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Science Advances

A chip-scale atomic beam for nonclassical light

B. M. Larsen, Hagan Hensley, Gabriela D. Martinez, Alexander L. Staron, William McGehee, John E. Kitching, James K. Thompson

Published Jun 3, 2026• 2 citations
Publisher

Abstract

Nonclassical light is a critical resource for a broad range of quantum technologies and fundamental science. However, leading platforms such as laser-cooled atoms and solid-state systems both present substantial challenges to scalability due to complexity and spectral drift. Here, we demonstrate a hybrid approach using a chip-scale rubidium beam coupled to a high-finesse cavity-quantum electrodynamics (QED) system. Specifically, we generate nonclassical light and observe optical nonlinearities at the few photon level. This is achieved without degradation of the cavity-QED system. By demonstrating the compatibility of these two technologies, we open a path for distributed sources of nonclassical light and set the stage for using cavity-QED to enhance the performance of chip-scale magnetometers and atomic clocks.

DOI
10.1126/sciadv.aec3179

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Nonclassical light is a critical resource for a broad range of quantum technologies and fundamental science. However, leading platforms such as laser-cooled atoms and solid-state systems both present substantial challenges to scalability due to complexity and spectral drift. Here, we demonstrate a hybrid approach using a chip-scale rubidium beam coupled to a high-finesse cavity-quantum electrodynamics (QED) system. Specifically, we generate nonclassical light and observe optical nonlinearities at the few photon level. This is achieved without degradation of the cavity-QED system. By demonstrating the compatibility of these two technologies, we open a path for distributed sources of nonclassical light and set the stage for using cavity-QED to enhance the performance of chip-scale magnetometers and atomic clocks.
Room temperature thermal atoms have proven to be a powerful resource for magnetometry, electrometry, atom-entanglement generation, and robust atomic clocks. Recent efforts have sought to realize compact and highly manufacturable atomic vapors and atomic beams for chip-scale magnetometry and atomic clocks. Here, we show that a chip-scale rubidium beam source can be integrated with a high finesse cavity-QED system to generate non-classical light. By demonstrating the compatibility of these two technologies, we open a new path for distributed sources of non-classical light and set the stage for using cavity-QED to enhance the performance of chip-scale magnetometers and atomic clocks.
Nonclassical states of light are an essential resource for many emerging quantum technologies and applications ranging from information processing, encrypted communications, and networking to sensing, metrology, and imaging. Nonlinear optical processes in solid-state materials are widely used for generating quantum light, including single photons, entangled-photon pairs, and quadrature-squeezed states. Recent advances in nonlinear photonics have enabled the functionality of benchtop nonlinear instruments to be scaled down to a single chip without sacrificing efficiency or degrading the key performance metrics. The dramatic improvement in the size, weight, power, cost, and stability enabled by photonic integrated circuits has been essential for enabling the chip-scale generation, manipulation, and detection of quantum light at a steadily increasing degree of complexity and scale. Within the last decade, the authors have seen the progression from few-component photonic circuits operating on two photons to arrays of 18 identical heralded single-photon sources and reconfigurable devices operating with more than 650 components for multidimensional entanglement and arbitrary two-photon quantum gates. In this review, the authors summarize the history and recent key technological developments of chip-scale nonlinear quantum light generation based on integrated nonlinear photonics, recent advances in heterogeneous integrated methods, and approaches for system-level integration and demonstrated applications.
The on-chip generation of nonclassical states of light is a key requirement for future optical quantum hardware. In solid-state cavity quantum electrodynamics, such nonclassical light can be generated from self-assembled quantum dots strongly coupled to photonic crystal cavities. Their anharmonic strong light-matter interaction results in large optical nonlinearities at the single photon level, where the admission of a single photon into the cavity may enhance (photon tunneling) or diminish (photon blockade) the probability for a second photon to enter the cavity. Here, we demonstrate that detuning the cavity and quantum-dot resonances enables the generation of high-purity nonclassical light from strongly coupled systems. For specific detunings we show that not only the purity but also the efficiency of single-photon generation increases significantly, making high-quality single-photon generation by photon blockade possible with current state-of-the-art samples.
Underlying matter and light are their building blocks of tiny atoms and photons. The ability to control and utilize matter-light interactions down to the elementary single atom and photon level at the nano-scale opens up exciting studies at the frontiers of science with applications in medicine, energy, and information technology. Of these, an intriguing front is the development of quantum networks where N >> 1 single-atom nodes are coherently linked by single photons, forming a collective quantum entity potentially capable of performing quantum computations and simulations. Here, a promising approach is to use optical cavities within the setting of cavity quantum electrodynamics (QED). However, since its first realization in 1992 by Kimble et al., current proof-of-principle experiments have involved just one or two conventional cavities. To move beyond to N >> 1 nodes, in this thesis we investigate a platform born from the marriage of cavity QED and nanophotonics, where single atoms at ~100 nm near the surfaces of lithographically fabricated dielectric photonic devices can strongly interact with single photons, on a chip. Particularly, we experimentally investigate three main types of devices: microtoroidal optical cavities, optical nanofibers, and nanophotonic crystal based structures. With a microtoroidal cavity, we realized a robust and efficient photon router where single photons are extracted from an incident coherent state of light and redirected to a separate output with high efficiency. We achieved strong single atom-photon coupling with atoms located ~100 nm near the surface of a microtoroid, which revealed important aspects in the atom dynamics and QED of these systems including atom-surface interaction effects. We present a method to achieve state-insensitive atom trapping near optical nanofibers, critical in nanophotonic systems where electromagnetic fields are tightly confined. We developed a system that fabricates high quality nanofibers with high controllability, with which we experimentally demonstrate a state-insensitive atom trap. We present initial investigations on nanophotonic crystal based structures as a platform for strong atom-photon interactions. The experimental advances and theoretical investigations carried out in this thesis provide a framework for and open the door to strong single atom-photon interactions using nanophotonics for chip-integrated quantum networks.