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Physical Review A

Origins of the intrinsic noise of zero-field metastable helium-4 optically pumped magnetometers

Alexandre Stathopulos, Rudy Romain, Sergey I. Mitryukovskiy, Agustin Palacios-Laloy

Published Jul 7, 2026• 0 citations
Publisher
DOI
10.1103/m7zt-mmr1

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Introduction Shortly after the inception of atomic magnetometry, alkali-vapor magnetometers were being used to measure the Earth's magnetic field to unprecedented precision. During the same era, Bell and Bloom first demonstrated all-optical atomic magnetometry through synchronous optical pumping [1] (see Chapters 1 and 6). In this approach, optical-pumping light is frequency- or amplitude-modulated at harmonics of the Larmor frequency ω L to generate a precessing spin polarization within an alkali vapor at finite magnetic field [2, 3]. Although this technique received considerable attention from the atomic physics community for its applicability to optical pumping experiments, Earth's-field alkali-vapor atomic magnetometers continued to rely on radiofrequency (RF) field excitation for several decades (see Chapter 4). Upon the advent of diode lasers addressing alkali and metastable helium transitions, synchronously pumped magnetometers experienced a revival beginning in the late 1980s. In recent years, such magnetometers have found applications in nuclear magnetic resonance detection [4] (see also Chapter 14), quantum control experiments [5], and chip-scale devices intended for spacecraft use [6] (see also Chapters 7 and 15). All-optical magnetometers possess several advantages over devices that employ RF coils. RF-driven magnetometers can suffer from cross-talk if two sensors are placed in close proximity, since the AC magnetic field driving resonance in one vapor cell can adversely affect the other. All-optical magnetometers are free from such interference. When operated in self-oscillating mode [7], RF-driven magnetometers require an added ±90° electronic phase shift in the feedback loop to counter the intrinsic phase shift between the RF field and the probe-beam modulation.

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Quantum sensing has appeared as a promising technique to push the sensitivities of sensors to inherent classical physical limitations. In particular, quantum magnetometers opens the possibilities of new range of applications where extreme sensitivities are needed. A zero field Optically Pumped Magnetometer (OPM), coupled to a conical magnetic guide (MG) is known as a promising technique to improve the spatial resolution of the sensor. This coupling, though, can produce disturbances in the optimal sensing point. In this work a set of compensating coils is designed to reduce the impact of the magnetic guide in the initial sub-15 $\fT/\sqrt{Hz}$ sensitivity of the commercial QuSpin QZFM. First, the system and different strategies are studied theoretically and later implemented experimentally, improving the sensitivity in the OPM-MG by an order of magnitude, from 100 $fT/\sqrt{Hz}$ originally, to 10 $fT/\sqrt{Hz}$.

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Optically pumped magnetometers usually rely on optical pumping using circularly or linearly polarized light. We study here zero-field magnetometers pumped with elliptically polarized light, preparing both atomic orientation and alignment with complementary geometries. We start by extending the three-step approach for elliptically polarized pumping. This allows us to study the Hanle effect in elliptical polarization by comparing the analytical absorption signals with experiments made on 4He^{4}\mathrm{He}4He metastable state. We then study parametric resonance magnetometers based on elliptical polarization by using the dressed-atom formalism with one and two radio-frequency fields. The results show good agreement with the experimental measurements and interesting perspectives for magnetometry where symmetry breaking by pumping light is mitigated.
Introduction Shortly after the inception of atomic magnetometry, alkali-vapor magnetometers were being used to measure the Earth's magnetic field to unprecedented precision. During the same era, Bell and Bloom first demonstrated all-optical atomic magnetometry through synchronous optical pumping [1] (see Chapters 1 and 6). In this approach, optical-pumping light is frequency- or amplitude-modulated at harmonics of the Larmor frequency ω L to generate a precessing spin polarization within an alkali vapor at finite magnetic field [2, 3]. Although this technique received considerable attention from the atomic physics community for its applicability to optical pumping experiments, Earth's-field alkali-vapor atomic magnetometers continued to rely on radiofrequency (RF) field excitation for several decades (see Chapter 4). Upon the advent of diode lasers addressing alkali and metastable helium transitions, synchronously pumped magnetometers experienced a revival beginning in the late 1980s. In recent years, such magnetometers have found applications in nuclear magnetic resonance detection [4] (see also Chapter 14), quantum control experiments [5], and chip-scale devices intended for spacecraft use [6] (see also Chapters 7 and 15). All-optical magnetometers possess several advantages over devices that employ RF coils. RF-driven magnetometers can suffer from cross-talk if two sensors are placed in close proximity, since the AC magnetic field driving resonance in one vapor cell can adversely affect the other. All-optical magnetometers are free from such interference. When operated in self-oscillating mode [7], RF-driven magnetometers require an added ±90° electronic phase shift in the feedback loop to counter the intrinsic phase shift between the RF field and the probe-beam modulation.
Quantum sensing has appeared as a promising technique to push the sensitivities of sensors to inherent classical physical limitations. In particular, quantum magnetometers opens the possibilities of new range of applications where extreme sensitivities are needed. A zero field Optically Pumped Magnetometer (OPM), coupled to a conical magnetic guide (MG) is known as a promising technique to improve the spatial resolution of the sensor. This coupling, though, can produce disturbances in the optimal sensing point. In this work a set of compensating coils is designed to reduce the impact of the magnetic guide in the initial sub-15 $\fT/\sqrt{Hz}$ sensitivity of the commercial QuSpin QZFM. First, the system and different strategies are studied theoretically and later implemented experimentally, improving the sensitivity in the OPM-MG by an order of magnitude, from 100 fT/HzfT/\sqrt{Hz}fT/Hz​ originally, to 10 fT/HzfT/\sqrt{Hz}fT/Hz​.