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Physical review. B./Physical review. B

Anisotropic second-harmonic generation in superconducting nanostructures

Sara Memarzadeh, Maciej Krawczyk, ARMEN M. GULIAN, Jarosław W. Kłos

Published Jun 2, 2026• 0 citations
Publisher

Abstract

Circuits based on superconducting nanostructures are among the most promising platforms for quantum computing. Understanding how device geometry governs nonlinear electrodynamics is crucial for implementing superconducting quantum technologies. However, to date, research has largely been limited to superconducting nanostructures with collinearly aligned static and dynamic applied magnetic fields. Here, we analyze the dynamics of Meissner currents and Abrikosov vortices in a superconducting nanocube exposed to combined static and microwave magnetic fields, extending the analysis to a more general excitation geometry. We demonstrate that, in a noncollinear configuration, the magnetization component parallel to the static field develops a dominant second-harmonic response under the microwave driving. This effect is strongly enhanced when Meissner currents saturate at static fields just below the thresholds for successive vortex nucleation. By numerically solving the time-dependent Ginzburg-Landau equations, we show that the response originates from Meissner-current saturation combined with the nonlinear oscillations of normal-phase indentations, yielding an anisotropic second-harmonic signal that is directionally separated from, and not overshadowed by, the first-harmonic component of the dynamic magnetization. These findings are relevant for superconducting devices that require controllable high-frequency nonlinearity.

DOI
10.1103/2kgf-28s2

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Previous time-dependent Ginzburg–Landau simulations demonstrated that Abrikosov vortex dynamics in superconductors can be influenced by Aharonov–Bohm-type curl-less vector potentials even in simply connected geometries, without closed-loop trajectories enclosing magnetic flux [A. M. Gulian et al., Phys. Lett. A 382 (2018) 1058]. The origin of this effect has remained unexplained. Here we investigate further nonequilibrium effects in which the relation between a curl-less vector potential and an evolving quantum state produces observable consequences. During transient nonequilibrium state evolution, collective quantum systems may develop measurable responses to curl-less gauge fields despite a simply connected final equilibrium configuration with no persistent current. Using superconducting condensates, we formulate protocols based on the gauge-invariant coupling between quantum phase and the curl-less vector potential, analyze their dynamics using time-dependent Ginzburg–Landau theory and interpret rapid phase formation within the Kibble–Zurek picture. The predicted transient supercurrents and voltage signals provide a physical interpretation of nonequilibrium sensitivity to curl-less gauge fields and motivate experimental tests.
The development of nonlinear and frequency-tunable superconducting microwave circuits for operation in large magnetic fields is of high relevance for hybrid quantum systems such as spin resonance spectrometers, microwave quantum magnonics, dark matter axion detectors or flux-mediated optomechanics. With these exciting perspectives in mind, we investigate niobium-based circuits with integrated nano-constriction quantum interferometers in magnetic in-plane fields of up to several hundred mT. Our experiments reveal an unexpected and pronounced field-induced asymmetry in the bias-flux response of the circuits, which is demonstrated to originate from a field-induced Josephson-diode effect within the nano-constrictions and which enhances the circuit figures of merit in a magnetic field. An intuitive macroscopic Josephson-diode model attributes the effect to inhomogeneous constriction properties and provides us with the diode current-phase relation as a function of the in-plane field. Finally, we demonstrate that in the diode-state the circuit Kerr nonlinearity is bimodal in frequency, not only eliminating alternative explanations for the bias-flux-asymmetries but also being potentially useful for quantum circuit applications. Overall, our report underlines the potential of niobium nano-constriction circuits for high-field hybrid quantum systems, provides a conceptually simple explanation for the diode effect in superconducting nano-structures, and reveals the untapped potential of combining Josephson nano-diodes with microwave quantum circuits.