As the field of superconducting quantum technology progresses beyond single-qubit control, scalable and multifunctional quantum architectures become increasingly vital. A central challenge is integrating fast, controllable superconducting circuits with components that offer longer coherence, richer physics, or new functionalities. Hybrid quantum systems, where superconducting microwave resonators interface with semiconducting or magnetic subsystems, have the capabilities to fulfil this need, yet they face significant engineering obstacles. Conventional superconducting resonator designs struggle under magnetic field biasing and electrostatic gating, both of which are essential for coupling to spin-based, semiconductor, or magnonic elements.This thesis explores solutions to these bottlenecks through the development of magnetic-field-resilient coplanar stripline (CPS) resonators based on thin-film NbTiN. These resonators retain a stable resonance frequency in in-plane magnetic fields up to 1T, can have high kinetic inductance and offer broad geometrical tunability, enabling strong and ultrastrong coupling to charge- and spin-based quantum systems. In the superconducting–semiconductor domain, we demonstrate high-impedance CPS resonators inductively coupled to Josephson junctions hosting Andreev bound states (ABSs), revealing both coherent pair transitions and single-quasiparticle excitations near the ultrastrong coupling regime. This opens the door to fast, gate-tunable qubits based on microscopic ABSs, distinct from conventional macroscopic qubit architectures, and lays the groundwork for spin–photon hybridisation, non-perturbative light–matter interactions, and parity-based quantum logic.In parallel, this work investigates rare-earth iron garnet (ReIG) ferrimagnetic insulators as low-loss spin-wave media compatible with superconducting devices. In sputtered thin-film thulium iron garnet (TmIG) with perpendicular magnetic anisotropy, we observe deterministic spin-orbit torque switching and multiple magnetisation polarity reversals. These properties showcase the attractiveness of TmIG both for low-dissipation magnonic information transport and as magnetic interfaces for superconducting hybrid devices. Taken together, the results of this thesis establish materials, device concepts, and measurement strategies for novel classes of hybrid quantum systems that combine robust superconducting circuitry, electrostatically tunable semiconductor excitations, and industry-scalable magnetic elements and pave the way for next-generation hybrid quantum systems. More broadly, they provide concrete routes to overcoming limitations of existing hybrid platforms and advance the development of versatile, low-dissipation quantum technologies.
As the field of superconducting quantum technology progresses beyond single-qubit control, scalable and multifunctional quantum architectures become increasingly vital. A central challenge is integrating fast, controllable superconducting circuits with components that offer longer coherence, richer physics, or new functionalities. Hybrid quantum systems, where superconducting microwave resonators interface with semiconducting or magnetic subsystems, have the capabilities to fulfil this need, yet they face significant engineering obstacles. Conventional superconducting resonator designs struggle under magnetic field biasing and electrostatic gating, both of which are essential for coupling to spin-based, semiconductor, or magnonic elements.This thesis explores solutions to these bottlenecks through the development of magnetic-field-resilient coplanar stripline (CPS) resonators based on thin-film NbTiN. These resonators retain a stable resonance frequency in in-plane magnetic fields up to 1T, can have high kinetic inductance and offer broad geometrical tunability, enabling strong and ultrastrong coupling to charge- and spin-based quantum systems. In the superconducting–semiconductor domain, we demonstrate high-impedance CPS resonators inductively coupled to Josephson junctions hosting Andreev bound states (ABSs), revealing both coherent pair transitions and single-quasiparticle excitations near the ultrastrong coupling regime. This opens the door to fast, gate-tunable qubits based on microscopic ABSs, distinct from conventional macroscopic qubit architectures, and lays the groundwork for spin–photon hybridisation, non-perturbative light–matter interactions, and parity-based quantum logic.In parallel, this work investigates rare-earth iron garnet (ReIG) ferrimagnetic insulators as low-loss spin-wave media compatible with superconducting devices. In sputtered thin-film thulium iron garnet (TmIG) with perpendicular magnetic anisotropy, we observe deterministic spin-orbit torque switching and multiple magnetisation polarity reversals. These properties showcase the attractiveness of TmIG both for low-dissipation magnonic information transport and as magnetic interfaces for superconducting hybrid devices. Taken together, the results of this thesis establish materials, device concepts, and measurement strategies for novel classes of hybrid quantum systems that combine robust superconducting circuitry, electrostatically tunable semiconductor excitations, and industry-scalable magnetic elements and pave the way for next-generation hybrid quantum systems. More broadly, they provide concrete routes to overcoming limitations of existing hybrid platforms and advance the development of versatile, low-dissipation quantum technologies.
