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Non-classical states in ultra-cold atoms for robust, high precision metrology

Samuel P. Nolan

Published Nov 16, 2018• 1 citation
Publisher

Abstract

Ultra-cold atoms are highly sensitive to both inertial effects and electromagnetic fields, making atom interferometers excellent candidates for a variety of precision sensing applications. Furthermore, highly tunable atomic interactions combined with well established experimental techniques for trapping, cooling and manipulating ensembles of ultra-cold atoms, make them well suited to quantum enhancement. For these reasons, ensembles of ultra-cold atoms are excellent candidates for quantum-enhanced measurement devices. Broadly, this thesis presents a number of theoretical results which share the aim of progressing the proof-of-principle regime of current experiments to genuinely useful, ultra-precise quantum enhanced sensors.In Chapter 4 we explore the challenge of devising a useful, quantum-enhanced inertial measurement - to date no such experiment has been performed. Specifically, we present a model of a spin-squeezed rotation sensor utilising the Sagnac effect in a spin-1 Bose-Einstein condensate in a ring trap. The two input states for the interferometer are seeded using Raman pulses with Laguerre-Gauss beams and are amplified by the bosonic enhancement of spin-exchange collisions, resulting in spin-squeezing and potential quantum enhancement in the interferometry. The ring geometry has an advantage over separated beam path atomic rotation sensors due to the uniform condensate density. We model the interferometer both analytically and numerically for realistic experimental parameters and find that significant quantum enhancement is possible. However, this enhancement is partially degraded when working in a regime with strong atomic interactions, indicating that perhaps interaction-based squeezing is not the best route to a quantum-enhanced inertial measurement.Continuing the theme of practical spin-squeezing with atomic interactions, in Chapter 5 we explore methods to combat detection noise, which is currently one of the most significant experimental limitations for quantum-enhanced atom interferometers. A useful quantum-enhanced interferometer requires nonclassical states with a high particle number and the (close to) optimal exploitation of the states' quantum correlations. Unfortunately, the single-particle detection resolution demanded by conventional protocols, such as spin squeezing via one-axis twisting, places severe limits on the particle number. Additionally, the challenge of finding optimal measurements (that saturate the quantum Cram´er-Rao bound) for an arbitrary nonclassical state limits most metrological protocols to only moderate levels of quantum enhancement. “Interaction-based readout” protocols have been shown to allow optimal interferometry or to provide robustness against detection noise at the expense of optimality. We prove that one has great flexibility in constructing an optimal protocol, thereby allowing it to also be robust to detection noise. This requires the full probability distribution of outcomes in an optimal measurement basis, which is typically easily-accessible and can be determined from specific criteria we provide. Additionally, we quantify the robustness of several classes of interaction-based readouts under realistic experimental constraints. We determine that optimal and robust quantum metrology is achievable in current spin-squeezing experiments.Macroscopic superposition states (known as spin-cat states in atomic ensembles) achieve the ultimate quantum precision limit. In Chapters 6 and 7 we turn our attention to studying decoherence that arises in creating and manipulating these states. In its simplest form, decoherence occurs when a quantum state is entangled with a second state, but the results of measurements made on the second state are not accessible. As the second state has effectively ``measured the first, in Chapter 6 we argue that the quantum Fisher information is the relevant metric for predicting and quantifying this kind of decoherence. In particular we apply this analysis to studying decoherence imparted on spin-cat states via atom-light interactions, which are an essential process in atom interferometry. We find that, compared to classical atomic states, spin-cat states are highly susceptible to this kind of decoherence. We investigate the required optical field occupation, such that this decoherence is negligible.Finally, in Chapter 7 we explore the deleterious effects of spatial and phase dynamics during the creation of spin-cat states via one-axis twisting in a two-component Bose-Einstein condensate. We simulate the breathing dynamics in 1 spatial dimension, employing the method of Sinatra and Castin, whereby the state is expanded into the Fock basis, with each basis state evolving within the Hartree-Fock approximation. This method is able to capture both multi-mode effects and quantum correlations, which allows us to calculate the quantum Fisher information. We find that so long as the time taken for the condensate to reach a spin-cat state is an integer multiple of the breathing period, it is sometimes possible to realise something extremely close to a spin-cat state, despite significant dynamics. These results indicate that large non-linearities, and the associated speed-up in entangling dynamics, are not fundamentally incompatible with the production of fragile, highly entangled states such as spin-cat states.

