Abstract The intrinsic hybridization of internal and external atomic degrees of freedom in a Kasevich--Chu interferometer enables engineered motional fluctuations to serve as an independent metrological resource while preserving standard-quantum-limit scaling. We develop a unified computational framework, based on quantum and classical Fisher information, for arbitrary uncorrelated motional inputs under both ideal and Doppler-modified atom--light interactions; a hybrid numerical integration scheme makes the highly oscillatory joint population--position calculation tractable. Applied to single-mode motional squeezed states, the framework predicts up to a twofold sensitivity gain over the semiclassical limit for population measurement through an enlarged atomic coherence length. Joint population--position measurement additionally exploits squeezing-induced reshaping of the spatial interference fringes, yielding substantial gains over a broader parameter regime and exceeding threefold in the quantum-enhancement-dominated regime. This enhancement remains robust to Doppler-induced pulse imperfections under strong momentum broadening and finite spatial resolution, while an optimal squeezing strength emerges from the competition between quantum enhancement and Doppler-induced suppression. Our results establish external motional fluctuations as a robust and underexplored single-particle resource for quantum-enhanced atom interferometry and provide a basis for extensions to correlated many-body systems.
Abstract The intrinsic hybridization of internal and external atomic degrees of freedom in a Kasevich--Chu interferometer enables engineered motional fluctuations to serve as an independent metrological resource while preserving standard-quantum-limit scaling. We develop a unified computational framework, based on quantum and classical Fisher information, for arbitrary uncorrelated motional inputs under both ideal and Doppler-modified atom--light interactions; a hybrid numerical integration scheme makes the highly oscillatory joint population--position calculation tractable. Applied to single-mode motional squeezed states, the framework predicts up to a twofold sensitivity gain over the semiclassical limit for population measurement through an enlarged atomic coherence length. Joint population--position measurement additionally exploits squeezing-induced reshaping of the spatial interference fringes, yielding substantial gains over a broader parameter regime and exceeding threefold in the quantum-enhancement-dominated regime. This enhancement remains robust to Doppler-induced pulse imperfections under strong momentum broadening and finite spatial resolution, while an optimal squeezing strength emerges from the competition between quantum enhancement and Doppler-induced suppression. Our results establish external motional fluctuations as a robust and underexplored single-particle resource for quantum-enhanced atom interferometry and provide a basis for extensions to correlated many-body systems.
Hybridization of internal and external atomic degrees of freedom in a Kasevich-Chu interferometer enables the possibility to enhance the sensitivity significantly even under quantum-standard limit. By introducing motional squeezing state as an input, we systematically derive the computational framework of quantum and classical Fisher information of two measurement protocols for arbitrary strength of Doppler effects. Through maximizing the corresponding classical Fisher information, we obtain the optimal control parameters and the corresponding quantum Fisher information. For population measurement, the largest sensitivity can be as large as four times than the semi-classical limit through enlarging the atom coherence length. For joint measurement of population and position, the competition between quantum enhancement and Doppler suppression induces two three behaviors, in one regime, the quantum enhancement dominates even in presence of strong Doppler broadening effects where the sensitivity is significantly enhanced; while in another regime, an optimal squeezing parameter is observed where the classical Fisher information reaches the maximum. Our results clearly demonstrate the robustness of external quantum enhancement against Doppler suppression. Our proposal can be readily applied to gravimeter of mobile platform where decoherence from noise will damage the many-body entanglement of internal spin squeezing.
