Quantum frequency conversion (QFC) plays a pivotal role in enabling coherent photonic interfaces across disparate quantum systems, serving as a foundation for scalable and interoperable quantum networks. Among various approaches, four-wave mixing (FWM) offers a promising path toward efficient, broadband QFC. In this work, we investigate the feasibility of phase-preserving frequency conversion, a necessary condition for coherent quantum state transfer, by characterizing the spectral phase mapping from input to output fields. We model nonlinear propagation through a gas-filled hollow-core capillary fiber, to demonstrate highly phase-coherent frequency conversion across a broad spectral range, including the infrared to ultraviolet, such as telecom (1550 nm) to visible (516 nm) and deep-UV (308 nm). We further examine how phase-mapping quality and conversion efficiency depend on key system parameters, including the intermediate pulse bandwidth and input pulse energy. Our results reveal optimal operating conditions for achieving future efficient and coherent QFC and provide valuable insights into the nonlinear dynamics underlying FWM-based transduction. These findings lay the groundwork for integrating heterogeneous quantum platforms across widely separated optical bands.
Quantum frequency conversion (QFC) plays a pivotal role in enabling coherent photonic interfaces across disparate quantum systems, serving as a foundation for scalable and interoperable quantum networks. Among various approaches, four-wave mixing (FWM) offers a promising path toward efficient, broadband QFC. In this work, we investigate the feasibility of phase-preserving frequency conversion, a necessary condition for coherent quantum state transfer, by characterizing the spectral phase mapping from input to output fields. We model nonlinear propagation through a gas-filled hollow-core capillary fiber, to demonstrate highly phase-coherent frequency conversion across a broad spectral range, including the infrared to ultraviolet, such as telecom (1550 nm) to visible (516 nm) and deep-UV (308 nm). We further examine how phase-mapping quality and conversion efficiency depend on key system parameters, including the intermediate pulse bandwidth and input pulse energy. Our results reveal optimal operating conditions for achieving future efficient and coherent QFC and provide valuable insights into the nonlinear dynamics underlying FWM-based transduction. These findings lay the groundwork for integrating heterogeneous quantum platforms across widely separated optical bands.
Quantum transduction, which enables the coherent conversion of quantum information between disparate physical platforms, is a cornerstone for realizing scalable and interoperable quantum networks. Among various approaches, parametric frequency mixing processes such as four-wave mixing (FWM) offer a promising pathway toward efficient and low-noise transduction. In this work, we demonstrate the feasibility of coherent quantum state transfer by indirectly verifying high-fidelity wavefunction's phase mapping (>99%) from the input field to the generated output field wave. Using a gas-filled hollow-core capillary fiber, we systematically investigate spectral phase evolution across a broad range, including infrared (IR) to ultraviolet (UV) transitions, as well as conversions from telecom-band (1550 nm) to visible (516 nm) and deep-UV (308 nm) wavelengths. Our results reveal that strong phase coherence can be maintained throughout these diverse conversion regimes. Because quantum properties such as coherence and entanglement are intrinsically encoded in both the amplitude and phase of a photonic wavefunction, preserving spectral phase is essential for faithful quantum information transfer. We further show that efficient and phase-preserving transduction can be achieved by tuning system parameters, offering valuable insights into nonlinear coupling dynamics. These findings establish a promising foundation for advancing FWM-based quantum transduction schemes and open new avenues for integrating heterogeneous quantum systems across wide spectral domains within future quantum communication networks.
In large-area quantum networks based on optical fibers, photons are the fundamental carriers of information as so-called flying qubits. They may also serve as the interconnect between different components of a hybrid architecture, which might comprise atomic and solid-state platforms operating at visible or near-infrared wavelengths, as well as optical links in the telecom band. Quantum frequency conversion is the pathway to change the color of a single photon while preserving its quantum state. Currently, nonlinear crystals are utilized for this process. However, their performance is limited by their acceptance bandwidth, tunability, polarization sensitivity, and undesired background emission. A promising alternative is based on stimulated Raman scattering (SRS) in gases. Here, we demonstrate polarization-preserving frequency conversion in a hydrogen-filled antiresonant hollow-core fiber. This approach holds promises for seamless integration into optical fiber networks and interfaces to single emitters. Disparate from related experiments that employ a pulsed pump field, we here take advantage of two coherent continuous-wave pump fields.
Interconnecting heterogeneous quantum systems is an important step toward realizing the quantum internet. We propose a quantum network hub that interfaces local quantum devices with dense wavelength-division multiplexing (DWDM) networks in the telecom band via quantum frequency conversion (QFC) with frequency-channel selectivity. We show that standard periodically poled lithium niobate waveguides used for QFC exhibit a dispersion sweet spot, for example around the 780 nm band, enabling wide tunability of the pump wavelength while maintaining phase matching. Experimentally, we demonstrate the network hub by implementing a channel-selective and polarization-insensitive QFC from 780 nm to telecom wavelengths around 1540 nm. We achieve a pump tuning range of 2 THz and successfully distribute polarization-encoded single photons into 16 frequency channels on the ITU-T DWDM grid with 25 GHz channel spacing, while preserving the quantum information. These results position the QFC-based hub as a versatile backbone for connecting a wide range of quantum devices, spanning both photonic and matter-based systems, across frequency-multiplexed telecom networks.
