Understanding quantum coherence and proposing protection mechanisms has become one of the fundamental challenges in quantum physics research. We investigate a generic driven open quantum system, i.e., the driven spin-boson model, beyond the rotating-wave approximation. Although steady-state coherence vanishes in Floquet-Markov and Bloch-Redfield approaches, it becomes finite within a time-non-local master equation with a memory kernel. We analytically reveal that the steady-state coherence is associated with the overlap between the spectral densities associated with neighboring Floquet quasifrequencies. Motivated by this, we show that increasing temperature and introducing mixed transverse and longitudinal baths broadens the spectral density, thereby enhancing steady-state coherence. This is described by resonance fluorescence spectra, which exhibit clear spectral broadening and enhanced steady-state values. For a transverse dissipative coupling to the bath, three transition frequencies emerge in the Floquet basis, corresponding to the Mollow triplet. For weak resonant driving, these quasienergies become nearly degenerate, leading to closely spaced peaks in the resonance fluorescence spectrum, and the steady-state quantum coherence asymptotically approaches its maximum. For a longitudinal coupling to the bath, the quantum system exhibits a single transition frequency, thereby resulting in a complete suppression of the steady-state quantum coherence. We systematically investigate the influences of driving strength, frequency, temperature, and various dissipative baths on steady-state quantum coherence. These findings provide a foundational framework for efficiently engineering steady-state quantum coherence in nanoscale open quantum devices under optical field excitation.
Understanding quantum coherence and proposing protection mechanisms has become one of the fundamental challenges in quantum physics research. We investigate a generic driven open quantum system, i.e., the driven spin-boson model, beyond the rotating-wave approximation. Although steady-state coherence vanishes in Floquet-Markov and Bloch-Redfield approaches, it becomes finite within a time-non-local master equation with a memory kernel. We analytically reveal that the steady-state coherence is associated with the overlap between the spectral densities associated with neighboring Floquet quasifrequencies. Motivated by this, we show that increasing temperature and introducing mixed transverse and longitudinal baths broadens the spectral density, thereby enhancing steady-state coherence. This is described by resonance fluorescence spectra, which exhibit clear spectral broadening and enhanced steady-state values. For a transverse dissipative coupling to the bath, three transition frequencies emerge in the Floquet basis, corresponding to the Mollow triplet. For weak resonant driving, these quasienergies become nearly degenerate, leading to closely spaced peaks in the resonance fluorescence spectrum, and the steady-state quantum coherence asymptotically approaches its maximum. For a longitudinal coupling to the bath, the quantum system exhibits a single transition frequency, thereby resulting in a complete suppression of the steady-state quantum coherence. We systematically investigate the influences of driving strength, frequency, temperature, and various dissipative baths on steady-state quantum coherence. These findings provide a foundational framework for efficiently engineering steady-state quantum coherence in nanoscale open quantum devices under optical field excitation.
Abstract We theoretically investigate basic properties of nonequilibrium steady states of periodically-driven open quantum systems based on the full solution of the Maxwell–Bloch equation. In a resonant driving condition, we find that the transverse relaxation, also known as decoherence, significantly destructs the formation of Floquet states while the longitudinal relaxation does not directly affect it. Furthermore, by evaluating the quasienergy spectrum of the nonequilibrium steady states, we demonstrate that Rabi splitting can be observed as long as the decoherence time is as short as one third of the Rabi-cycle. Moreover, we find that Floquet states can be formed even under significant dissipation when the decoherence time is substantially shorter than the cycle of driving, once the driving field strength becomes strong enough. In an off-resonant condition, we demonstrate that the Floquet states can be realized even in weak field regimes because the system is not excited and the decoherence mechanism is not activated. Once the field strength becomes strong enough, the system can be excited by multi-photon absorption and the decoherence process becomes active. As a result, the Floquet states are significantly disturbed by the environment even in the off-resonant condition. Thus, we show here that the suppression of energy transfer from light to matter is a key condition for the realization of Floquet states in both on- and off-resonant conditions not only because it prevents material damage but also because it contributes to preserving coherence.
We theoretically investigate basic properties of nonequilibrium steady states of periodically-driven open quantum systems based on the full solution of the Maxwell–Bloch equation. In a resonant driving condition, we find that the transverse relaxation, also known as decoherence, significantly destructs the formation of Floquet states while the longitudinal relaxation does not directly affect it. Furthermore, by evaluating the quasienergy spectrum of the nonequilibrium steady states, we demonstrate that Rabi splitting can be observed as long as the decoherence time is as short as one third of the Rabi-cycle. Moreover, we find that Floquet states can be formed even under significant dissipation when the decoherence time is substantially shorter than the cycle of driving, once the driving field strength becomes strong enough. In an off-resonant condition, we demonstrate that the Floquet states can be realized even in weak field regimes because the system is not excited and the decoherence mechanism is not activated. Once the field strength becomes strong enough, the system can be excited by multi-photon absorption and the decoherence process becomes active. As a result, the Floquet states are significantly disturbed by the environment even in the off-resonant condition. Thus, we show here that the suppression of energy transfer from light to matter is a key condition for the realization of Floquet states in both on- and off-resonant conditions not only because it prevents material damage but also because it contributes to preserving coherence.