Circuit quantum electrodynamics has received an increasing amount of attention over the last decade in light of its potential use in quantum information processing. The underlying principle of this architecture is the coherent coupling between microwave photons stored in superconducting resonators and superconducting qubits made from non-linear, non-dissipative electrical circuits. This architecture can be extended to other solid-state systems with transition frequencies in the microwave regime, such as nuclear and electron spins or Andreev bound states. These hybrid devices would allow the coherent exchange of information between such systems and superconducting qubits mediated by a microwave resonator. This could lead to advances in quantum information processing and new insights in the physics governing these interacting systems. In this dissertation experimental work with different types of hybrid quantum circuits is presented. A first experiment investigates the coherent coupling of microwave photons with a spin ensemble in a correlated and uncorrelated state. The coupling strength and magnetic resonance is studied as a function of temperature and magnetic field direction. A pronounced temperature dependent anisotropy of the magnetic resonance is observed, which can be attributed to the onset of antiferromagnetic correlations in the spin ensemble when cooled below T=4 K. A simple one-dimensional model gives a good description of this anisotropy. A next experiment studies the transport characteristics of carbon nanotubes electrically accessed with normal and superconducting contacts. These devices were characterised using both DC and RF reflectometry techniques. The carbon nanotube devices with superconducting contacts exhibit transport characteristics of Josephson junctions with critical currents of up to Ic~18 nA, as well as multiple Andreev reflections. These semiconductor-superconductor hybrid Josephson junctions are then used to realise a carbon-nanotube-based superconducting qubit with voltage tunable transition frequency using a local electrostatic gate. Strong coupling (g~100 MHz) to a coplanar waveguide resonator is demonstrated via a resonator frequency shift dependent on applied gate voltage. Qubit parameters are extracted from spectroscopy and correspond well to the DC measurements of the carbon nanotube Josephson junctions. Qubit relaxation and coherence times in the range 10-100 ns are observed. The hybrid devices investigated in this work present potential building blocks for more extensive hybrid architectures for quantum information processing.
The technology of quantum computing is believed to solve certain computational problems significantly faster than classical computers, enabling classically inaccessible problems. However, the technology is still in its infancy and it is still too early to conclude which physical system(s) will form the basis of tomorrow's quantum computer. Small-scale quantum processors, built on the superconducting transmon qubit, demonstrated already the anticipated quantum speed-up. Despite this tremendous milestone, scaling up to a full-fledged quantum computer is far from trivial: with these qubits, the flux-control causes crosstalk between qubits and heating, the room-temperature microwave control is hardly scalable and comes with high energetic radiation, and most importantly, the loss of quantum information in time leads to computational errors. Recent advances in various hybrid semiconductor materials enabled novel voltage-controlled transmons, gatemons, which are less susceptible to heating and crosstalk. Even more exciting, gatemons can be designed to host Majorana zero modes in a way that renders the qubit inherently protected against decoherence. In order to induce Majorana zero modes in such nanowire systems strong magnetic fields are required. Problematically, magnetic fields destroy the superconductivity that these microwave circuits rely on. In this thesis we integrate three types of hybrid Josephson junctions in magnetic field compatible microwave devices. Chapter 4 demonstrates the first graphene-based transmon. Due to the mono-atomic thickness of graphene in combination with magnetic field resilient coplanar waveguide resonators, we are able to operate the transmon circuit at an in-plane magnetic field of 1 Tesla. Chapter 5 embeds an InAs-Al semiconducting nanowire Josephson junction in a high quality factor superconducting transmission line resonator, demonstrating