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Physical Review A

Generation and control of high-order harmonics in a cesium-atom magnetic-resonance system under strong radio-frequency driving

Ao-dong Xie, Xu‐xing Geng, Wangwang Tang, Yan Yan, Su-jing Liu, Hui Huang, Yang Guo-Qing, Guangming Huang, Gao‐xiang Li

Published Jul 9, 2026• 0 citations
Publisher
DOI
10.1103/j8rl-7th8

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The magnetic-resonance lines of alkali atoms are broadened considerably by the spin-exchange collisions for a radio-frequency magnetometer operating at high temperature. The resonance linewidths of cesium atoms are derived by solving the relaxation equations. When spin-exchange relaxation dominates, a light narrowing effect is predicted. For the cesium atomic radio-frequency magnetometer operates at high temperature, a remarkable narrowing of the cesium magnetic-resonance lines are observed by increasing the pump power. The Cs-Cs spin-exchange relaxation is partially suppressed by light narrowing. This study helps to expand the applications of radio-frequency magnetometers in the high-sensitivity radio-frequency magnetic-field detection.
A longitudinal radio-frequency (rf) magnetic field resonating at the Larmor frequency along the $\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{z}$ direction in the presence of a static transverse magnetic field s investigated. Optical-radio-frequency double resonance in 85Rb^{85}\mathrm{Rb}85Rb characterizes the strength of an external magnetic field through the precession frequency of 85Rb^{85}\mathrm{Rb}85Rb atoms. The measurements are carried out in a paraffin-coated 85Rb^{85}\mathrm{Rb}85Rb cell with a spin alignment configuration. An intriguing discovery of magnetic resonance peaks is observed at subharmonics of the Larmor frequency, accompanied by the emergence of nonlinear effects in the vicinity of the resonance. Notably, when the Larmor frequency reaches zero, the optical rotation signals induced by the rf magnetic field demonstrate a superposition of high-order harmonics of the rf frequency. Based on the simplified density matrix formalism and perturbation treatment, analytical expressions for the optical rotation are consistent with experimental outcomes. These findings hold the potential of extending our understanding on unveiling the dynamics of population and coherence among Zeeman sublevels, thereby advancing our knowledge in the field of alignment magnetometry.