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Physical Review Letters

Thermodynamics and Melting of a Quantum Quasicrystal

Anonymous, Thomas G. Kiely, Leon Balents, Glenn H. Fredrickson

Published Jul 1, 2026• 0 citations
Publisher

Abstract

A quantum quasicrystal was proposed to exist by mean-field, variational arguments in two-dimensional Rashba spin-orbit coupled BECs with dipolar interactions. Despite this remarkable prediction, there is little known about the superfluid character or stability of this quasicrystalline state against thermal and quantum fluctuations, whose importance is implied by the massive single-particle degeneracy of the Rashba Hamiltonian. Here, we apply field-theoretic numerical simulations based on a boson coherent state path integral representation to simulate the finite-temperature behavior of a periodic approximant of an octagonal quasicrystal. We find that the quasicrystal state maintains a 50% superfluid fraction down to low temperature, suggesting supersolid character. We compute a phase diagram that depicts a region of thermodynamic stability for the octagonal quasicrystal phase at low temperature. At intermediate temperature, the quasicrystal undergoes a first-order transition into a crystalline BEC with hexagonal symmetry. Our findings support a possible experimental realization of the octagonal quasicrystal in ^{164}Dy quantum gases below a temperature of 75 nK.

DOI
10.1103/3646-v33q

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A quantum quasicrystal was proposed to exist by mean-field, variational arguments in two-dimensional Rashba spin-orbit coupled BECs with dipolar interactions. Despite this remarkable prediction, there is little known about the superfluid character or stability of this quasicrystalline state against thermal and quantum fluctuations, whose importance is implied by the massive single-particle degeneracy of the Rashba Hamiltonian. Here, we apply field-theoretic numerical simulations based on a boson coherent state path integral representation to simulate the finite-temperature behavior of a periodic approximant of an octagonal quasicrystal. We find that the quasicrystal state maintains a 50% superfluid fraction down to low temperature, suggesting supersolid character. We compute a phase diagram that depicts a region of thermodynamic stability for the octagonal quasicrystal phase at low temperature. At intermediate temperature, the quasicrystal undergoes a first-order transition into a crystalline BEC with hexagonal symmetry. Our findings support a possible experimental realization of the octagonal quasicrystal in ^{164}Dy quantum gases below a temperature of 75 nK.
We study the emergence of quasicrystal configurations in the ground-state phase diagram of bosonic systems interacting through pair potentials of Lifshitz's type. By using a variational mean-field approach, we determine the relevant features of the corresponding potential interaction kind stabilizing such quasicrystalline states in two dimensions. Unlike their classical counterpart, in which the interplay between only two wave vectors determines the resulting symmetries of the solutions, the quantum picture relates in a more complex way to the instabilities of the excitation spectrum. Moreover, the quantum quasicrystal patterns are found to emerge as the ground state with no need of moderate thermal fluctuations. The study extends to the exploration of the excitation properties and the possible existence of superquasicrystals, i.e., supersolidlike quasicrystalline states in which the long-range nonperiodic density profile coexists with a nonzero superfluid fraction. Our calculations suggest that, in an intermediate region between the homogeneous superfluid and the normal quasicrystal phases, these exotic states indeed exist at zero temperature. Comparison with full numerical simulations provides a solid verification of the variational approach adopted in this paper.
The supersolid phase of soft-core bosons in two dimensions is investigated using the self-consistent Hartree-Fock and quantum Monte Carlo methods. An approximate phase diagram at finite temperatures is initially constructed using the mean-field approach, which is subsequently validated through precise path-integral simulations, enabling a microscopic characterization of the various phases. Superfluid and melting/freezing transitions are analyzed through the superfluid density and the long-range behavior of correlation functions associated with positional and orientational order, in accordance with the general picture of Berezinskii-Kosterlitz-Thouless transitions. A broad region at low temperatures is identified where the supersolid phase exists, separating the uniform superfluid phase from the normal quasicrystal phase. Additionally, a potential intermediate hexatic phase with quasi-long-range orientational order is identified in a narrow region between the normal solid and fluid phases. These findings establish self-consistent Hartree-Fock theory beyond the local density approximation as an effective tool, complementary to computationally intensive quantum Monte Carlo simulations, for investigating the melting of the supersolid phase and the possible emergence of the hexatic superfluid phase in bosonic systems with various interaction potentials.
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We study quasi-two-dimensional dipolar Bose gases in which the bosons experience a Rashba spin-orbit coupling. We show that the degenerate dispersion minimum due to the spin-orbit coupling, combined with the long-range dipolar interaction, can stabilize a number of quantum crystalline and quasicrystalline ground states. Coupling the bosons to a fermionic species can further stabilize these phases. We estimate that the crystalline and quasicrystalline phases should be detectable in realistic dipolar condensates, e.g., dysprosium, and discuss their symmetries and excitations.
We determine the finite-temperature phase diagram of two-dimensional bosons with two hyperfine (pseudospin) states coupled via a Rashba-Dresselhaus spin-orbit interaction using classical field Monte Carlo calculations. For anisotropic spin-orbit coupling, we find a transition to a Berezinskii-Kosterlitz-Thouless superfluid phase with quasi-long-range order. We show that the spin order of the quasicondensate is driven by the anisotropy of the interparticle interaction, favoring either a homogeneous plane-wave state or stripe phase with broken translational symmetry. Both phases show characteristic behavior in the algebraically decaying spin-density correlation function. For a fully isotropic interparticle interaction, our calculations indicate a fractionalized quasicondensate where the mean-field degeneracy of the plane-wave and stripe phase remains robust against critical fluctuations. In the case of fully isotropic spin-orbit coupling, the circular degeneracy of the single-particle ground state destroys the algebraic ordered phase in the thermodynamic limit, but a crossover remains for finite-size systems.
We study the emergence of Bose glass phases in self sustained bosonic quasicrystals induced by a pair interaction between particles of Lifshitz–Petrich type. By using a mean-field variational method designed in momentum space as well as Gross–Pitaevskii simulations we determine the phase diagram of the model. The study of the local and global superfluid fraction allows the identification of supersolid, super quasicrystal, Bose glass and insulating phases. The Bose glass phase emerges as a quasicrystal phase in which the global superfluidity is essentially zero, while the local superfluidity remains finite in certain ring structures of the quasicrystalline pattern. Furthermore, we perform continuous space Path Integral Monte Carlo simulations for a case in which the interaction between particles stabilizes a quasicrystal phase. Our results show that as the strength of the interaction between particles is increased the system undergoes a sequence of states consistent with the super quasicrystal, Bose glass, and quasicrystal insulator thermodynamic phases.