on-chip microwave generation. The gate-controllable semiconducting platform lends itself for fast pulse control, providing a perspective for the coherent on-chip manipulation of artificial two-level systems, in particular superconducting qubits such as transmons. Chapter 6 continues the development of InAs-Al nanowire transmons. The offset-charge-sensitive regime, additional plunger gates and magnetic field compatibility prepares the platform for the detection of coherent coupling between Majorana zero modes, a phenomena which unfortunately still remains unobserved. Additionally, we realise the first InSb-Al gatemon. The higher spin-orbit coupling makes InSb to be a preferred material in the search for Majorana signatures. Chapter 7 reports on the dynamics of quasiparticle tunneling events in real-time across the InAs-Al nanowire junction in a transmon architecture. The magnetic field compatibility of our device up to 1 Tesla together with in-situ voltage-controlled quasiparticle trap engineering, allows us to measure the survival of the charge-parity lifetime up to strong magnetic fields. A result which is extremely important in the research field of topological quantum computing, where the qubit space is defined in the charge-parity.
Hybrid semiconductor-superconductor qubits have recently emerged as a promising alternative to traditional platforms, combining material advantages with device-level tunability. A defining feature is their gate-tunable Josephson coupling, enabling superconducting qubit architectures with full electric-field control and offering a path toward scalable, low-crosstalk quantum processors. This approach seeks to merge benefits of superconducting and semiconductor qubits, for instance by encoding quantum information in the spin of a quasiparticle occupying an Andreev bound state, thus combining long coherence times with fast, flexible control. Progress has accelerated through bottom-up engineering of Andreev states in coupled quantum dot arrays, leading to architectures such as minimal Kitaev chains hosting Majorana zero modes. In parallel, Hamiltonian-protected designs aim to enhance resilience against local noise and decoherence by exploiting superconducting phase dynamics and discrete charge or flux degrees of freedom. This article reviews recent theoretical and experimental advances in hybrid qubits, providing an overview of physical mechanisms, device implementations, and emerging architectures, with emphasis on their potential for (topologically) protected quantum information processing. While many designs remain at proof-of-concept stage, rapid progress suggests practical demonstrations may soon be achievable.
The performance and coherence of superconducting quantum systems are fundamentally tied to the quality of the materials from which they are built. In superconducting transmon qubits, many loss mechanisms and sources of decoherence originate from material imperfections or unwanted oxide formation. Likewise, semiconductor–superconductor hybrid systems depend on high-quality interfaces to ensure strong coupling between electronic states in the two materials. In such hybrid devices, the accessible operating regime is often dictated by the intrinsic material properties of either the semiconductor or the superconductor. Advancing quantum device performance therefore requires exploring new material systems and optimizing their physical characteristics. In this thesis, we present the development of several superconducting material platforms for quantum technologies, including superconducting qubits, single-photon detectors, and semiconductor superconductor hybrid devices. We focus on the growth and characterization of superconducting films and heterostructures, and we establish clear connections between their material properties and the resulting device performance. First, we will present a novel semiconductor-superconductor hybrid material based on in-situ deposited epitaxial layers of Nb and Al on a shallow InAs quantum well. In this structure, the Al interlayer provides an epitaxial connection between an in-situ magnetron sputtered Nb or NbTi thin film and a shallow InAs two dimensional electron gas. This metal-to-metal epitaxy is achieved by optimization of the material stack and results in an induced superconducting gap of approximately 1 meV, determined from transport measurements of superconductor semiconductor Josephson junctions. This induced gap is approximately five times