-specifically, the condition permitting a stationary-state solution to approximate the non-stationary problem. Our results hold for an arbitrary number of interacting modes and an arbitrary photon number.
By stating the adiabatic theorem of quantum mechanics in a clear and rigorous way, we establish a necessary condition and a sufficient condition for its validity, where the latter is obtained employing our recently developed adiabatic perturbation theory. Also, we simplify further the sufficient condition into a useful and simple practical test at the expense of its mathematical rigor. We present results for the most general case of quantum systems, i.e., those with degenerate energy spectra. These conditions are of upmost importance for assessing the validity of practical implementations of non-Abelian braiding and adiabatic quantum computation. To illustrate the degenerate adiabatic approximation, and the necessary and sufficient conditions for its validity, we analyze in depth an exactly solvable time-dependent degenerate problem.
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Generation of Schrödinger cat-like states via degenerate dual pump spontaneous four-wave mixing in a χ(3)χ^{(3)}χ(3) microring resonator
We theoretically investigate the generation of non-Gaussian quantum states, specifically Schrödinger cat-like states (SCLSs), via degenerate dual-pump spontaneous four-wave mixing in a χ(3)χ^{(3)}χ(3)-based microring resonator. By introducing a unitary transformation that exactly decouples the self-phase modulation (SPM) and cross-phase modulation (XPM) terms, we reduce the full nonlinear Hamiltonian to an effective three-mode interaction. The resulting dynamics (decoupled and full Hamiltonians) are studied using the Lindblad master equation, accounting for cavity losses. Unlike semiclassical or parametric approximations, our full quantum mechanical approach explicitly includes quantum pump depletion, which enables the emergence and observation of non-Gaussian features. We compute the Wigner function, photon number distributions, quadrature variances, Fano factor, Schmidt number, and fidelity to characterize the generated states. For the non-dissipative case, we find that the signal mode b^3\hat{b}_3b^3​ or a^3\hat{a}_3a^3​ exhibits clear non-Gaussian features with a structured Wigner function and even-dominated photon number distribution, characteristic of an even coherent state. In the presence of dissipation (γj=0.2γ_j = 0.2γj​=0.2), the interference fringes become faint, odd photon numbers appear, and the fidelity with the ideal state remains high (>0.9>0.9>0.9), indicating robustness. The pump mode b^1\hat{b}_1b^1​ or a^1\hat{a}_1a^1​ remains Gaussian, while both modes display super-Poissonian statistics and entanglement (>2>2>2). Our results demonstrate that degenerate dual-pump spontaneous four-wave mixing in microring resonators is a promising platform for generating and controlling cat-like states under dissipative conditions.