Strong periodic driving of cavity-quantum electrodynamics (QED) in the ultrastrong-coupling regime creates nonequilibrium states whose dissipation is governed by Floquet quasienergies rather than undriven dressed resonances. However, modeling such a regime is a significant theoretical challenge, including a number of subtle problems such as the need to ensure gauge invariance for truncated matter-cavity systems with time-dependent driving. To fill this theoretical gap, we introduce a nonsecular Floquet generalized master equation framework for strongly driven open cavity-QED systems, formulated in the dressed basis of the quantum Rabi model and applicable to structured reservoirs without rotating-wave approximations. Our theory can thus model Floquet-driven dynamics in open ultrastrong-coupling cavity-QED, and demonstrates a wide range of quantum state control. Using strong optical pumping and parametric mechanical modulation, we compute long-time populations, fluorescence spectra, and the Floquet-Liouville eigenspectra, resolving observable resonances into hybridized quasienergy channels and decay rates. By systematically comparing with conventional time-independent dressed-basis generalized master equations, we show that static approaches only reproduce steady-state populations in restricted excitation regimes, and fail for frequency-resolved observables and break down under appropriate Floquet engineering, surprisingly, even for spectrally flat baths. Structured environments, such as Lorentzian-Ohmic reservoirs, further amplify these discrepancies through sideband-selective decay. Our results demonstrate that dissipation in driven ultrastrong cavity-QED is intrinsically quasienergy resolved and we establish Floquet-dissipative theory as an accurate and powerful framework for predicting spectra, controlling decay pathways, and engineering nonequilibrium quantum states and reservoirs.
The dynamics of open quantum systems is commonly described by quantum master equations derived under the assumption of weak system-bath coupling and a separation of timescales between system and bath. When the system is additionally subjected to a periodic driving, the validity of the resulting Floquet master equations is further restricted to regimes of weak or high-frequency driving. Here, we benchmark a set of commonly used Floquet master equations for a model of two locally driven spins coupled to a shared Ohmic reservoir at finite temperature. We systematically probe the accuracy of the equations as a function of the driving parameters, thus identifying limits of their applicability. Dynamical maps predicted by each master equation are compared against numerically exact non-Markovian simulations, tracking the full relaxation dynamics. We find that the accuracy of each master equation closely reflects the assumptions underlying its derivation. For the Floquet-Lindblad equation, errors can be strongly amplified near resonances where the secular approximation breaks down, while approaches that avoid the secular approximation perform better and exhibit a more systematic dependence of the error on driving frequency and amplitude.
Time-periodic quantum systems are present all over science and technology. They have been successfully studied using Floquet theory, and a broad diversity of interesting phenomena such as coherent destruction of tunnelling, dynamical localization and creation of new phases of matter have been discovered. Furthermore, periodic driving has also been introduced as a tool for engineering novel quantum systems that have no static analogue. Besides these remarkable achievements for isolated systems, in reality, systems always interact with their surroundings. Taking the effect of the environment into account, time-periodic quantum systems have been mainly described using the Floquet-Markov approach, which consists in deriving a weak coupling master equation in the Floquet basis. In this thesis, we focus on how to overcome these standard approximations in the description of driven open quantum systems. We start by providing a general review on the topics of isolated driven systems, open quantum systems and the Floquet-Markov approach, before presenting the main results of this work. Under the effect of high-frequency driving, we provide an analytic solution to a large class of open quantum systems. Our method relies on discrete symmetries of the system-bath Hamiltonian and grants access to the time evolution operator of the full system, including bath degrees of freedom. The solution can be interpreted as the stroboscopic evolution of a family of observables under the influence of an effective static Hamiltonian. This provides a flexible simulation procedure of nontrivial Hamiltonians. The results are exemplified with the driven spin-boson model, where a coherent control of dissipation is observed. By a novel combination of Floquet theory, full counting statistics and a Markovian embedding strategy (reaction coordinate mapping), more intricate scenarios with additional driven system-environment interactions are addressed. Hereby, we can access the dynamics and thermodynamics of a periodically driven thermal machine. For the particular case where the working medium is a two-level system, we identify four different operating regimes, including a heat engine and a refrigerator. As the coupling strength is increased, their efficiency and coefficient of performance decrease and the refrigerator regime disappears. Notably, our model reproduces the setup of laser cooling of trapped ions in a specific parameter limit. Following the same combination of methods, we investigate electron pumping through a single quantum dot with periodically modulated energy and tunnelling amplitudes. In the high-frequency regime, the direction of the current can be controlled with the driving phase and a rectification effect that is exclusive to the non-Markovian character of the model is observed. In the low-frequency regime, we apply an additional transformation to view the model as three independent transport channels and observe that the coupling strength also controls the current direction. Studying charge fluctuations we validate that our model behaves as a single-electron source.
Nonequilibrium energy flows in a driven quantum system coupled to two heat baths are investigated to describe microscopic driven-dissipative processes, based on both a canonical transformation and full counting statistics. The main focus is to understand the interference between the coherent driving and bath induced dissipation. We aim to explore efficient modulation of the quantum energy transport, characterized as transient energy flow, by the Rabi driving and the temperature bias. In particular, steady-state energy flow is divided into three components: temperature bias flow, driving flow, and coherence flow. The driving flow is dominated by the external field driving, and the coherence flow is determined by the interference of two side peaks that are blueshifted and redshifted in Mollow's triplet. The energy flow is mainly contributed by the temperature bias flow at a weak driving limit, and the driving flow is in a strong driving regime. The effects of driving amplitude and temperature bias on the steady-state flow are discussed comprehensively. The results may provide guidance for the efficient control of energy and the information transport in nanodevices driven by an optical field.