Ultra-cold atoms are highly sensitive to both inertial effects and electromagnetic fields, making atom interferometers excellent candidates for a variety of precision sensing applications. Furthermore, highly tunable atomic interactions combined with well established experimental techniques for trapping, cooling and manipulating ensembles of ultra-cold atoms, make them well suited to quantum enhancement. For these reasons, ensembles of ultra-cold atoms are excellent candidates for quantum-enhanced measurement devices. Broadly, this thesis presents a number of theoretical results which share the aim of progressing the proof-of-principle regime of current experiments to genuinely useful, ultra-precise quantum enhanced sensors.In Chapter 4 we explore the challenge of devising a useful, quantum-enhanced inertial measurement - to date no such experiment has been performed. Specifically, we present a model of a spin-squeezed rotation sensor utilising the Sagnac effect in a spin-1 Bose-Einstein condensate in a ring trap. The two input states for the interferometer are seeded using Raman pulses with Laguerre-Gauss beams and are amplified by the bosonic enhancement of spin-exchange collisions, resulting in spin-squeezing and potential quantum enhancement in the interferometry. The ring geometry has an advantage over separated beam path atomic rotation sensors due to the uniform condensate density. We model the interferometer both analytically and numerically for realistic experimental parameters and find that significant quantum enhancement is possible. However, this enhancement is partially degraded when working in a regime with strong atomic interactions, indicating that perhaps interaction-based squeezing is not the best route to a quantum-enhanced inertial measurement.Continuing the theme of practical spin-squeezing with atomic interactions, in Chapter 5 we explore methods to combat detection noise, which is currently one of the most significant experimental limitations for quantum-enhanced atom interferometers. A useful quantum-enhanced interferometer requires nonclassical states with a high particle number and the (close to) optimal exploitation of the states' quantum correlations. Unfortunately, the single-particle detection resolution demanded by conventional protocols, such as spin squeezing via one-axis twisting, places severe limits on the particle number. Additionally, the challenge of finding optimal measurements (that saturate the quantum Cram´er-Rao bound) for an arbitrary nonclassical state limits most metrological protocols to only moderate levels of quantum enhancement. “Interaction-based readout” protocols have been shown to allow optimal interferometry or to provide robustness against detection noise at the expense of optimality. We prove that one has great flexibility in constructing an optimal protocol, thereby allowing it to also be robust to detection noise. This requires the full probability distribution of outcomes in an optimal measurement basis, which is typically easily-accessible and can be determined from specific criteria we provide. Additionally, we quantify the robustness of several classes of interaction-based readouts under realistic experimental constraints. We determine that optimal and robust quantum metrology is achievable in current spin-squeezing experiments.Macroscopic superposition states (known as spin-cat states in atomic ensembles) achieve the ultimate quantum precision limit. In Chapters 6 and 7 we turn our attention to studying decoherence that arises in creating and manipulating these states. In its simplest form, decoherence occurs when a quantum state is entangled with a second state, but the results of measurements made on the second state are not accessible. As the second state has effectively ``measured the first, in Chapter 6 we argue that the quantum Fisher information is the relevant metric for predicting and quantifying this kind of decoherence. In particular we apply this analysis to studying decoherence imparted on spin-cat states via atom-light interactions, which are an essential process in atom interferometry. We find that, compared to classical atomic states, spin-cat states are highly susceptible to this kind of decoherence. We investigate the required optical field occupation, such that this decoherence is negligible.Finally, in Chapter 7 we explore the deleterious effects of spatial and phase dynamics during the creation of spin-cat states via one-axis twisting in a two-component Bose-Einstein condensate. We simulate the breathing dynamics in 1 spatial dimension, employing the method of Sinatra and Castin, whereby the state is expanded into the Fock basis, with each basis state evolving within the Hartree-Fock approximation. This method is able to capture both multi-mode effects and quantum correlations, which allows us to calculate the quantum Fisher information. We find that so long as the time taken for the condensate to reach a spin-cat state is an integer multiple of the breathing period, it is sometimes possible to realise something extremely close to a spin-cat state, despite significant dynamics. These results indicate that large non-linearities, and the associated speed-up in entangling dynamics, are not fundamentally incompatible with the production of fragile, highly entangled states such as spin-cat states.
