Tomography of Electron Quantum States in Phase Space

Thibaut Jullien, P. Roulleau, B. Roche +3 more

Amir H. Tavabi, Alessio D'Errico, Paolo Rosi +10 more

The physical properties of a quantum system, whether pure or mixed, are described fully by its density matrix. Recovery of the density matrix through projective measurements -- referred to as quantum state tomography -- is a cornerstone of quantum optics and metrology. The implementation of this approach in transmission electron microscopy, in particular for the characterisation of an electron beam after inelastic scattering, has remained a longstanding challenge as a result of the complexity of scanning high-dimensional phase spaces, with the number of required measurements growing quadratically with space dimensionality. Here, we introduce a simplified approach by restricting tomography to the electron orbital angular momentum (OAM) subspace. By using an electron optical device known as an OAM sorter, we discretise the phase space into a finite set of measurable states, thus significantly reducing the experimental and computational burden. The resulting measurements suffice to probe essential features of inelastic scattering. We demonstrate the technique by studying the inelastic scattering of a structured electron probe exciting volume plasmons in a carbon film. The combined use of a structured beams and OAM-resolved quantum tomography reveals symmetry-breaking effects and offers insight into the coherence and evolution of the scattered quantum states. Analysis of the diagonalised density matrices further reveals the nature of the induced state transitions, demonstrating the power of the approach for quantum tomography of electron scattering.

Markus Grassl

Ian A. Walmsley, Leon J. Waxer

Emission tomography provides a method for the characterization of quantum states of those degrees of freedom of material quantum systems that are coupled to electronic states of the system. In such systems, the time-dependent fluorescence spectrum contains complete information about the non-electronic degree of freedom. Phase-space or, in certain cases, density matrix representations of the state can be reconstructed from the spectrum using standard methods of computer-assisted tomography or linear algebra. The principles and implementation of this procedure are described in detail and applied to the specific example of the reconstruction of the quantum state of the vibrational mode of a diatomic molecule excited into a non-stationary wavepacket state.

J. D. Fletcher, Nathan Johnson, Elina Locane +7 more

Initializing and measuring the wave-function of single freely-propagating particles are challenging but fundamental tasks for applications in quantum information processing and enhanced sensing. Recently, continuous-variable quantum tomography techniques developed for atomic beams and photonic modes have been adapted for on-demand electronic excitations but are limited to the region in energy-time phase space immediately around the Fermi level. Here we present a general, broad-band method for mapping the single-particle phase space Wigner distribution. We reconstruct the Wigner representation of the mixed-state density matrix for \textit{solitary} electrons emitted by an on-demand source. This reveals highly localised distributions isolated from the Fermi sea. Our method can be used to test the degree of `quantumness' of an electron source from measurements of the phase-space density. While both source purity and detector fidelity are suppressed by classical fluctuations, here we resolve fine structure of the wavepackets (a chirp controlled by emission conditions) and find that the resolution should be sufficient to enable quantum-limited measurements. Our technique will provide key information required to master electron coherence and entanglement at the individual particle level, for instance to create excitations from multiple sources that are indistinguishable.

Jeff S. Lundeen, Alejandro Feito, Hendrik B. Coldenstrodt-Ronge +6 more