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arXiv:2607.29565

Quantum tomography of inelastic electron scattering \emph{via} orbital angular momentum states

Amir H. Tavabi, Alessio D'Errico, Paolo Rosi, Giovanni Bertoni, Enzo Rotunno, Luca Belsito, Alberto Roncaglia, Stefano Frabboni, Gian Carlo Gazzadi, Peter Tiemeijer, Rafal E. Dunin-Borkowski, Ebrahim Karimi, Vincenzo Grillo

quant-phSubmitted Jul 31, 2026• Announced Aug 3, 2026

Abstract

The physical properties of a quantum system, whether pure or mixed, are described fully by its density matrix. Recovery of the density matrix through projective measurements -- referred to as quantum state tomography -- is a cornerstone of quantum optics and metrology. The implementation of this approach in transmission electron microscopy, in particular for the characterisation of an electron beam after inelastic scattering, has remained a longstanding challenge as a result of the complexity of scanning high-dimensional phase spaces, with the number of required measurements growing quadratically with space dimensionality. Here, we introduce a simplified approach by restricting tomography to the electron orbital angular momentum (OAM) subspace. By using an electron optical device known as an OAM sorter, we discretise the phase space into a finite set of measurable states, thus significantly reducing the experimental and computational burden. The resulting measurements suffice to probe essential features of inelastic scattering. We demonstrate the technique by studying the inelastic scattering of a structured electron probe exciting volume plasmons in a carbon film. The combined use of a structured beams and OAM-resolved quantum tomography reveals symmetry-breaking effects and offers insight into the coherence and evolution of the scattered quantum states. Analysis of the diagonalised density matrices further reveals the nature of the induced state transitions, demonstrating the power of the approach for quantum tomography of electron scattering.

Comments: 9 pages, 3 figure and is accompanied by Supplementary Information

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The physical properties of a quantum system, whether pure or mixed, are described fully by its density matrix. Recovery of the density matrix through projective measurements -- referred to as quantum state tomography -- is a cornerstone of quantum optics and metrology. The implementation of this approach in transmission electron microscopy, in particular for the characterisation of an electron beam after inelastic scattering, has remained a longstanding challenge as a result of the complexity of scanning high-dimensional phase spaces, with the number of required measurements growing quadratically with space dimensionality. Here, we introduce a simplified approach by restricting tomography to the electron orbital angular momentum (OAM) subspace. By using an electron optical device known as an OAM sorter, we discretise the phase space into a finite set of measurable states, thus significantly reducing the experimental and computational burden. The resulting measurements suffice to probe essential features of inelastic scattering. We demonstrate the technique by studying the inelastic scattering of a structured electron probe exciting volume plasmons in a carbon film. The combined use of a structured beams and OAM-resolved quantum tomography reveals symmetry-breaking effects and offers insight into the coherence and evolution of the scattered quantum states. Analysis of the diagonalised density matrices further reveals the nature of the induced state transitions, demonstrating the power of the approach for quantum tomography of electron scattering.

Quantum state tomography is an important tool for quantum communication, computation, metrology, and simulation. Efficient quantum state tomography on a high dimensional quantum system is still a challenging problem. Here, we propose a novel quantum state tomography method, auxiliary Hilbert space tomography, to avoid pre-rotations before measurement in a quantum state tomography experiment. Our method requires projective measurements in a higher dimensional space that contains the subspace that includes the prepared states. We experimentally demonstrate this method with orbital angular momentum states of photons. In our experiment, the quantum state tomography measurements are as simple as taking a photograph with a camera. We experimentally verify our method with near-pure- and mixed-states of orbital angular momentum with dimension up to

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, and achieve greater than 95 % state fidelities for all states tested. This method dramatically reduces the complexity of measurements for full quantum state tomography, and shows potential application in various high dimensional quantum information tasks.

