Quantum transduction, which enables the coherent conversion of quantum information between disparate physical platforms, is a cornerstone for realizing scalable and interoperable quantum networks. Among various approaches, parametric frequency mixing processes such as four-wave mixing (FWM) offer a promising pathway toward efficient and low-noise transduction. In this work, we demonstrate the feasibility of coherent quantum state transfer by indirectly verifying high-fidelity wavefunction's phase mapping (>99%) from the input field to the generated output field wave. Using a gas-filled hollow-core capillary fiber, we systematically investigate spectral phase evolution across a broad range, including infrared (IR) to ultraviolet (UV) transitions, as well as conversions from telecom-band (1550 nm) to visible (516 nm) and deep-UV (308 nm) wavelengths. Our results reveal that strong phase coherence can be maintained throughout these diverse conversion regimes. Because quantum properties such as coherence and entanglement are intrinsically encoded in both the amplitude and phase of a photonic wavefunction, preserving spectral phase is essential for faithful quantum information transfer. We further show that efficient and phase-preserving transduction can be achieved by tuning system parameters, offering valuable insights into nonlinear coupling dynamics. These findings establish a promising foundation for advancing FWM-based quantum transduction schemes and open new avenues for integrating heterogeneous quantum systems across wide spectral domains within future quantum communication networks.
Quantum transduction, which enables the coherent conversion of quantum information between disparate physical platforms, is a cornerstone for realizing scalable and interoperable quantum networks. Among various approaches, parametric frequency mixing processes such as four-wave mixing (FWM) offer a promising pathway toward efficient and low-noise transduction. In this work, we demonstrate the feasibility of coherent quantum state transfer by indirectly verifying high-fidelity wavefunction's phase mapping (>99%) from the input field to the generated output field wave. Using a gas-filled hollow-core capillary fiber, we systematically investigate spectral phase evolution across a broad range, including infrared (IR) to ultraviolet (UV) transitions, as well as conversions from telecom-band (1550 nm) to visible (516 nm) and deep-UV (308 nm) wavelengths. Our results reveal that strong phase coherence can be maintained throughout these diverse conversion regimes. Because quantum properties such as coherence and entanglement are intrinsically encoded in both the amplitude and phase of a photonic wavefunction, preserving spectral phase is essential for faithful quantum information transfer. We further show that efficient and phase-preserving transduction can be achieved by tuning system parameters, offering valuable insights into nonlinear coupling dynamics. These findings establish a promising foundation for advancing FWM-based quantum transduction schemes and open new avenues for integrating heterogeneous quantum systems across wide spectral domains within future quantum communication networks.
Quantum frequency conversion (QFC) plays a pivotal role in enabling coherent photonic interfaces across disparate quantum systems, serving as a foundation for scalable and interoperable quantum networks. Among various approaches, four-wave mixing (FWM) offers a promising path toward efficient, broadband QFC. In this work, we investigate the feasibility of phase-preserving frequency conversion, a necessary condition for coherent quantum state transfer, by characterizing the spectral phase mapping from input to output fields. We model nonlinear propagation through a gas-filled hollow-core capillary fiber, to demonstrate highly phase-coherent frequency conversion across a broad spectral range, including the infrared to ultraviolet, such as telecom (1550 nm) to visible (516 nm) and deep-UV (308 nm). We further examine how phase-mapping quality and conversion efficiency depend on key system parameters, including the intermediate pulse bandwidth and input pulse energy. Our results reveal optimal operating conditions for achieving future efficient and coherent QFC and provide valuable insights into the nonlinear dynamics underlying FWM-based transduction. These findings lay the groundwork for integrating heterogeneous quantum platforms across widely separated optical bands.
In a fiber-based quantum network, the utilization of the telecom band is crucial for long-distance quantum information (QI) transmission between quantum nodes. However, the near-infrared wavelength is identified as optimal for storing and processing QI through alkaline atoms. Recognizing the challenge of efficiently bridging the frequency gap between atomic quantum devices and telecom fibers while maintaining the QI carried by photons, quantum frequency conversion (QFC) serves as a pivotal quantum interface. In this study, we explore an efficient telecom-band QFC mechanism based on diamond-type four-wave mixing (FWM) with rubidium energy levels. The mechanism enables the conversion of photons between the near-infrared wavelength of 795 nm and the telecom band of 1367 or 1529 nm. Using the Heisenberg-Langevin approach, we optimize conversion efficiency (CE) across varying optical depths while considering quantum noises and present corresponding experimental parameters. Unlike previous works neglecting the applied field absorption loss, our results are more relevant to practical scenarios. Moreover, by employing the reduced-density-operator theory to construct a theoretical framework, we demonstrate that this diamond-type FWM scheme can maintain the quantum characteristics of input photons with high fidelity, such as quadrature variances and photon statistics. Importantly, these properties remain unaffected by vacuum field noise, enabling the system to achieve high-purity QFC. Another significant contribution lies in examining how this scheme impacts QI encoded in photon-number, path, and polarization degrees of freedom. These encoded qubits exhibit remarkable entanglement retention under sufficiently high CE. In the case of perfect CE, the scheme can achieve unity fidelity. This comprehensive exploration establishes a theoretical foundation for the application of the diamond-type QFC scheme based on atomic ensembles in quantum networks, laying essential groundwork for advancing the scheme in distributed quantum computing and long-distance quantum communication.
