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arXiv:2405.03550 · PRX Quantum

Cavity Microscope for Micrometer-Scale Control of Atom-Photon Interactions

Francesca Orsi, Nick Sauerwein, Rohit Prasad Bhatt, Jonas Faltinath, Ekaterina Fedotova, Nicola Reiter, Tigrane Cantat-Moltrecht, Jean-Philippe Brantut

Published Dec 2, 2024• 9 citations
arXivHTMLPDF

Abstract

Cavity quantum electrodynamics offers the possibility of observing and controlling the motion of a few or individual atoms, enabling the realization of various quantum technological tasks such as quantum enhanced metrology or quantum simulation of strongly correlated matter. A core limitation of these experiments lies in the mode structure of the cavity field, which is hard coded in the shape and geometry of the mirrors. As a result, most applications of cavity QED trade spatial resolution for enhanced sensitivity. Here, we propose and demonstrate a cavity-microscope device capable of controlling in space and time the coupling between atoms and light in a single-mode high-finesse cavity, reaching a spatial resolution an order of magnitude lower than the cavity-mode waist. This is achieved through local Floquet engineering of the atomic level structure, imprinting a corresponding atom-field coupling. We illustrate this capability by engineering micrometer-scale coupling, using cavity-assisted atomic measurements and optimization. Our system forms an optical device with a single optical axis, has the same footprint and complexity as a standard Fabry-Perot cavity or confocal lens pair, and can be used for any atomic species. This technique opens a wide range of perspectives, from ultrafast cavity-enhanced midcircuit readout to the quantum simulation of fully connected models of quantum matter such as the Sachdev-Ye-Kitaev model. Published by the American Physical Society 2024

DOI
10.1103/prxquantum.5.040333

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Cavity quantum electrodynamics (QED) studies the interaction between atoms and a single electromagnetic mode. When the atoms form a degenerate quantum gas, the resulting lightâ matter interaction reflects the underlying quantum statistics of the particles. Recently, degenerate Fermi gases have been coupled to optical cavities, enabling the exploration of strongly correlated fermionic systems with interactions mediated by cavity photons. Remarkably, when disorder is introduced into such systems, the resulting model realizes fermions with random, long-range interactions characteristic of the Sachdevâ Yeâ Kitaev Hamiltonian. This platform therefore offers a possible route toward the experimental investigation of holographic duality, linking strongly interacting quantum matter to black hole physics through the AdS/CFT correspondence. As a step toward realizing this model, we developed a new technology: the cavity microscope. This device combines the strong light-matter coupling of cavity QED with the micrometer-scale spatial resolution provided by high-numerical-aperture optics. This thesis presents the operation and the first experimental results obtained with this new platform. First, the high-resolution addressing capability of the cavity microscope was used to locally modify the level structure of thermal atoms within the cavity mode. This allowed us to extract spatially resolved information about the atomic density from a global cavity measurement. In doing so, we overcome a longstanding limitation of cavity QED experiments, where the spatial structure of the light-matter interaction is typically fixed by the cavity mode and cannot be freely tuned. Second, we implemented a tightly focused optical trap that enabled the extraction of a small degenerate Fermi gas from a larger atomic cloud, coupled to the cavity mode. We then systematically investigated the light-matter interaction between this tweezer-trapped Fermi gas and the cavity mode by studying the superradiant phase transition of atoms in the cavity. We find that the transition can be either facilitated or suppressed by the fermionic occupation of phase space. The crossover between these two regimes occurs when the scattering wavevector becomes approximately twice the Fermi wavevector, revealing the crucial role of Fermi statistics in cavity-mediated interactions. These results pave the way toward the deterministic preparation of few-fermion systems inside an optical cavity, enabling the study of finite-size and trap-filling effects in cavity QED. In an upgraded version of the cavity microscope, the number of atoms can approach the cavity cooperativity, bringing the system into a new regime where entanglement can extend across the entire ensemble. Finally, by introducing time-dependent randomization of cavity-mediated interactions, this platform could realize low-rank SYK models, opening the door to experimental investigations of fast scrambling, thermalization, and quantum chaos in strongly interacting quantum matter.