DOI
10.14264/uql.2018.793

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Ultra-cold atoms are highly sensitive to both inertial effects and electromagnetic fields, making atom interferometers excellent candidates for a variety of precision sensing applications. Furthermore, highly tunable atomic interactions combined with well established experimental techniques for trapping, cooling and manipulating ensembles of ultra-cold atoms, make them well suited to quantum enhancement. For these reasons, ensembles of ultra-cold atoms are excellent candidates for quantum-enhanced measurement devices. Broadly, this thesis presents a number of theoretical results which share the aim of progressing the proof-of-principle regime of current experiments to genuinely useful, ultra-precise quantum enhanced sensors.In Chapter 4 we explore the challenge of devising a useful, quantum-enhanced inertial measurement - to date no such experiment has been performed. Specifically, we present a model of a spin-squeezed rotation sensor utilising the Sagnac effect in a spin-1 Bose-Einstein condensate in a ring trap. The two input states for the interferometer are seeded using Raman pulses with Laguerre-Gauss beams and are amplified by the bosonic enhancement of spin-exchange collisions, resulting in spin-squeezing and potential quantum enhancement in the interferometry. The ring geometry has an advantage over separated beam path atomic rotation sensors due to the uniform condensate density. We model the interferometer both analytically and numerically for realistic experimental parameters and find that significant quantum enhancement is possible. However, this enhancement is partially degraded when working in a regime with strong atomic interactions, indicating that perhaps interaction-based squeezing is not the best route to a quantum-enhanced inertial measurement.Continuing the theme of practical spin-squeezing with atomic interactions, in Chapter 5 we explore methods to combat detection noise, which is currently one of the most significant experimental limitations for quantum-enhanced atom interferometers. A useful quantum-enhanced interferometer requires nonclassical states with a high particle number and the (close to) optimal exploitation of the states' quantum correlations. Unfortunately, the single-particle detection resolution demanded by conventional protocols, such as spin squeezing via one-axis twisting, places severe limits on the particle number. Additionally, the challenge of finding optimal measurements (that saturate the quantum Cram´er-Rao bound) for an arbitrary nonclassical state limits most metrological protocols to only moderate levels of quantum enhancement. “Interaction-based readout” protocols have been shown to allow optimal interferometry or to provide robustness against detection noise at the expense of optimality. We prove that one has great flexibility in constructing an optimal protocol, thereby allowing it to also be robust to detection noise. This requires the full probability distribution of outcomes in an optimal measurement basis, which is typically easily-accessible and can be determined from specific criteria we provide. Additionally, we quantify the robustness of several classes of interaction-based readouts under realistic experimental constraints. We determine that optimal and robust quantum metrology is achievable in current spin-squeezing experiments.Macroscopic superposition states (known as spin-cat states in atomic ensembles) achieve the ultimate quantum precision limit. In Chapters 6 and 7 we turn our attention to studying decoherence that arises in creating and manipulating these states. In its simplest form, decoherence occurs when a quantum state is entangled with a second state, but the results of measurements made on the second state are not accessible. As the second state has effectively ``measured the first, in Chapter 6 we argue that the quantum Fisher information is the relevant metric for predicting and quantifying this kind of decoherence. In particular we apply this analysis to studying decoherence imparted on spin-cat states via atom-light interactions, which are an essential process in atom interferometry. We find that, compared to classical atomic states, spin-cat states are highly susceptible to this kind of decoherence. We investigate the required optical field occupation, such that this decoherence is negligible.Finally, in Chapter 7 we explore the deleterious effects of spatial and phase dynamics during the creation of spin-cat states via one-axis twisting in a two-component Bose-Einstein condensate. We simulate the breathing dynamics in 1 spatial dimension, employing the method of Sinatra and Castin, whereby the state is expanded into the Fock basis, with each basis state evolving within the Hartree-Fock approximation. This method is able to capture both multi-mode effects and quantum correlations, which allows us to calculate the quantum Fisher information. We find that so long as the time taken for the condensate to reach a spin-cat state is an integer multiple of the breathing period, it is sometimes possible to realise something extremely close to a spin-cat state, despite significant dynamics. These results indicate that large non-linearities, and the associated speed-up in entangling dynamics, are not fundamentally incompatible with the production of fragile, highly entangled states such as spin-cat states.