Preserving the underlying statistical properties of light during frequency transduction is essential for interfacing spectrally disparate quantum systems. To do this successfully, the process needs to be highly efficient, broadband and noiseless. Despite significant progress in this field, satisfying all these conditions remains challenging. Recently, molecular modulation-based transduction in hollow-core fibers has emerged as a promising approach, where biphoton correlations were proven to be preserved during frequency up-conversion. However, beyond this previous demonstration of correlation-maintaining conversion, whether molecular modulation can preserve more general statistical properties of light remains experimentally unexplored. Here, we demonstrate the conservation of photon-number statistics during selective frequency transduction by Raman molecular modulation in a hydrogen-filled hollow-core fiber. As a proof of concept, weak 585-nm signals are selectively converted to 773 nm in the near-infrared and to 471 nm in the blue spectral region with near-unity efficiencies. Phase matching between the generated coherence waves and the transitions of interest is achieved through the effective dispersion of the system, enabling independent selection of the frequency up- and down-conversion processes. The preservation of the photon-number statistics of the shifted signals, along with the large frequency shifts, broad tunability and compatibility with quantum-optical fields, provides a versatile fiber-based platform for quantum frequency transduction. In particular, the demonstrated interfacing between visible and near-infrared wavelengths using low pump energies and low gas pressures offers a route towards connecting spectrally distinct quantum systems, including quantum emitters, sensors and atomic quantum memories, within hybrid quantum networks.
In large-area quantum networks based on optical fibers, photons are the fundamental carriers of information as so-called flying qubits. They may also serve as the interconnect between different components of a hybrid architecture, which might comprise atomic and solid-state platforms operating at visible or near-infrared wavelengths, as well as optical links in the telecom band. Quantum frequency conversion is the pathway to change the color of a single photon while preserving its quantum state. Currently, nonlinear crystals are utilized for this process. However, their performance is limited by their acceptance bandwidth, tunability, polarization sensitivity, and undesired background emission. A promising alternative is based on stimulated Raman scattering (SRS) in gases. Here, we demonstrate polarization-preserving frequency conversion in a hydrogen-filled antiresonant hollow-core fiber. This approach holds promises for seamless integration into optical fiber networks and interfaces to single emitters. Disparate from related experiments that employ a pulsed pump field, we here take advantage of two coherent continuous-wave pump fields.
Quantum transduction is essential for the future hybrid quantum networks, connecting devices across different spectral ranges. In this regard, molecular modulation in hollow-core fibers has proven to be exceptional for efficient and tunable frequency conversion of arbitrary light fields down to the single-photon limit. However, insights into this conversion method for quantum light have remained elusive beyond standard semi-classical models. In this Letter, we employ a quantum Hamiltonian framework to characterize the behavior of entanglement during molecular modulation while describing the quantum dynamics of both molecules and photons in agreement with recent experiments. In particular, apart from obtaining analytical expressions for the final opto-molecular states, our model predicts a close correlation between the evolution of the average photon numbers and the transfer of entanglement between the interacting parties. These results will contribute to the development of new fiber-based strategies to tackle the challenges associated with the upcoming generation of lightwave quantum technologies.
Efficient frequency conversion is crucial for interfacing photons with a variety of quantum systems ranging from matter qubits (color centers, quantum dots, atoms), optical fibers, detectors, that often operate at widely different wavelengths. Frequency conversion is also a resource to process quantum information.1, 2 Parametric processes such as sum frequency generation (SFG) and Bragg scattering four wave mixing (BS-FWM) offer a good versatility for such frequency conversion. It is well understood that those nonlinear processes have to be strong enough and satisfy phase matching to achieve a high conversion efficiency. While it is enough to consider those two aspects for moderate conversion efficiency up to 50%, the analysis is a bit more complicated when targeting efficiencies closely approaching unity. We are reviewing the pitfall that must be avoided to indeed reach near unity frequency transduction.