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Supporting Data for the manuscript "Photonic hyperentanglement in polarisation and frequency via joint spectrum shaping"

Tommaso Faleo, Fabian Steinhauser, Gregor Weihs, Stefan Frick, Robert Keil

Published Mar 2, 2026• 1 citation
Publisher

Abstract

Overview This repository contains the complete dataset supporting the experimental results presented in "Photonic hyperentanglement in polarisation and frequency via joint spectrum shaping". Refer to the manuscript for a detailed discussion of the experiment. The dataset includes: Domain engineering of the SPDC crystal Joint spectral intensity (JSI) measurements from time-of-flight spectrometry (TOFS) Biphoton interference measurements, referred here as intra-pair Hong-Ou-Mandel (HOM) interference, of the frequency-entangled state (separable in the polarisation degree of freedom). Heralded two-photon interference measurements, referred here as intra-pair Hong-Ou-Mandel (HOM) interference, of the frequency-entangled state (separable in the polarisation degree of freedom). Polarisation-resolved biphoton interference measurements of the hyperentangled state. Polarisation-resolved TOFS of the hyperentangled state. Folder structure Domain Engineering Frick_UIBKv3.csv contains the domain structure of the KTP crystal: First column: sign (orientation) of the crystal domain Second column: starting position (in um) of the domains Third column: ending position (in um) of the domains. InterPair HOM IndependentHOM_2354_Power14.0mW_Temp23.0C.csv: the file contains heralded two-photon (Hong-Ou-Mandel) interference measurements recorded without the use of spectral filtering (only lowpass filters to cut the pump laser). Measurement procedure: The relative delay between interfering photons is scanned with a translation stage, and single and coincidence events are recorded for 60 seconds for each point with a time-tagging system. Eighteen iterations of the measurement are performed. Content of the file: First row: Position of the translation stage that sets the relative delay between interfering photons in millimetres. Second row: Total four-fold coincidences, for each position, in the heralded two-photon interference. Third to sixth row: Total single counts, for each position, recorded by each channel's detector. Seventh to twenty-fourth row: Four-fold coincidences, for each position, at each iteration of the measurement. IntraPair HOM DependentHOM_2335_Power15.0mW_T80.168C.csv: the file contains intra-pair two-photon (Hong-Ou-Mandel) interference measurements recorded without the use of spectral filtering (only lowpass filters to cut the pump laser), for the frequency-entangled state (separable state in the polarisation degree of freedom). Measurement procedure: The relative delay between interfering photons is scanned with a translation stage, and single and coincidence events are recorded for 20 seconds for each point with a time-tagging system. Content of the file: First row: Position of the translation stage that sets the relative delay between interfering photons in millimetres. Second row: Total two-fold coincidences, for each position, in the two-photon interference. Third to fourth row: Total single counts, for each position, recorded by each channel's detector. Polarisation Resolved Intra Pair HOM The directory contains two folders with intra-pair Hong-Ou-Mandel (HOM) interference measurements of the hyperentangled state. Each folder is associated with a specific input polarisation Bell state, as specified in the folder name ($\psi^{+}$ or $\psi^-$). For each Bell state, measurements are recorded for different pairs of polarisation projection bases (HH, HV, VV, AA, DA, DD) at the two tomography stages connected to the outputs of the fibre beam splitter. Only the HH and DD projections are used in the results presented in the main text; the remaining bases are included for completeness. Setup geometry: Each tomography stage (j=1, 2) is placed at one output of the fibre beam splitter and consists of a quarter-wave plate, a half-wave plate, and a polarising beam splitter (PBS), yielding a transmitted (Tj) and a reflected (Rj) output channel, for a total of four single-photon detector channels. Measurement procedure: The relative temporal delay between the interfering signal and idler photons is scanned with a motorised translation stage, and single-photon counts as well as all coincidence events among the four detector channels are recorded for 20 seconds per delay point using a time-tagging