Cavity quantum electrodynamics (QED) studies the interaction between atoms and a single electromagnetic mode. When the atoms form a degenerate quantum gas, the resulting lightâ matter interaction reflects the underlying quantum statistics of the particles. Recently, degenerate Fermi gases have been coupled to optical cavities, enabling the exploration of strongly correlated fermionic systems with interactions mediated by cavity photons. Remarkably, when disorder is introduced into such systems, the resulting model realizes fermions with random, long-range interactions characteristic of the Sachdevâ Yeâ Kitaev Hamiltonian. This platform therefore offers a possible route toward the experimental investigation of holographic duality, linking strongly interacting quantum matter to black hole physics through the AdS/CFT correspondence. As a step toward realizing this model, we developed a new technology: the cavity microscope. This device combines the strong light-matter coupling of cavity QED with the micrometer-scale spatial resolution provided by high-numerical-aperture optics. This thesis presents the operation and the first experimental results obtained with this new platform. First, the high-resolution addressing capability of the cavity microscope was used to locally modify the level structure of thermal atoms within the cavity mode. This allowed us to extract spatially resolved information about the atomic density from a global cavity measurement. In doing so, we overcome a longstanding limitation of cavity QED experiments, where the spatial structure of the light-matter interaction is typically fixed by the cavity mode and cannot be freely tuned. Second, we implemented a tightly focused optical trap that enabled the extraction of a small degenerate Fermi gas from a larger atomic cloud, coupled to the cavity mode. We then systematically investigated the light-matter interaction between this tweezer-trapped Fermi gas and the cavity mode by studying the superradiant phase transition of atoms in the cavity. We find that the transition can be either facilitated or suppressed by the fermionic occupation of phase space. The crossover between these two regimes occurs when the scattering wavevector becomes approximately twice the Fermi wavevector, revealing the crucial role of Fermi statistics in cavity-mediated interactions. These results pave the way toward the deterministic preparation of few-fermion systems inside an optical cavity, enabling the study of finite-size and trap-filling effects in cavity QED. In an upgraded version of the cavity microscope, the number of atoms can approach the cavity cooperativity, bringing the system into a new regime where entanglement can extend across the entire ensemble. Finally, by introducing time-dependent randomization of cavity-mediated interactions, this platform could realize low-rank SYK models, opening the door to experimental investigations of fast scrambling, thermalization, and quantum chaos in strongly interacting quantum matter.
Cavity quantum electrodynamics (QED) studies the interaction between atoms and a single electromagnetic mode. When the atoms form a degenerate quantum gas, the resulting lightâ matter interaction reflects the underlying quantum statistics of the particles. Recently, degenerate Fermi gases have been coupled to optical cavities, enabling the exploration of strongly correlated fermionic systems with interactions mediated by cavity photons. Remarkably, when disorder is introduced into such systems, the resulting model realizes fermions with random, long-range interactions characteristic of the Sachdevâ Yeâ Kitaev Hamiltonian. This platform therefore offers a possible route toward the experimental investigation of holographic duality, linking strongly interacting quantum matter to black hole physics through the AdS/CFT correspondence. As a step toward realizing this model, we developed a new technology: the cavity microscope. This device combines the strong light-matter coupling of cavity QED with the micrometer-scale spatial resolution provided by high-numerical-aperture optics. This thesis presents the operation and the first experimental results obtained with this new platform. First, the high-resolution addressing capability of the cavity microscope was used to locally modify the level structure of thermal atoms within the cavity mode. This allowed us to extract spatially resolved information about the atomic density from a global cavity measurement. In doing so, we overcome a longstanding limitation of cavity QED experiments, where the spatial structure of the light-matter interaction is typically fixed by the cavity mode and cannot be freely tuned. Second, we implemented a tightly focused optical trap that enabled the extraction of a small degenerate Fermi gas from a larger atomic cloud, coupled to the cavity mode. We then systematically investigated the light-matter interaction between this tweezer-trapped Fermi gas and the cavity mode by studying the superradiant phase transition of atoms in the cavity. We find that the transition can be either facilitated or suppressed by the fermionic occupation of phase space. The crossover between these two regimes occurs when the scattering wavevector becomes approximately twice the Fermi wavevector, revealing the crucial role of Fermi statistics in cavity-mediated interactions. These results pave the way toward the deterministic preparation of few-fermion systems inside an optical cavity, enabling the study of finite-size and trap-filling effects in cavity QED. In an upgraded version of the cavity microscope, the number of atoms can approach the cavity cooperativity, bringing the system into a new regime where entanglement can extend across the entire ensemble. Finally, by introducing time-dependent randomization of cavity-mediated interactions, this platform could realize low-rank SYK models, opening the door to experimental investigations of fast scrambling, thermalization, and quantum chaos in strongly interacting quantum matter.