We present a model of a spin-squeezed rotation sensor utilizing the Sagnac effect in a spin-1 Bose-Einstein condensate in a ring trap. The two input states for the interferometer are seeded using Raman pulses with Laguerre-Gauss beams and are amplified by the bosonic enhancement of spin-exchange collisions, resulting in spin-squeezing and potential quantum enhancement of the interferometry. The ring geometry has an advantage over separated beam path atomic rotation sensors due to the uniform condensate density. We model the interferometer both analytically and numerically for realistic experimental parameters and find that significant quantum enhancement is possible, but this enhancement is partially degraded when working in a regime with strong atomic interactions.
Useful quantum metrology requires nonclassical states with a high particle number and (close to) the optimal exploitation of the state's quantum correlations. Unfortunately, the single-particle detection resolution demanded by conventional protocols, such as spin squeezing via one-axis twisting, places severe limits on the particle number. Additionally, the challenge of finding optimal measurements (that saturate the quantum Cramér-Rao bound) for an arbitrary nonclassical state limits most metrological protocols to only moderate levels of quantum enhancement. "Interaction-based readout" protocols have been shown to allow optimal interferometry or to provide robustness against detection noise at the expense of optimality. In this Letter, we prove that one has great flexibility in constructing an optimal protocol, thereby allowing it to also be robust to detection noise. This requires the full probability distribution of outcomes in an optimal measurement basis, which is typically easily accessible and can be determined from specific criteria we provide. Additionally, we quantify the robustness of several classes of interaction-based readouts under realistic experimental constraints. We determine that optimal and robust quantum metrology is achievable in current spin-squeezing experiments.
Quantum Sensors, like atom interferometers (AI), can be employed for high-precision measurements of inertial forces, including their application as gravimeters, gradiometers, accelerometers, and gyroscopes. Their measurement principle relies on ultracold atoms that are prepared in quantum-mechanical superposition states in external degrees of freedom. These states can be prepared by a momentum transfer of a Raman laser. Then the superposition state senses the effect of an inertial force, which induce a corresponding relative phase. The phase is read out by a final coupling which converts the interferometric phase into a atom number difference between the two states. The difference provides an estimate of the interferometric phase and the corresponding quantity of interest. The quantum mechanical noise of the atomic ensemble cause a fundamental uncertainty of this estimation, which I analyze for generic AIs. For small atomic densities, the quantum phase noise of the ensemble limits the interferometric sensitivity. For large densities, quantum number fluctuations generate density fluctuations, which generates phase noise. I show that these two competing effects result in an optimal atom number with a maximal interferometer resolution. Squeezed atomic samples allow for a reduction of the quantum noise of one quantity at the expense of an increased noise along of a conjugate quantity. Phase and number are such quantities which obey to a variant of Heisenberg’s uncertainty principle. Neither phase nor number squeezing can improve the maximal interferometer resolution. As one main result of this thesis, I show how an optimal squeezing in between number and phase squeezing, allows for a fundamental improvement. I evaluate possible experimental paths to implement the proposed protocol. Concepts for a squeezing-enhanced operation of external-degree AIs have not yet been demonstrated. I propose and implement an atomic gravimeter, which is designed to accept spin-squeezed atomic states as input states. The interferometer is designed such that the interferometer couplings are performed in spin space, while the phase accumulation is performed in momentum states. For this interferometer, the squeezed input can be directly obtained from spin dynamics in spinor Bose-Einstein condensates. The main noise contributions in the experiment are analyzed, which results in a factor of 84 above the relevant quantum limit, preventing a squeezing enhancement so far. I outline a suppression of the main noise source, uncontrolled AC Stark shift on the squeezed mode and propose future important applications, including test of spontaneous collapse theories and an improvement of large-scale, high-precision gradiometers.