system. Files' structure: File format: .csv files and one .txt file containing the measurement settings. Naming convention: Data_Measurement_Basis_<XX>.csv, where <XX> specifies the pair of polarisation projections at the two tomography stages (e.g., DA denotes a diagonal projection at stage 1 and an anti-diagonal projection at stage 2). Content of the files: Each CSV file contains a header row followed by 99 data rows with 15 columns: Position_mm — Position of the motorised translation stage in millimetres, setting the relative temporal delay between the interfering photons. Counts_T1, Counts_R1, Counts_T2, Counts_R2 — Raw single-photon counts at each of the four detector channels, where the subscript labels the tomography stage and T/R denotes the transmitted/reflected port of the corresponding PBS. Coinc_T1_T2, Coinc_T1_R1, Coinc_T1_R2, Coinc_R1_T2, Coinc_R1_R2, Coinc_T2_R2 — All six pairwise two-fold coincidence counts among the four detectors. These constitute the primary observables of the measurement. Coincidences between detectors belonging to different tomography stages (i.e., different outputs of the fibre beam splitter) — namely T1–T2, T1–R2, R1–T2, and R1–R2 — correspond to anti-bunching (cross-output) events, while coincidences between detectors within the same tomography stage — T1–R1 and T2–R2 — correspond to bunching (same-output) events. Coinc_T1_R1_T2, Coinc_T1_R1_R2, Coinc_T1_T2_R2, Coinc_R1_T2_R2 — All four three-fold coincidence counts. Coinc_T1_R1_T2_R2 — Four-fold coincidence count (all four detectors firing within the coincidence window). All count values are raw (unnormalised) photon detection events accumulated over the 20-second integration time per delay point. The higher-order (three- and four-fold) coincidences are recorded for diagnostic purposes. Polarisation Resolved TOFS The directory contains polarisation-resolved joint spectral intensity measurements of the hyperentangled state obtained via TOFS. The used Bell state is $\phi^+$. Measurements are recorded for different pairs of polarisation projection bases (AA, AD, AH, AL, AR, AV, DA,…) at the two tomography stages connected to the inputs of the dispersion modules of the TOFS. File structure. File format: .csv files and one .txt file containing the measurement settings. Naming convention: JSI_<XX>.csv, where <XX> specifies the pair of polarisation projections at the two tomography stages (e.g., DA denotes a diagonal projection at stage 1 and an anti-diagonal projection at stage 2). Content of the files: Each CSV file contains a two-dimensional matrix with raw, three-fold coincidence events between (1) pulsed pump trigger, (2) signal and (3) idler down-converted photons as a function of trigger-signal delay and trigger-idler delay in picoseconds (see .txt file containing the measurement settings) TOFS Contains Joint Spectral Intensity measurements for three different configurations of the pump spectral shaping: File format: .txt files. Naming convention: JSI_Sagnac_80psBin_<XX>.txt where <XX> specifies the resulting JSI (symmetric 2x2, asymmetric 2x2, asymmetric3x2) from the used shaping configuration. Content: Two-dimensional matrix with raw, three-fold coincidence events between (1) pulsed pump trigger, (2) signal and (3) idler down-converted photons as a function of trigger-signal delay and trigger-idler delay in picoseconds: Delays: first row and first column (ps). Three-folds: all other elements

DOI
10.5281/zenodo.18833942

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Overview This repository contains the complete dataset supporting the experimental results presented in "Photonic hyperentanglement in polarisation and frequency via joint spectrum shaping". Refer to the manuscript for a detailed discussion of the experiment. The dataset includes: Domain engineering of the SPDC crystal Joint spectral intensity (JSI) measurements from time-of-flight spectrometry (TOFS) Biphoton interference measurements, referred here as intra-pair Hong-Ou-Mandel (HOM) interference, of the frequency-entangled state (separable in the polarisation degree of freedom). Heralded two-photon interference measurements, referred here as intra-pair Hong-Ou-Mandel (HOM) interference, of the frequency-entangled state (separable in the polarisation degree of freedom). Polarisation-resolved biphoton interference measurements of the hyperentangled state. Polarisation-resolved TOFS of the hyperentangled state. Folder structure Domain Engineering Frick_UIBKv3.csv contains the domain structure of the KTP