Quantum computers are expected to offer significant advantages over classical computers by using quantum mechanical phenomena such as superposition and entanglement. Potential future quantum networks may rely on hybrid architectures that combine the advantages of different qubit platforms. In such networks, quantum information must be transferred between stationary and flying qubits, typically photons. A major challenge, however, is that different quantum systems operate at vastly different wavelengths, making direct interconnection impossible. This challenge is addressed by quantum frequency conversion (QFC), which enables the transfer of quantum information between different spectral regions while preserving the quantum state. Most current QFC approaches employ the second-order nonlinearity of crystals. An alternative approach is based on the third-order nonlinearity of gases. In particular, coherent Raman scattering processes such as coherent Stokes and anti-Stokes Raman scattering (CSRS/CARS) enable polarization-independent, broadband and tunable frequency conversion through virtual energy levels. Within the Cluster of Excellence Matter and Light for Quantum Computing (ML4Q), a hydrogen-filled hollow-core fiber is used to realize continuous-wave CSRS-based frequency conversion. The goal is to convert photons emitted by InAs/GaAs quantum dots at approximately 865 nm into the telecom O-band around 1350 nm, thereby enabling the use of these quantum dots in fiber-based quantum communication networks. In this thesis, the conversion stage evolved from a short gas-cell configuration to a hollow-core fiber system providing interaction lengths of several meters. The development and optimization of the experimental setup, including the selection of laser wavelengths, hollow-core fibers, and the design of custom hydrogen chambers are discussed. A detailed characterization of the frequency-conversion system is performed, focusing on the dependence of the conversion efficiency on pressure, intensity, and interaction length, as well as on polarization and bandwidth. Special attention is given to conversion efficiency compared to optical losses and background contributions, which ultimately limit the performance of the current implementation. The key challenges are identified and potential strategies for future improvements are discussed. The central achievement of this work is the experimental demonstration of quantum-correlation-preserving frequency conversion. Using entangled photon pairs generated by spontaneous parametric down-conversion, the preservation of quantum correlations is verified by comparing the cross-correlation functions before and after the conversion process. This work lays the foundation for further experiments with continuous-wave CSRS-based quantum frequency conversion, including measurements with InAs/GaAs quantum dots.
Efficient quantum frequency conversion (QFC) across large spectral gaps remains a challenge for quantum networking. We theoretically investigate a cascaded QFC in hydrogen-filled hollow-core photonic crystal fiber (HC-PCF) to convert telecom photons (1550 nm) to the visible spectrum (676 nm) via two anti-Stokes Raman shifts. Although simultaneous phase matching is impractical across such a wide window, operating in a high-pressure regime overcomes phase mismatches because the high-gain Raman coherence wave has a shorter spatial extent than the nonlinear coherence length. Maxwell-Bloch simulations show conversion efficiencies exceeding 50%. This approach offers a flexible, low-loss path for integrating disparate quantum technologies in a single fiber platform.
In a fiber-based quantum network, the utilization of the telecom band is crucial for long-distance quantum information (QI) transmission between quantum nodes. However, the near-infrared wavelength is identified as optimal for storing and processing QI through alkaline atoms. Recognizing the challenge of efficiently bridging the frequency gap between atomic quantum devices and telecom fibers while maintaining the QI carried by photons, quantum frequency conversion (QFC) serves as a pivotal quantum interface. In this study, we explore an efficient telecom-band QFC mechanism based on diamond-type four-wave mixing (FWM) with rubidium energy levels. The mechanism enables the conversion of photons between the near-infrared wavelength of 795 nm and the telecom band of 1367 or 1529 nm. Using the Heisenberg-Langevin approach, we optimize conversion efficiency (CE) across varying optical depths while considering quantum noises and present corresponding experimental parameters. Unlike previous works neglecting the applied field absorption loss, our results are more relevant to practical scenarios. Moreover, by employing the reduced-density-operator theory to construct a theoretical framework, we demonstrate that this diamond-type FWM scheme can maintain the quantum characteristics of input photons with high fidelity, such as quadrature variances and photon statistics. Importantly, these properties remain unaffected by vacuum field noise, enabling the system to achieve high-purity QFC. Another significant contribution lies in examining how this scheme impacts QI encoded in photon-number, path, and polarization degrees of freedom. These encoded qubits exhibit remarkable entanglement retention under sufficiently high CE. In the case of perfect CE, the scheme can achieve unity fidelity. This comprehensive exploration establishes a theoretical foundation for the application of the diamond-type QFC scheme based on atomic ensembles in quantum networks, laying essential groundwork for advancing the scheme in distributed quantum computing and long-distance quantum communication.