Atom interferometers measure the relative phase shifts between coherent matter-wave paths that arise from interactions with external fields or inertial forces. Due to their exceptional phase sensitivity, atom interferometers became an essential tool for precision measurements and fundamental physics experiments, finding applications in geodesy, gravimetry, and inertial navigation. However, their measurement precision is limited by quantum projection noise, which arises from the Heisenberg uncertainty principle, preventing the measurement of atomic states with absolute precision. The generation of entanglement between the atoms offers a path to surpass this so-called standard quantum limit, thereby enhancing the interferometer’s phase sensitivity beyond classical measurement bounds. This thesis reports on the development of an atom interferometer experiment designed to realize cavity-mediated, squeezed Mach-Zehnder-type interferometry with ultra-cold 87Rb atoms. The experiment combines cavity-aided spin-squeezing with cavity-mediated Mach-Zehnder interferometry to demonstrate entanglement-enhanced phase sensitivity. The experiment is centered on a triangular optical cavity that mediates all relevant atom-light interactions. The cavity provides optical trapping, spin-squeezing, and Raman beam-splitter operations, enabling to perform interferometry on a continuously trapped atomic ensemble. The thesis elaborates on the fundamental theoretical framework, the cavity design, and the full optical setup, including the detailed configuration of the developed laser stabilization methods. Experimentally, continuous loading methods were explored, resulting in an accumulation of up to 4 × 106 atoms in the dipole trap within a cycle time of 500 ms. The AC Stark shift compensation method developed for continuous loading was further applied for in-trap cooling to 10 µK, and optical pumping for efficient atomic state preparation. Coherent state control was verified via observation of microwave-driven Rabi oscillations, and used to characterize atom-cavity coupling. These presented results establish the experimental groundwork for the future development of cavity-mediated, entanglement-enhanced Mach-Zehnder-type atom interferometry.
Atomic sensors are among the best devices for precision measurements of time, electric and magnetic fields, and inertial forces. However, all atomic sensors that utilise uncorrelated particles are ultimately limited by quantum projection noise, as is already the case for state-of-the-art atomic clocks. This so-called standard quantum limit (SQL) can be overcome by employing entanglement, a prime example being the spin-squeezed states. Spin squeezing can be produced in a quantum non-demolition (QND) measurement of the collective spin, particularly with cavity quantum electrodynamical (cQED) interactions. In this thesis, I present the second-generation trapped-atom clock on a chip (TACC) experiment, where we combine a metrology-grade compact clock with a miniature cQED platform to test quantum metrology protocols at a metrologically-relevant precision level. In a standard Ramsey spectroscopy, the stability of the apparatus is confirmed by a fractional frequency Allan deviation of 6E-13 at 1 s. We demonstrate spin squeezing by QND measurement, reaching 8(1) dB for 1.7E4 atoms, currently limited by decoherence due to technical noise. Cold collisions between atoms play an important role at this level of precision, leading to rich spin dynamics. Here we find that the interplay between cavity measurements and collisional spin dynamics manifests itself in a quantum amplification effect of the cavity measurement. A simple model is proposed, and is confirmed by initial measurements. New experiments in this direction may shed light on the surprising many-body physics in this sytem of interacting cold atoms.
In an ensemble of two-level atoms that can be described in terms of a collective spin, entangled states can be used to enhance the sensitivity of interferometric precision measurements. While non-Gaussian spin states can produce larger quantum enhancements than spin-squeezed Gaussian states, their use requires the measurement of observables that are nonlinear functions of the three components of the collective spin. In this paper we develop strategies that achieve the optimal quantum enhancements using non-Gaussian states produced by a nonlinear one-axis-twisting Hamiltonian, and show that measurement-after-interaction techniques, known to amplify the output signals in quantum parameter estimation protocols, are effective in measuring nonlinear spin observables. Including the presence of the relevant decoherence processes from atomic experiments, we determine analytically the quantum enhancement of non-Gaussian over-squeezed states as a function of the noise parameters for arbitrary atom numbers.