larger than the values reported for Al-based hybrid materials and indicates the formation of highly-transparent interfaces that are required in high-quality hybrid material platforms. Then, we discuss a different approach in the next chapter where we develop a hybrid material based on a molecular beam epitaxy grown InAsSb surface quantum well with an in-situ deposited Nb layer directly on top of the quantum well. Relative to conventional Al-InAs based systems, the InAsSb surface quantum well offers a lower effective mass and stronger spin-orbit interaction, while the Nb layer has a higher critical temperature and a larger critical magnetic field. The in-situ deposition of the Nb layer directly on top of the quantum well results in a high-quality interface that enables strong coupling to the InAsSb quantum well. Transport measurements on Josephson junctions reveal an induced superconducting gap of 1.3 meV and a critical current density of 3.75 × 10³A/cm². Furthermore, a planar asymmetric SQUID is realized, exhibiting gate-tunable superimposed oscillations originating from both the individual Josephson junction and the full SQUID loop. The large induced superconducting gap combined with strong spin-orbit interaction position this material as an attractive platform for experiments exploring gate-tunable superconductivity and topological superconducting devices. In the next chapter, we will focus on establishing a link between Nb film crystal properties and their performance in superconducting circuits. In this study, we investigate the microwave properties of niobium resonators with different crystalline properties and related surface topographies. We analyze a series of magnetron sputtered films in which the Nb crystal orientation and surface topography are changed by varying the substrate temperatures between room temperature and 975 K. The lowest-loss resonators that we measure have quality factors of over 10⁶ at single-photon powers, among the best ever recorded using the Nb on sapphire platform. We observe the highest quality factors in films grown at an intermediate temperature regime of the growth series (550 K) where the films display both preferential ordering of the crystal domains and low surface roughness. Furthermore, we analyze the temperature-dependent behavior of our resonators to learn about how the quasi-particle density in the Nb film is affected by the niobium crystal structure and the presence of grain boundaries. Then, we explore yet a different material platform by attempting to realize onchip NbTiN single photon detectors on LiNbO₃, an emerging photonic platform with high potential for scalable quantum information processing. We use DC reactive magnetron sputtering to grow high-quality NbTiN thin films and investigate the impact of substrate temperature during NbTiN growth. We achieve four nm thick superconducting films with a critical temperature (𝑇𝑐) of 12.3 K grown at a substrate temperature of 825 K. We demonstrate that the increased substrate temperature reduces the oxygen concentration in our films and improves the overall stoichiometry. In addition, we integrate these films with the LiNbO3 platform and investigate the obtained interface quality. Finally, we fabricate superconducting nanowire single photon detectors from the NbTiN film on LiNbO₃ and characterize the detector performance. Lastly, we report a gate-tunable Josephson diode effect in hybrid nanowire junctions consisting of a spin-orbit-coupled semiconductor core coated with epitaxial ferromagnetic insulator and superconductor shells. The wires display a hysteretic superconducting window as a function of axial magnetic field. In the superconducting regime, the devices exhibit nonreciprocal current transport, with the diode efficiency showing a strong dependence on back-gate voltage. The effect persists in a remanent magnetization state following a controlled demagnetization procedure, establishing zero-field operation. The combination of results presented in this thesis stress the importance of a material-focused approach in advancing the performance of quantum hardware. The novel hybrid material platforms developed in this thesis expand the operating regime of devices, which could enable future experiments involving gate-tunable superconductivity or topological properties. Similarly, we demonstrate that optimizing superconductor crystal structure benefits quantum devices, such as single-photon detectors and superconducting resonators.