This thesis reports on quantum simulation experiments conducted on strongly correlated fermionic atoms coupled to light in an optical cavity. To this day, the quantum-mechanical description of strongly correlated many-body systems remains a considerable theoretical challenge. Quantum simulation experiments with ultracold atoms contribute to the understanding of such systems through controlled studies of complex, engineered many-body states. Advances in measurement and control techniques continuously drive the development of this field, enabling the creation, detection, and manipulation of novel states of matter. The experiments presented in this thesis build upon the prior observation of cavity-induced density-wave ordering in a gas of strongly interacting 6Li atoms. In particular, we report on an extension of the cavity quantum electrodynamics setup through the implementation of a high-resolution imaging system. The imaging setup enables the in situ observation of the density waves through resonant absorption imaging within a single experimental realization. Using this technique, we investigate ordering both following adiabatic preparation and after a quench of the cavity-induced long-range interaction. Our observations support the expectation of a density modulation with a single spatial frequency and phase that extends across the entire atomic cloud. We further present a correlation study between atomic and photonic observables, confirming their correspondence and thereby directly testing the theoretical foundation of cavity-mediated interactions. By imaging density waves in the vicinity of the first higher-order transverse cavity mode, we demonstrate the capability of the imaging setup to reveal local order beyond global observables. Additionally, this thesis presents two studies of density-wave ordering based on measurements of the cavity photon leakage. The first study focuses on the dynamics of order formation following an instantaneous quench. We observe an exponential growth of the order parameter, with a growth rate predominantly governed by the quench strength, in agreement with a theoretical description based on a random phase approximation. In the second study, we realize a system of three mutually coupled orders, enabled by the simultaneous coupling of light to atoms and atom pairs via a photoassociation resonance. In combination with the strong correlations present in the gas, this gives rise to three coupled order parameters: the cavity photon field, a density wave, and a pair-density wave. The mutual competition and enhancement between these orders result in a measurable shift of the density-wave order phase boundary. We conclude the thesis by reporting on recent experimental advances in the implementation of a homogeneous trapping potential, leading to a uniform atomic density along two spatial directions. This represents work towards an ideal starting point for a range of exciting future experiments, including spectroscopic measurements, local potential patterning, and correlation studies in long-range interacting Fermi gases, leveraging the numerical aperture of the imaging system.
Cavity quantum electrodynamics offers the possibility of observing and controlling the motion of a few or individual atoms, enabling the realization of various quantum technological tasks such as quantum enhanced metrology or quantum simulation of strongly correlated matter. A core limitation of these experiments lies in the mode structure of the cavity field, which is hard coded in the shape and geometry of the mirrors. As a result, most applications of cavity QED trade spatial resolution for enhanced sensitivity. Here, we propose and demonstrate a cavity-microscope device capable of controlling in space and time the coupling between atoms and light in a single-mode high-finesse cavity, reaching a spatial resolution an order of magnitude lower than the cavity-mode waist. This is achieved through local Floquet engineering of the atomic level structure, imprinting a corresponding atom-field coupling. We illustrate this capability by engineering micrometer-scale coupling, using cavity-assisted atomic measurements and optimization. Our system forms an optical device with a single optical axis, has the same footprint and complexity as a standard Fabry-Perot cavity or confocal lens pair, and can be used for any atomic species. This technique opens a wide range of perspectives, from ultrafast cavity-enhanced midcircuit readout to the quantum simulation of fully connected models of quantum matter such as the Sachdev-Ye-Kitaev model. Published by the American Physical Society 2024
Coupling between quantum emitters and modes of light is foundational to studies of quantum systems. Coherent interactions between matter and light have greatly advanced the development of quantum technologies. When an ensemble of atoms interacts with light that is confined within a cavity---a resonator for photons---light also mediates atom-atom interactions, leading to collective phenomena that cannot be extrapolated from microscopic behaviors. Understanding how interactions among quantum particles lead to macroscopic phenomena, such as phase transitions and breaking of symmetries, remains a challenge in modern physics. In this dissertation, I present results addressing this challenge in the context of mesoscopic arrays of optical-tweezer-trapped atoms interfaced with a high-finesse optical cavity. In particular, the physics we investigate arises from the collective scattering of light. Utilizing the ability to place atoms with nanometer-scale precision, we engineer superradiant and subradiant states, where control over interference of the emission from multiple atoms leads to collectively enhanced or suppressed amounts of scattered light. Building on this work, we investigate the emergence of optomechanical self-organization, mediated by superradiance in the cavity electromagnetic field. By coupling atoms to the same cavity mode, the atoms exert forces on one another through the exchange of photons, leading them to autonomously order themselves spatially. We characterize mesoscopic fluctuations and their effect on symmetry-breaking dynamics associated with self-organization. Finally, we extend this framework to theoretically investigate how the phase of the atom-cavity coupling can be altered to generate higher symmetries. Our analysis reveals first-order phase transitions and instabilities induced by non-reciprocal forces. Altogether, this work establishes a path towards realizing mesoscopic systems of complex phases of matter in cavity quantum electrodynamics with unprecedented programmability.