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Motivated to develop quantum technologies and to study ever-more complex quantum systems,scientists are developing increasingly sophisticated experimental tools to control and\nmeasure quantum samples such as ensembles of ultracold atoms. A high-finesse optical\ncavity can be used to measure the state of atoms within its photonic mode with precision\nlimited only by quantum uncertainty. Such a cavity can also be used to mediate interactions\nbetween different atoms within the cavity mode. High-resolution microscope objectives have\nbeen interfaced with ultracold atom experiments to allow researchers to image single atoms\nwithin optical lattices, to trap single atoms in microtweezer arrays, and to imprint arbitrary\noptical patterns onto atomic ensembles. Among other applications, these technologies have\nallowed researchers to investigate many-body quantum systems, engineer novel interactions,\nand realize high-fidelity quantum operations.This dissertation presents the details of the design, construction, and operation of a new, versatileatomic physics apparatus that combines these two experimental tools. The apparatus\nincludes a high-finesse optical cavity into which atoms are optically transported. In addition,\nthere is a high-numerical-aperture objective aligned to image, with micron-scale resolution,\natoms trapped within the center of the optical cavity. We present results demonstrating\nthe capability of this apparatus to deliver and study ultracold atomic samples, ranging from\nsingle atoms to Bose-Einstein condensates. We demonstrate a dispersive shift of the cavity\nresonance due to the presence of atoms in the cavity mode and the trapping and imaging of\nsingle atoms in optical microtweezers. We also present an atomic scanning probe microscopy\ntechnique with which a single atom in a microtweezer is used to map out the spatial amplitude\npattern of an optical cavity mode standing wave by monitoring the position-dependent\nscattering properties of the atom.