crystal: First column: sign (orientation) of the crystal domain Second column: starting position (in um) of the domains Third column: ending position (in um) of the domains. InterPair HOM IndependentHOM_2354_Power14.0mW_Temp23.0C.csv: the file contains heralded two-photon (Hong-Ou-Mandel) interference measurements recorded without the use of spectral filtering (only lowpass filters to cut the pump laser). Measurement procedure: The relative delay between interfering photons is scanned with a translation stage, and single and coincidence events are recorded for 60 seconds for each point with a time-tagging system. Eighteen iterations of the measurement are performed. Content of the file: First row: Position of the translation stage that sets the relative delay between interfering photons in millimetres. Second row: Total four-fold coincidences, for each position, in the heralded two-photon interference. Third to sixth row: Total single counts, for each position, recorded by each channel's detector. Seventh to twenty-fourth row: Four-fold coincidences, for each position, at each iteration of the measurement. IntraPair HOM DependentHOM_2335_Power15.0mW_T80.168C.csv: the file contains intra-pair two-photon (Hong-Ou-Mandel) interference measurements recorded without the use of spectral filtering (only lowpass filters to cut the pump laser), for the frequency-entangled state (separable state in the polarisation degree of freedom). Measurement procedure: The relative delay between interfering photons is scanned with a translation stage, and single and coincidence events are recorded for 20 seconds for each point with a time-tagging system. Content of the file: First row: Position of the translation stage that sets the relative delay between interfering photons in millimetres. Second row: Total two-fold coincidences, for each position, in the two-photon interference. Third to fourth row: Total single counts, for each position, recorded by each channel's detector. Polarisation Resolved Intra Pair HOM The directory contains two folders with intra-pair Hong-Ou-Mandel (HOM) interference measurements of the hyperentangled state. Each folder is associated with a specific input polarisation Bell state, as specified in the folder name (ψ+\psi^{+}ψ+ or ψ−\psi^-ψ−). For each Bell state, measurements are recorded for different pairs of polarisation projection bases (HH, HV, VV, AA, DA, DD) at the two tomography stages connected to the outputs of the fibre beam splitter. Only the HH and DD projections are used in the results presented in the main text; the remaining bases are included for completeness. Setup geometry: Each tomography stage (j=1, 2) is placed at one output of the fibre beam splitter and consists of a quarter-wave plate, a half-wave plate, and a polarising beam splitter (PBS), yielding a transmitted (Tj) and a reflected (Rj) output channel, for a total of four single-photon detector channels. Measurement procedure: The relative temporal delay between the interfering signal and idler photons is scanned with a motorised translation stage, and single-photon counts as well as all coincidence events among the four detector channels are recorded for 20 seconds per delay point using a time-tagging system. Files' structure: File format: .csv files and one .txt file containing the measurement settings. Naming convention: Data_Measurement_Basis_<XX>.csv, where <XX> specifies the pair of polarisation projections at the two tomography stages (e.g., DA denotes a diagonal projection at stage 1 and an anti-diagonal projection at stage 2). Content of the files: Each CSV file contains a header row followed by 99 data rows with 15 columns: Position_mm — Position of the motorised translation stage in millimetres, setting the relative temporal delay between the interfering photons. Counts_T1, Counts_R1, Counts_T2, Counts_R2 — Raw single-photon counts at each of the four detector channels, where the subscript labels the tomography stage and T/R denotes the transmitted/reflected port of the corresponding PBS. Coinc_T1_T2, Coinc_T1_R1, Coinc_T1_R2, Coinc_R1_T2, Coinc_R1_R2, Coinc_T2_R2 — All six pairwise two-fold coincidence counts among the four detectors. These constitute the primary observables of the measurement. Coincidences between detectors belonging to different tomography stages (i.e., different outputs of the fibre beam splitter) — namely T1–T2, T1–R2, R1–T2, and R1–R2 — correspond to anti-bunching (cross-output) events, while coincidences between detectors within the same tomography stage — T1–R1 