This thesis investigates two largely independent topics in many-body and quantum optical physics. The first concerns the thermalization of classical one-dimensional (1D) gases through three-body collisions, while the second explores collective light–matter interactions in atomic arrays and waveguide quantum electrodynamics, with an emphasis on subradiance, superradiance, and computational methods for many-body dynamics. The first part studies thermalization in dilute classical 1D gases, where conventional twobody collisions cannot establish thermal equilibrium. Using Monte Carlo calculations of the three-body collision kernel together with the Boltzmann equation and molecular dynamics simulations, we characterize the thermalization dynamics for particles interacting through inverse power-law and Lennard–Jones potentials. We show that the Boltzmann and molecular dynamics approaches agree in the dilute limit and derive the thermalization rate for inverse power-law interactions.The second part investigates realistic effects in collective light–matter systems. We first study the influence of finite trapping potentials on subradiant states in atomic arrays coupled through free space or a one-dimensional waveguide. We show that atomic motion fundamentally limits subradiant lifetimes through wavefunction delocalization, recoil heating, and dipole-force-induced motion, leading to decoherence and reduced quantum memory fidelity. These results identify optimal trapping and array configurations for long-lived collective excitations.The final chapters develop theoretical methods for describing photon emission in chiral and symmetric waveguide QED systems. Using higher-order mean-field approximations, we model collective emission in experimentally relevant chiral waveguides, obtaining agreement with recent experiments and deriving analytical expressions for photon statistics. We demonstrate that fourth-order correlations are required to capture the emergence of second-order coherence from a fully inverted state. Finally, in the thermodynamic limit of large atom number and fixed optical depth, we show that a second-order mean-field theory becomes exact, yielding analytical solutions for photon emission statistics in both chiral and symmetric waveguides. We characterize the crossover between enhanced superradiant and subradiant emission, establish the suppression of emission fluctuations in the large-system limit, and clarify the role of finite-size effects in generating nontrivial photon correlations.
This thesis investigates two largely independent topics in many-body and quantum optical physics. The first concerns the thermalization of classical one-dimensional (1D) gases through three-body collisions, while the second explores collective light–matter interactions in atomic arrays and waveguide quantum electrodynamics, with an emphasis on subradiance, superradiance, and computational methods for many-body dynamics. The first part studies thermalization in dilute classical 1D gases, where conventional twobody collisions cannot establish thermal equilibrium. Using Monte Carlo calculations of the three-body collision kernel together with the Boltzmann equation and molecular dynamics simulations, we characterize the thermalization dynamics for particles interacting through inverse power-law and Lennard–Jones potentials. We show that the Boltzmann and molecular dynamics approaches agree in the dilute limit and derive the thermalization rate for inverse power-law interactions.The second part investigates realistic effects in collective light–matter systems. We first study the influence of finite trapping potentials on subradiant states in atomic arrays coupled through free space or a one-dimensional waveguide. We show that atomic motion fundamentally limits subradiant lifetimes through wavefunction delocalization, recoil heating, and dipole-force-induced motion, leading to decoherence and reduced quantum memory fidelity. These results identify optimal trapping and array configurations for long-lived collective excitations.The final chapters develop theoretical methods for describing photon emission in chiral and symmetric waveguide QED systems. Using higher-order mean-field approximations, we model collective emission in experimentally relevant chiral waveguides, obtaining agreement with recent experiments and deriving analytical expressions for photon statistics. We demonstrate that fourth-order correlations are required to capture the emergence of second-order coherence from a fully inverted state. Finally, in the thermodynamic limit of large atom number and fixed optical depth, we show that a second-order mean-field theory becomes exact, yielding analytical solutions for photon emission statistics in both chiral and symmetric waveguides. We characterize the crossover between enhanced superradiant and subradiant emission, establish the suppression of emission fluctuations in the large-system limit, and clarify the role of finite-size effects in generating nontrivial photon correlations.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
Waveguide quantum electrodynamics (WQED) offers a powerful framework for controlling light-matter interactions and realizing collective phenomena such as super- and subradiance. In general waveguide settings, the quantum dynamics spans the full Hilbert space, rendering exact theoretical treatments exponentially difficult and currently out of reach, and only a few models have exact, analytical solutions. Motivated by recent experiments, we treat the thermodynamic limit of the number of atoms, N→∞, while the homogeneous atom-waveguide coupling β→0 keeping the optical depth 4Nβ fixed. In this limit, a second order mean field method is exact, giving analytical solutions for the statistics of the photons emitted in the waveguide both for chiral and symmetric configurations starting from full inversion. As N→∞, the emission in freespace approaches that of an independent ensemble. However, until a special time, ≈1.59× the lifetime of a single-atom, we show an exponentially enhanced superradiance in the waveguide as the optical depth increases. After the special time, the emission into the waveguide exhibits subradiance. We also show that the initial shot-to-shot fluctuations in the rate of emission into the waveguide diminish in a chiral system and vanish in a symmetric system as N approaches ∞. Additionally, the equal-time second-order correlation becomes trivial, showing that finite-size effects are essential to observe the emergence of second-order coherence. Finally, going beyond the thermodynamic limit requires higher order mean field methods. Our results illustrate finite- and infinite-body collective effects in symmetric and symmetry-lacking systems.