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Acta Physica Sinica•Jan 1, 2023•0 citations
Cavity quantum electrodynamics offers the possibility of observing and controlling the motion of a few or individual atoms, enabling the realization of various quantum technological tasks such as quantum enhanced metrology or quantum simulation of strongly correlated matter. A core limitation of these experiments lies in the mode structure of the cavity field, which is hard coded in the shape and geometry of the mirrors. As a result, most applications of cavity QED trade spatial resolution for enhanced sensitivity. Here, we propose and demonstrate a cavity-microscope device capable of controlling in space and time the coupling between atoms and light in a single-mode high-finesse cavity, reaching a spatial resolution an order of magnitude lower than the cavity-mode waist. This is achieved through local Floquet engineering of the atomic level structure, imprinting a corresponding atom-field coupling. We illustrate this capability by engineering micrometer-scale coupling, using cavity-assisted atomic measurements and optimization. Our system forms an optical device with a single optical axis, has the same footprint and complexity as a standard Fabry-Perot cavity or confocal lens pair, and can be used for any atomic species. This technique opens a wide range of perspectives, from ultrafast cavity-enhanced midcircuit readout to the quantum simulation of fully connected models of quantum matter such as the Sachdev-Ye-Kitaev model. Published by the American Physical Society 2024
Cavity quantum electrodynamics (QED) with cooperativity far greater than unity enables high-fidelity quantum sensing and information processing.The high-cooperativity regime is often reached through the use of short single-mode resonators.More complicated multimode resonators, such as the near-confocal optical Fabry-Pérot cavity, can provide intracavity atomic imaging in addition to high cooperativity.This capability has recently proved important for exploring quantum many-body physics in the driven-dissipative setting.In this work, we show that a confocal-cavity-QED microscope can realize cooperativity in excess of 110.This cooperativity is on par with the very best single-mode cavities (which are far shorter) and 21 times greater than single-mode resonators of similar length and mirror radii.The 1.7-µm imaging resolution is naturally identical to the photon-mediated interaction range.We measure these quantities by determining the threshold of cavity superradiance when small optically tweezed Bose-Einstein condensates are pumped at various intracavity locations.Transmission measurements of an ex situ cavity corroborate these results.We provide a theoretical description that shows how cooperativity enhancement arises from the dispersive coupling to the atoms of many near-degenerate modes.
Neutral-atom array and cavity quantum electrodynamics offer complementary strengths for quantum science: scalable, reconfigurable qubit architectures and strong coherent light-matter coupling. Combining them in a single platform requires an optical cavity with simultaneously high cooperativity, sufficient mode volume to accommodate atom array, and ample side optical access for atom trapping, imaging, cooling, and rearrangement, a combination that is challenging to achieve. Here we realize an atomic array integrated with a millimeter-scale Fabry--Pérot cavity whose optically-characterized single-atom cooperativity reaches ηcav=125±13η_{\mathrm{cav}}=125\pm13ηcav​=125±13. Atom-cavity transmission spectra of trapped atoms yield an effective spectroscopic cooperativity ηspec=106±3η_{\mathrm{spec}}=106\pm 3ηspec​=106±3, providing an in-situ verification of strong coupling in the integrated platform. In this integrated system, we achieve a state-measurement fidelity of 99.925−18+15%99.925^{+15}_{-18}\%99.925−18+15​% for a single atom with a 4-μμμs readout time. We also demonstrate simultaneous coupling of up to 21 individually trapped atoms to the antinode of the cavity mode. The key technical advance is a two-step mirror-fabrication method combining precision mechanical shaping and carbon-dioxide laser polishing, which produces concave fused-silica mirrors with sub-millimeter radii of curvature and residual roughness below 2 A˚2~Å2 A˚. Our results establish a regime of cavity-integrated atomic array that simultaneously provides high cooperativity, large mode volume, and flexible manipulation of individual atoms, opening opportunities for cavity-assisted quantum state readout and long-range entanglement-engineering in atom-array platforms.
Cavity quantum electrodynamics (QED) studies the interaction between atoms and a single electromagnetic mode. When the atoms form a degenerate quantum gas, the resulting lightâ matter interaction reflects the underlying quantum statistics of the particles. Recently, degenerate Fermi gases have been coupled to optical cavities, enabling the exploration of strongly correlated fermionic systems with interactions mediated by cavity photons. Remarkably, when disorder is introduced into such systems, the resulting model realizes fermions with random, long-range interactions characteristic of the Sachdevâ Yeâ Kitaev Hamiltonian. This platform therefore offers a possible route toward the experimental investigation of holographic duality, linking strongly interacting quantum matter to black hole physics through the AdS/CFT correspondence. As a step toward realizing this model, we developed a new technology: the cavity microscope. This device combines the strong light-matter coupling of cavity QED with the micrometer-scale spatial resolution provided by high-numerical-aperture optics. This thesis presents the operation and the first experimental results obtained with this new platform. First, the high-resolution addressing capability of the cavity microscope was used to locally modify the level structure of thermal atoms within the cavity mode. This allowed us to extract spatially resolved information about the atomic density from a global cavity measurement. In doing so, we overcome a longstanding limitation of cavity QED experiments, where the spatial structure of the light-matter interaction is typically fixed by the cavity mode and cannot be freely tuned. Second, we implemented a tightly focused optical trap that enabled the extraction of a small degenerate Fermi gas from a larger atomic cloud, coupled to the cavity mode. We then systematically investigated the light-matter interaction between this tweezer-trapped Fermi gas and the cavity mode by studying the superradiant phase transition of atoms in the cavity. We find that the transition can be either facilitated or suppressed by the fermionic occupation of phase space. The crossover between these two regimes occurs when the scattering wavevector becomes approximately twice the Fermi wavevector, revealing the crucial role of Fermi statistics in cavity-mediated interactions. These results pave the way toward the deterministic preparation of few-fermion systems inside an optical cavity, enabling the study of finite-size and trap-filling effects in cavity QED. In an upgraded version of the cavity microscope, the number of atoms can approach the cavity cooperativity, bringing the system into a new regime where entanglement can extend across the entire ensemble. Finally, by introducing time-dependent randomization of cavity-mediated interactions, this platform could realize low-rank SYK models, opening the door to experimental investigations of fast scrambling, thermalization, and quantum chaos in strongly interacting quantum matter.