and T2–R2 — correspond to bunching (same-output) events. Coinc_T1_R1_T2, Coinc_T1_R1_R2, Coinc_T1_T2_R2, Coinc_R1_T2_R2 — All four three-fold coincidence counts. Coinc_T1_R1_T2_R2 — Four-fold coincidence count (all four detectors firing within the coincidence window). All count values are raw (unnormalised) photon detection events accumulated over the 20-second integration time per delay point. The higher-order (three- and four-fold) coincidences are recorded for diagnostic purposes. Polarisation Resolved TOFS The directory contains polarisation-resolved joint spectral intensity measurements of the hyperentangled state obtained via TOFS. The used Bell state is ϕ+\phi^+ϕ+. Measurements are recorded for different pairs of polarisation projection bases (AA, AD, AH, AL, AR, AV, DA,…) at the two tomography stages connected to the inputs of the dispersion modules of the TOFS. File structure. File format: .csv files and one .txt file containing the measurement settings. Naming convention: JSI_<XX>.csv, where <XX> specifies the pair of polarisation projections at the two tomography stages (e.g., DA denotes a diagonal projection at stage 1 and an anti-diagonal projection at stage 2). Content of the files: Each CSV file contains a two-dimensional matrix with raw, three-fold coincidence events between (1) pulsed pump trigger, (2) signal and (3) idler down-converted photons as a function of trigger-signal delay and trigger-idler delay in picoseconds (see .txt file containing the measurement settings) TOFS Contains Joint Spectral Intensity measurements for three different configurations of the pump spectral shaping: File format: .txt files. Naming convention: JSI_Sagnac_80psBin_<XX>.txt where <XX> specifies the resulting JSI (symmetric 2x2, asymmetric 2x2, asymmetric3x2) from the used shaping configuration. Content: Two-dimensional matrix with raw, three-fold coincidence events between (1) pulsed pump trigger, (2) signal and (3) idler down-converted photons as a function of trigger-signal delay and trigger-idler delay in picoseconds: Delays: first row and first column (ps). Three-folds: all other elements
Hong-Ou-Mandel interference between independent photon sources (HOMI-IPS) plays an important role in quantum information processing. A variety of HOMI-IPS experiments have been demonstrated at near-infrared wavelengths or telecom wavelengths [1]. In all the previous HOMI-IPS experiments, the HOM dips are obtained by recording the four-fold coincidence counts as a function of the temporal delay. However, the spectral correlation during the interference is omitted, partially due to technical difficulties, e.g., the acquisition time is too long for measuring a joint spectral distribution. Spectral information, as the conjugate of the temporal information in the Fourier transformation, is definitely of great importance and should be investigated. Very recently, a new technique of spectral correlation measurement in a HOM interference has been developed by Gerrits, et al [2]. This technique has the merits of high speed and high resolution, therefore, has been used as a powerful tool to analyse the spectral correlation in a HOM interference between signal and idler photons from one spontaneous parametric down conversion (SPDC) source. In this work, we measure the joint spectral distribution in HOMI-IPS using the new technique developed in [2]. The experimental setup is shown in Fig. 1 (Left). The two independent sources are based on SPDC from two 30-mm-long periodically poled KTiOPO4 (PPKTP) crystals pumped by picosecond laser pulses (76 MHz, 792 nm, temporal duration ~ 2 ps). In Fig. 1 (Left), the dispersion compensation fiber model (DCFMs), the superconducting nanowire single-photon detectors (SNSPDs) [3,4,5] and the time interval analyzer (TIA) constitute a fiber spectral analyzer [6]. Fig. 1(Right: (a)) is the measured four-fold HOM interference between signal1 and signal2, with idler1 and idler2 as heralders. Without subtraction of any background counts, the raw visibility of the HOM dip is 69.9±3.2%, which is consistent with our previous results in [1,7,8]. Fig. 1(Right: (b)-(g)) are the measured joint spectral intensities at different delay positions. The splitting phenomenon in the joint spectral distribution is clearly observed. The experimental results agree well with our theoretical simulations. This experiment not only can deepen our understanding of HOMI-IPS from the viewpoint of spectral domain, but also can be used to improve the visibility of HOMI-IPS by temporal filtering.