High-dimensional (HD) entanglement enables an encoding of more bits than in the two-dimensional case and promises to increase communication capacity over quantum channels and to improve robustness to noise. In practice, however, one of the central challenges is to devise efficient methods to quantify the HD entanglement explicitly. Full quantum state tomography is a standard technology to obtain all the information about the quantum state, but it becomes impractical because the required measurements increase exponentially with the dimension in HD systems. Hence, it is highly anticipated that a new method will be found for characterizing the HD entanglement with as few measurements as possible and without introducing unwarranted assumptions. Here, we present and demonstrate a scan-free tomography method independent of dimension, which only requires two measurements for the characterization of two-photon HD orbital angular momentum (OAM) entanglement. Taking Laguerre-Gaussian modes of photons as an example, the density matrices of OAM entangled states are experimentally reconstructed with very high fidelity. Our method is also generalized to the mixed HD OAM entanglement. Our results provide realistic approaches for quantifying more complex OAM entanglement in many scientific and engineering fields such as multiphoton HD quantum systems and quantum process tomography.

Abstract Photons carrying orbital angular momentum (OAM) are excellent qudits and are widely used in several applications, such as long distance quantum communication, d -dimensional teleportation and high-resolution imaging and metrology. All these protocols rely on quantum tomography to characterise the OAM state, which currently requires complex measurements involving spatial light modulators and mode filters. To simplify the measurement and characterisation of OAM states, here we apply a recent tomography protocol [Asadian et al , Phys. Rev. A 94 010301 (2016)]. Our scheme for OAM tomography in d dimensions requires only a set of measurements on a path qubit, i.e., a two-dimensional system. This replaces the current complexity of OAM measurements by the ability to perform generalized Pauli operators X d , Z d on OAM states. Our scheme can be adapted in principle to other degrees of freedom, thus opening the way for more complex qudit tomography.

Orbital angular momentum (OAM) of light is a promising degree of freedom for quantum communication and quantum computation. However, efficient methods to transform and measure OAM modes are still not available readily. Here, we propose a method for full quantum state tomography for arbitrary OAM states of light. The key component in our scheme is the helicity sorter, a device that can sort OAM modes of a light beam based on their Helicity. We present two setups to implement the Helicity sorted, one requires

\mathcal{O}(N)

number of optical elements for

2^N

OAM modes, and the other uses spatial light modulators and is independent of the number of OAM modes. Ours is the first method to provide the efficient and scalable full quantum state tomography of the OAM modes and can be extremely important for quantum communication and quantum computation.

While measuring the orbital angular momentum state of bright light beams can be performed using imaging techniques, a full characterization at the single-photon level is challenging. For applications to quantum optics and quantum information science, such characterization is an essential capability. Here, we present a setup to perform the quantum state tomography of photonic qubits encoded in this degree of freedom. The method is based on a projective technique using spatial mode projection via fork holograms and single-mode fibers inserted into an interferometer. The alignment and calibration of the device is detailed as well as the measurement sequence to reconstruct the associated density matrix. Possible extensions to higher-dimensional spaces are discussed.

Determining the quantum state of a given quantum-mechanical system is a fundamental task in physics. Quantum-state tomography has been pivotal for establishing quantum optics [1-4] and for revealing the properties of bound charges in materials [5-7]. An emerging other object for studying and utilizing quantum effects are free electrons, elementary particles that are central to high-resolution microscopy [8,9], electron-based quantum optics [10-17], ul-trafast electron microscopy [18-24] and particle accelerators [25-27]. However, free electrons are intrinsically incoherent, and we lack a broadly applicable method to measure and control their quantum state beyond special cases with discrete energy sidebands [28,29]. Here, we report a universal approach to measure arbitrary free-electron quantum states in continuous variables. Two monochromatic but spectrally shifted laser waves produce interfering quan-tum paths that directly reveal the density matrix and thus all essential properties of the pure wavepackets, the ensemble, and their interlinks. As a first application, we show how the quantum state of a single electron is modified by many-body Coulomb interactions of a sur-rounding electron gas. The reported concepts and results provide insight into otherwise hid-den correlations in electron beams and enable the controlled optimization of exceptional quantum states for free-electron quantum optics or quantum electron microscopy.