Motivated to develop quantum technologies and to study ever-more complex quantum systems,scientists are developing increasingly sophisticated experimental tools to control and\nmeasure quantum samples such as ensembles of ultracold atoms. A high-finesse optical\ncavity can be used to measure the state of atoms within its photonic mode with precision\nlimited only by quantum uncertainty. Such a cavity can also be used to mediate interactions\nbetween different atoms within the cavity mode. High-resolution microscope objectives have\nbeen interfaced with ultracold atom experiments to allow researchers to image single atoms\nwithin optical lattices, to trap single atoms in microtweezer arrays, and to imprint arbitrary\noptical patterns onto atomic ensembles. Among other applications, these technologies have\nallowed researchers to investigate many-body quantum systems, engineer novel interactions,\nand realize high-fidelity quantum operations.This dissertation presents the details of the design, construction, and operation of a new, versatileatomic physics apparatus that combines these two experimental tools. The apparatus\nincludes a high-finesse optical cavity into which atoms are optically transported. In addition,\nthere is a high-numerical-aperture objective aligned to image, with micron-scale resolution,\natoms trapped within the center of the optical cavity. We present results demonstrating\nthe capability of this apparatus to deliver and study ultracold atomic samples, ranging from\nsingle atoms to Bose-Einstein condensates. We demonstrate a dispersive shift of the cavity\nresonance due to the presence of atoms in the cavity mode and the trapping and imaging of\nsingle atoms in optical microtweezers. We also present an atomic scanning probe microscopy\ntechnique with which a single atom in a microtweezer is used to map out the spatial amplitude\npattern of an optical cavity mode standing wave by monitoring the position-dependent\nscattering properties of the atom.
Optical cavities are a foundational technology for controlling light-matter interactions. While interfacing a single cavity to either an atom or ensemble has become a standard tool, the advent of single-atom control in large atomic arrays has spurred interest in a new frontier of “many-cavity QED,” featuring many independent resonators capable of separately addressing individual quantum emitters. In this fast-evolving landscape, the was recently introduced—employing free space intracavity optics to engineer a two-dimensional array of tightly spaced cavity TEM 00 modes with wavelength-scale waists, ideally suited for interfacing with atom arrays. Here, we realize the next generation of this architecture, achieving hundreds of degenerate cavity modes with improved, uniform finesse, and explore the technical features of the system which will enable further scalability. In particular, we study imperfections, including optical aberrations, field of view constraints, array nondegeneracies, and losses from optical elements. We identify the sensitivity to these various factors and exposit the control knobs and techniques necessary to align and operate the system in a stable manner. Ultimately, we lay out a pathway toward operation with tens of thousands of independent cavities while maintaining compatibility with existing atom arrays, paving the way to myriad applications including highly parallelized remote entanglement generation, fast and nondestructive midcircuit readout, and the implementation of hybrid atom-photon Hamiltonians.
Cavity quantum electrodynamic system with strongly coupled single atoms provides a good platform for studying quantum information processing, quantum simulation, quantum network, and distributed quantum computing. Cooling and trapping single atoms is a crucial technique in the quantum technology. At present, in a high-finesse cavity with finite space, cooling and trapping single atoms is a big challenge, even though it is a mature technique for free space. Great efforts have been made to cool and trap single atoms inside a cavity, and for a trapped atom its lifetime has reached as long as tens of seconds. Developing a more flexible method of cooling and trapping single atoms in a cavity is still essential for a strongly coupled cavity quantum electrodynamic system. In this work, we demonstrate experimentally that a single cesium atom in a cavity can be trapped by utilizing a single optical tweezer settled in cavity mode, and its lifetime is (2.60 ± 0.18) s. The experiment is carried out in a Fabry-Perot cavity, which is assembled by two concave mirrors each with a curvature radius of 100 mm, and cavity length of 335 μm. The concave surfaces are highly reflective, and the cavity has a finesse of 6.1 × 104. The 1080 nm optical tweezer with a waist of 2 μm is formed by an achromatic lens group with a numerical aperture of 0.4. At first, the precooled atomic assemble released from the magneto-optical trap (MOT) is transferred into cavity mode by an optical dipole trap with a waist of 36 μm. Then, one of the successfully transferred atoms is captured by the optical tweezer with the aid of cavity cooling mechanism. A blue detuned cavity locking laser is used as a standing-wave optical trap along the cavity axis. The signal of successfully trapped one atom is obtained by recording transmission of the cavity that will decrease owing to the strong coupling induced vacuum Rabi splitting. Finally, we demonstrate the precise manipulation of the atom-cavity coupling strength, which is achieved by scanning the position of the trapped atom step by step by using a high-precision translation stage. The system realized in this work can be used to study the dynamics of single atom-photon interactions with adjustable coupling strength. In addition, the mechanism adopted in this work is compatible with constructing tweezer arrays inside cavity mode, and thus possesses more flexibility and great potentials in cavity-based quantum entanglement and quantum simulation.