En information quantique, un encodage sur les degrés de liberté temps et fréquence donne accès à un espace de Hilbert de grande dimension pour les états photoniques ce qui autorise le traitement en parallèle d'un grand nombre de qubits voire de qudits. C'est dans ce cadre que se situe cette thèse sur la génération et la manipulation d'états quantiques photoniques aux longueurs d'onde télécom. Nous présentons trois réalisations. La première est la génération efficace de paires de photons par processus non-linéaire du second et du troisième ordre dans des sources intégrées innovantes : un guide en niobate de lithium sur isolant, en couche mince et à inversion de domaines periodique, et un micro-résonateur en silicium sur isolant possédant un intervalle spectral libre de 21 GHz. La deuxième est le développement de concepts, de modèles et d'optimisations numériques pour la manipulation de qubits et qudits photoniques dans les espaces temps fréquence avec des éléments linéaires. Nous utilisons des filtres programmables (PF) et des modulateurs de phase électro-optiques (EOM). Nous comparons les performances théoriques de portes à 1 qubit pour deux configurations de composants [EOM-PF-EOM] et [PF-EOM-PF] dans les deux types d'encodage temps et fréquence. La troisième est la démonstration expérimentale d'une telle manipulation de qubits fréquentiels issus du microrésonateur en Silicium. Nous utilisons la configuration [EOM-PF-EOM] pour implémenter une porte quantique reconfigurable et accordable. Un seul paramètre variable permet de passer d'une porte identité à une porte Hadamard, ainsi qu'à un continuum de portes intermédiaires. Nous démontrons la parallélisation de 34 de ces portes appliquées à 17 états à deux qubits intriqués en fréquence générés par le résonateur. Nous utilisons ensuite ces portes pour réaliser la tomographie quantique des états intriqués et pour mettre en oeuvre un protocole de distribution de clef quantique basé sur l'intrication des deux photons en fréquence. Nous faisons finalement la démonstration inédite d'un réseau multi-utilisateur sans nœuds sécurisés en encodage fréquentiel. Cette expérience constitue une preuve de principe pour la distribution de clé quantique dans le domaine fréquentiel avec un débit de 2 bits par seconde en simultané pour chacune des paires d'utilisateurs dans un réseau de 5 utilisateurs.
Interference between independent photon sources is the key technique to realize complex quantum systems for more sophisticated applications such as multi-photon entanglement generation and quantum teleportation. Here, we report Hong-Ou-Mandel interference (HOMI) between two independent 1.55 m all-fiber photon pair sources over two 100 GHz dense wave division multiplexing (DWDM) channels, whose visibility reaches 53.2%8.4% (82.9%5.3%) without (with) back ground counts subtracted. In addition, we theoretically describe in detail the single photon spectral purity of the photon source generated in dispersion shifted fiber (DSF), simulate the influences of the pulse width and filter bandwidth on the purity, and obtain the optimized condition. The optimized pump pulse width is 8 ps and filter bandwidth is about 40 GHz or less. A home-made 1550.1 nm mode-locked fiber laser source, whose pulse width and repetition rate are 25 ps and 27.9 MHz respectively, acts as a pump of photon source. A tunable attenuator is used to adjust the pump power of the photon source, and the broad band background fluorescence photons are filtered out by cascade 100 GHz DWDM filters. The clean pump beam is divided into two equal parts by the 50 : 50 optical coupler to pump two 300 m DSFs (cooled by liquid nitrogen) to generate independent photon sources. Then the strong pump beam and noise photon from Raman scattering in orthogonal polarization are removed by 2 groups of 200 GHz DWDM filters and fiber polarization rotator and polarizer. Then two 100 GHz DWDMs are used for separating photons at correlated channel pairs. The relative delay between the two independent photons is adjusted by tunable fiber delay line. Photons from the same channels are combined in a second beam splitter for interference, and the other two photons are used as trigger signals. The two triggered photons are detected by two free running InGaAs avalanched single photon detectors (APD1, APD4, ID Quanta, ID220, 20% detection efficiency, 3 s dead time, dark count rate 4k cps), and the outputs of detectors APD1 and APD4 are used to trigger two single-photon detectors running in the gated mode (APD2, APD3, Qasky, Hefei, China, 100 MHz, free gating single photon detectors, 20% detection efficiency, dark count probability 410-5 per gate) for twophoton coincidence measurement. Detection output signals from APD2 and APD3 are sent to our coincidence count device (Pico quanta, TimeHarp 260, 1.6 ns coincidence window) for four-photon coincidence measurement. Before measuring the HOMI, we obtain a maximum-coincidence-to-accidental-coincidence ratio (CAR) of 131 by cooling the fiber in liquid nitrogen when the pump power is 23 W. There are a few remarks we want to point out.Firstly, the photon sources are not operated at the optimized pump pulse width for pure single photon generation, but narrow band 100 GHz filters are used in the experiments to increase the purity of the sources. Secondly, single photon detectors used in our experiment have lower detection efficiency and much higher dark counts than nano-wire single photon detectors, if we have high-performance nano-wire single photon detector, experimental results will be greatly improved due to the four-fold coincidences and dark coincidences scaling quadruplicate with the detection efficiency and dark count probability of a single detector. Thirdly, we use relatively high pump power for each DSF (0.12 mW) to reduce measurement time for photon coincidence, which will lead to a very poor raw visibility certainly. Finally, though only a 100 GHz channel pair is used in our experiment, we can use other channels for multiplexing such interference processes to improve the channel capacity in future quantum communication tasks theoretically. Our study shows greatly promising integrated optical elements for future scalable quantum information processing.