Motivated to develop quantum technologies and to study ever-more complex quantum systems,scientists are developing increasingly sophisticated experimental tools to control and\nmeasure quantum samples such as ensembles of ultracold atoms. A high-finesse optical\ncavity can be used to measure the state of atoms within its photonic mode with precision\nlimited only by quantum uncertainty. Such a cavity can also be used to mediate interactions\nbetween different atoms within the cavity mode. High-resolution microscope objectives have\nbeen interfaced with ultracold atom experiments to allow researchers to image single atoms\nwithin optical lattices, to trap single atoms in microtweezer arrays, and to imprint arbitrary\noptical patterns onto atomic ensembles. Among other applications, these technologies have\nallowed researchers to investigate many-body quantum systems, engineer novel interactions,\nand realize high-fidelity quantum operations.This dissertation presents the details of the design, construction, and operation of a new, versatileatomic physics apparatus that combines these two experimental tools. The apparatus\nincludes a high-finesse optical cavity into which atoms are optically transported. In addition,\nthere is a high-numerical-aperture objective aligned to image, with micron-scale resolution,\natoms trapped within the center of the optical cavity. We present results demonstrating\nthe capability of this apparatus to deliver and study ultracold atomic samples, ranging from\nsingle atoms to Bose-Einstein condensates. We demonstrate a dispersive shift of the cavity\nresonance due to the presence of atoms in the cavity mode and the trapping and imaging of\nsingle atoms in optical microtweezers. We also present an atomic scanning probe microscopy\ntechnique with which a single atom in a microtweezer is used to map out the spatial amplitude\npattern of an optical cavity mode standing wave by monitoring the position-dependent\nscattering properties of the atom.
Coherent light-matter interactions between a quantum gas and light in a high-finesse cavity can drive self-ordering phase transitions. To date, such phenomena have involved exclusively single-atom coupling to light, resulting in coupled charge-density or spin-density wave and superradiant order. In this work, we engineer simultaneous coupling of cavity photons to both single atoms and fermionic pairs, which are also mutually coupled due to strong correlations in the unitary Fermi gas. This interplay gives rise to an interference between the charge-density wave and a pair-density wave, where the short-range pair correlation function is spontaneously modulated in space. We observe this effect by tracking the onset of superradiance as the photon-pair coupling is varied in strength and sign, revealing constructive or destructive interference of the three orders with a coupling mediated by strong light-matter and atom-atom interactions. Our observations are compared with mean-field theory where the coupling strength between atomic- and pair-density waves is controlled by higher-order correlations in the Fermi gas. These results demonstrate the potential of cavity quantum electrodynamics to produce and observe exotic orders in strongly correlated matter, paving the way for the quantum simulation of complex quantum matter using ultracold atoms.
Lasing [1, 2] and superradiance [3‐5] phenomena are currently enjoying a renaissance as research topics in atomic physics. Fundamentally based on the interaction of matter with an electromagnetic (light) field, the atomic dipoles in a “lasing medium” collectively emit into selected modes of the electromagnetic field and thereby create an amplified and coherent source of light. Present-day lasers use di erent types of gain media and cover a wide range of output frequencies for application in both, fundamental research and industry. A recent string of papers has reported on superradiance [6, 7] and lasing-type instabilities using Bose gases of various type (thermal atoms [8, 9], photon gases [10] and Bose-Einstein condensed atoms [11‐14]) in optical cavities. Buoyed by experimental control over essentially single excitation quanta of atoms and photons [15‐19] in cavity quantum electrodynamics, these works o er intriguing prospects for the next wave of experiments on strongly interacting light-mattter systems including a new regime where unexpected many-body and quantum fluctuation e ects of the lasing medium may become visible. Bohnet et al. [20] recently operated a superradiant “bad-cavity” laser in the few-photon regime based on coherent oscillations of the inter-atomic, collective dipole of the ultracold atoms in the cavity [21]. In this paper, we point out that a quantum degenerate Fermi gas has remarkable features as a lasing medium in a transversally driven cavity as sketched in Fig. 1. We show that the quantum statistics of the Fermi gas puts the coupled cavity+atoms system generically close to superradiance threshold as a consequence of the Pauli exclusion principle (“Pauli pressure”). Physically, this arises from enhanced scattering of fermions between di erent points on the Fermi surface with radiusjkFj by exchanging relatively large photon momenta Q from the cavity as illustrated in Fig. 1. By changing the power of the pump laser at a given density of the Fermi gas, the lasing transition is concomitant with the spontaneous formation of a charge density wave oscillating with 1=Q in real space. Tuning the ratiojkFj=jQj allows to generate a cavity spectrum with “broadband light” in certain spectral ranges or, for energies outside the particle-hole continuum of the fermions, light with relatively narrow linewidth. The normal mode splitting of the cavity by a single atom is completely replaced by many-body Ω |kF| Q