Waveguide Quantum Electrodynamics (WQED) offers a suitable stage for controlling the interaction of light with atoms, allowing for collective phenomena such as super- and subradiance. In a chiral waveguide setup, the quantum state evolves through all the Hilbert space, rendering an exact theoretical treatment exponentially hard and unobtained to date for more than ∼20 atoms. In this work, we use a computationally efficient higher order mean-field approximation to model the radiation dynamics in a chirally coupled array of atoms, showing good agreement with recent experimental results. Further, based on a perturbative approximation of the full dynamics, we develop an analytical solution that captures photon statistics for a moderate atom number, N, and a homogeneous atom-waveguide coupling, β. Finally, we show that capturing the onset of second-order coherence from a fully inverted state requires a fourth-order mean-field approximation, as lower-order treatments fail to account for the necessary four-body correlations. These results illustrate the complex behavior of a symmetry-lacking system, and the methods discussed here provide systematic analytical solutions to which semi-classical methods such as the cumulant expansion or the truncated Wigner approximation can be benchmarked.
Superradiance and subradiance are collective effects that emerge from coherent interactions between quantum emitters. Due to their many-body nature, theoretical studies of extended samples with length larger than the atomic transition wavelength are usually restricted to their early-time behavior or to the few-excitation limit. We use herein a mean-field approach to reduce the complex many-body system to an effective two-atom master equation that includes all correlations up to second order and that can be numerically propagated in time. We find that three-dimensional and two-dimensional inverted atomic arrays sustain superradiance below a critical lattice spacing and quantify the scaling of the superradiant peak for both dimensionalities. Finally, we study the late-time dynamics of the system and demonstrate that a subradiant phase appears before the system finally relaxes.
Collective radiance effects in quantum degenerate systems, such as superradiance and subradiance of a partially inverted ensemble, are shaped by the interplay of spatial confinement and exchange statistics. We investigate this interplay using a purely dissipative field theoretic quartic Lindblad master equation, which captures the nonlinear dynamics of the combined motional and electronic manifolds. This approach captures the interplay between the permutational symmetry of the Lindbladian and the exchange symmetry of the particles, quantifying how bosonic enhancement and Pauli blocking dictate superradiant and subradiant scaling. We identify two distinct routes to distinguishable dynamics: thermal dilution of the initial state at high temperatures and the dynamical breakdown of collective order via recoil induced transport in soft traps. This analysis provides a benchmark for collective emission in quantum-degenerate atomic systems with coupled motional and internal dynamics, such as optical lattice clocks and spinor gases, when dissipation is engineered to control recoil and motional heating.
Coupling between quantum emitters and modes of light is foundational to studies of quantum systems. Coherent interactions between matter and light have greatly advanced the development of quantum technologies. When an ensemble of atoms interacts with light that is confined within a cavity---a resonator for photons---light also mediates atom-atom interactions, leading to collective phenomena that cannot be extrapolated from microscopic behaviors. Understanding how interactions among quantum particles lead to macroscopic phenomena, such as phase transitions and breaking of symmetries, remains a challenge in modern physics. In this dissertation, I present results addressing this challenge in the context of mesoscopic arrays of optical-tweezer-trapped atoms interfaced with a high-finesse optical cavity. In particular, the physics we investigate arises from the collective scattering of light. Utilizing the ability to place atoms with nanometer-scale precision, we engineer superradiant and subradiant states, where control over interference of the emission from multiple atoms leads to collectively enhanced or suppressed amounts of scattered light. Building on this work, we investigate the emergence of optomechanical self-organization, mediated by superradiance in the cavity electromagnetic field. By coupling atoms to the same cavity mode, the atoms exert forces on one another through the exchange of photons, leading them to autonomously order themselves spatially. We characterize mesoscopic fluctuations and their effect on symmetry-breaking dynamics associated with self-organization. Finally, we extend this framework to theoretically investigate how the phase of the atom-cavity coupling can be altered to generate higher symmetries. Our analysis reveals first-order phase transitions and instabilities induced by non-reciprocal forces. Altogether, this work establishes a path towards realizing mesoscopic systems of complex phases of matter in cavity quantum electrodynamics with unprecedented programmability.