Hyperentanglement offers enhanced capacity for quantum information processing and communication protocols, especially in combination with robust high-dimensional degrees of freedom such as frequency-bin encoding. Here, we present a single-pass, unfiltered, down-conversion source of hyperentangled photon pairs in polarisation and frequency-bin degrees of freedom with dynamically tunable state dimension and composition at telecom wavelengths. We achieve this by optimal tailoring of the photons' joint spectral amplitude via pump and nonlinearity shaping. Using polarisation-resolved time-of-flight spectrometry and Hong-Ou-Mandel interference, we characterise the hyperentangled states and demonstrate for the polarisation component fidelities exceeding 99% averaged over frequency bins and concurrences above 98%. The degree of spectral entanglement, quantified by the Hong-Ou-Mandel visibility, is measured as 90%, well in line with numerical simulations. This approach provides a scalable route toward high-dimensional quantum states for quantum communication and computing applications.
Traitement quantique de l'information dans le domaine des fréquences d'états photoniques quantiques multimodes générés par des sources intégrées aux longueurs d'ondes télécom En information quantique, un encodage sur les degrés de liberté temps et fréquence donne accès à un espace de Hilbert de grande dimension pour les états photoniques ce qui autorise le traitement en parallèle d'un grand nombre de qubits voire de qudits. C'est dans ce cadre que se situe cette thèse sur la génération et la manipulation d'états quantiques photoniques aux longueurs d'onde télécom. Nous présentons trois réalisations. La première est la génération efficace de paires de photons par processus non-linéaire du second et du troisième ordre dans des sources intégrées innovantes : un guide en niobate de lithium sur isolant, en couche mince et à inversion de domaines periodique, et un micro-résonateur en silicium sur isolant possédant un intervalle spectral libre de 21 GHz. La deuxième est le développement de concepts, de modèles et d'optimisations numériques pour la manipulation de qubits et qudits photoniques dans les espaces temps fréquence avec des éléments linéaires. Nous utilisons des filtres programmables (PF) et des modulateurs de phase électro-optiques (EOM). Nous comparons les performances théoriques de portes à 1 qubit pour deux configurations de composants [EOM-PF-EOM] et [PF-EOM-PF] dans les deux types d'encodage temps et fréquence. La troisième est la démonstration expérimentale d'une telle manipulation de qubits fréquentiels issus du microrésonateur en Silicium. Nous utilisons la configuration [EOM-PF-EOM] pour implémenter une porte quantique reconfigurable et accordable. Un seul paramètre variable permet de passer d'une porte identité à une porte Hadamard, ainsi qu'à un continuum de portes intermédiaires. Nous démontrons la parallélisation de 34 de ces portes appliquées à 17 états à deux qubits intriqués en fréquence générés par le résonateur. Nous utilisons ensuite ces portes pour réaliser la tomographie quantique des états intriqués et pour mettre en oeuvre un protocole de distribution de clef quantique basé sur l'intrication des deux photons en fréquence. Nous faisons finalement la démonstration inédite d'un réseau multi-utilisateur sans nœuds sécurisés en encodage fréquentiel. Cette expérience constitue une preuve de principe pour la distribution de clé quantique dans le domaine fréquentiel avec un débit de 2 bits par seconde en simultané pour chacune des paires d'utilisateurs dans un réseau de 5 utilisateurs.