Spin squeezing in atomic ensembles enables atom interferometry with sensitivities below the shot-noise limit, but the associated entanglement is highly susceptible to loss, making imperfections in atom optics a central limitation. Bragg diffraction is an established technique for driving transitions between atomic momentum states and enables large-momentum transfer through higher-order diffraction while preserving the internal state. However, it is intrinsically limited by two competing mechanisms: Short light pulses induce parasitic diffraction into off-resonant orders beyond an effective two-level description, while long pulses face velocity selectivity. We derive analytical expressions in a second-quantized framework for the atom optics and phase uncertainty of a Mach-Zehnder interferometer including these effects. We demonstrate that sub-shot-noise scaling is achieved only in a regime of intermediate pulse duration. Furthermore, we show that deleterious effects of higher-order diffraction are partially mitigated by optimizing the input quantum state.
The Einstein-Bohr recoiling-slit gedankenexperiment, a cornerstone of quantum complementarity, has long been constrained by the zero-point fluctuations of the atomic slit -- the spatial Standard Quantum Limit (SQL). Here we transcend this fundamental boundary through active quantum state engineering of a single-atom slit. By implementing a non-adiabatic quench-evolve-quench protocol, we prepare the atomic motion in a squeezed state, dynamically redistributing phase-space uncertainty to suppress which-path information and restore high-visibility interference beyond the static vacuum limit. We report an intrinsic visibility of 0.938−0.008+0.004, violating the SQL (0.819) by over 10 standard deviations, corresponding to 7.6(2) dB of effective squeezing. Our work reveals Kerr-induced non-Gaussian dynamics and reinterprets the traditional interferometer as a powerful tool for continuous-variable Wigner tomography, bridging the gap between quantum foundations and advanced metrology.
Abstract An ensemble of atoms can operate as a quantum sensor by placing atoms in a superposition of two different states. Upon measurement of the sensor, each atom is individually projected into one of the two states. Creating quantum correlations between the atoms, that is entangling them, could lead to resolutions surpassing the standard quantum limit 1–3 set by projections of individual atoms. Large amounts of entanglement 4–6 involving the internal degrees of freedom of laser-cooled atomic ensembles 4–16 have been generated in collective cavity quantum-electrodynamics systems, in which many atoms simultaneously interact with a single optical cavity mode. Here we report a matter-wave interferometer in a cavity quantum-electrodynamics system of 700 atoms that are entangled in their external degrees of freedom. In our system, each individual atom falls freely under gravity and simultaneously traverses two paths through space while entangled with the other atoms. We demonstrate both quantum non-demolition measurements and cavity-mediated spin interactions for generating squeezed momentum states with directly observed sensitivity 3.4−0.9+1.1 3 . 4 − 0.9 + 1.1 dB and 2.5−0.6+0.6 2 . 5 − 0.6 + 0.6 dB below the standard quantum limit, respectively. We successfully inject an entangled state into a Mach–Zehnder light-pulse interferometer with directly observed sensitivity 1.7−0.5+0.5 1 . 7 − 0.5 + 0.5 dB below the standard quantum limit. The combination of particle delocalization and entanglement in our approach may influence developments of enhanced inertial sensors 17,18 , searches for new physics, particles and fields 19–23 , future advanced gravitational wave detectors 24,25 and accessing beyond mean-field quantum many-body physics 26–30 .
Harnessing quantum resources in the atomic external degrees of freedom, particularly matter-wave states with large momentum broadening, holds significant potential for enhancing the sensitivity of Kasevich-Chu atom gravimeters at the standard quantum limit. However, a fully quantum-mechanical investigation of the critical Doppler effect inherent to this approach remains lacking. Employing SU(2) Lie group theory, we derive a generic scalar Riccati equation governing the unitary dynamics of the Rabi model within a linear potential and analyze the Doppler effect's impact on Rabi oscillations because of the strong coupling between the internal and external states. Furthermore, by integrating Fisher information theory, we demonstrate the approximate universality and high metrological gain of phase-rotation measurement protocols under strong Doppler broadening induced by large-momentum width. This theoretical work provides insightful implications for broader generalization, such as extensions to finite-temperature scenarios or multi-pulse sequences, exemplified by the π/2−π−π/2 pulse sequence characteristic of Kasevich-Chu atom gravimeters. Thus this study lays a theoretical foundation for developing high-sensitivity, noise-resistant atom gravimeters that leverage external-state quantum resources.