A practical quantum computer demands a physical quantum bit (qubit) that is scalable, has a well-defined initial state, and brings together coherence with reliable control and read-out. A compelling idea is to put together a locally protected Majorana qubit with a superconducting qubit. The superconducting qubit is used to read out the Majorana states while the Majorana qubit may act as a quantum memory. This thesis presents a series of studies on quantum transport in semiconducting nanowires coupled to superconductors to investigate various platforms for realizing Majorana. These studies are followed by microwave measurements on superconducting circuits compatible with semiconducting-superconducting heterostructures. We first evaluate the potential of Ge/Si core/shell nanowires by achieving induced superconductivity as well as estimating spin-orbit coupling. Next we explore the transport mediated by Andreev bound states formed in InSb nanowire quantum. A subgap negative differential conductance is investigated together with the coalescing Andreev resonances at zero bias relevant for the correct interpretation of Majorana experiments done on the same structures. We conclude our studies of semiconducting nanowires by exploring tunnel junctions in Sn-InSb nanowires that are prepared by in-situ shadowing using nearby nanowires and flakes. Tin shells are found to induce a hard superconducting gap persisting up to high magnetic fields. We observe the two-electron charging effect from a small superconducting island of Sn-InSb. This effect is attributed to charge parity stability, which makes this nanowire system an intriguing candidate for superconducting and topological quantum circuits. These Sn-InSb junctions are then used as the nonlinear element in a transmon qubit design where we observe a dispersive coupling between this nanowire Josephson junction and a superconducting resonator. We also present our progress towards building a magnetic field resilient superconducting circuit that allows integration with semiconducting and topological structures. In the last chapter, InSb semiconducting nanowires are utilized as shadow masks prior to superconductor deposition on an InAs quantum well. We study Josephson current properties in Josephson junctions made from these nanowire shadows. Our results point to highly transparent junctions that can be developed further for hybrid superconductor-semiconductor qubit systems.
One of the key elements in circuit quantum electrodynamics (cQED) is the superconducting microwave resonator, which can enable strong coupling to and between nanoscale quantum systems, and as a result has emerged as an essential tool for both quantum information and quantum sensing. In this thesis, I will discuss new applications of superconducting resonators in both of these fields, which illustrates how quantum information and quantum sensing can be strongly tied together. As the field of quantum information continues to grow, various platforms for realizing a quantum computer have been proposed. One attractive platform is to control and manipulate the spin of an electron to form spin qubits, which have demonstrated a long coherence time, weak coupling to the environment, and high fidelity single- and two-qubit gates. However, scaling beyond two qubits has proven challenging, as has incorporating long-range coupling, although both are crucial for making spin qubits a scalable quantum computing platform. The confinement of electromagnetic fields in superconducting resonators enables strong coupling to small systems, such as the single electrons of a spin qubit. In the first part of this thesis, I will describe how a singlet-triplet spin qubit coupled to a high-impedance superconducting resonator constitutes a promising architecture for mediating long-ranged interactions based on a longitudinal coupling between the resonator and qubit. I will discuss the technical developments needed to successfully implement this novel type of interaction in a hybrid spin qubit-resonator device. This type of interaction has several advantages over the more commonly studied transverse coupling scheme: it does not require careful tuning of the qubit frequency to match that of the resonator, which facilitates scaling to a large number of qubits, and also avoids the loss of coherence, which is inevitable in resonant coupling. This type of interaction therefore opens promising paths for generating high-fidelity long-ranged two-qubit coupling by employing superconducting microwave resonators. By adapting techniques used in quantum information, we have also developed a new technique in quantum sensing, where we employ superconducting resonators as a probe of quantum materials such as mesoscopic systems, two-dimensional materials, and heterostructures, which are otherwise challenging to experimentally access with conventional techniques. In the second part of my thesis, I will discuss how implementing cQED techniques from quantum information allows us to probe the symmetry of the order parameter in unconventional superconductors. Unconventional superconductors are not readily available, and we therefore study an engineered system that comprises of interfacing a ferromagnet and superconductor, in which unconventional pairing can be induced into the ferromagnet. This platform allows us to simultaneously excite spin waves, a collective excitation of spins, in the ferromagnet, which opens new directions for studying interactions between coherently coupled magnons (quanta of spin waves) and unconventional superconducting states. Finally, by applying the same technique to a two-dimensional (2D) superconductor, tungsten ditelluride, we leverage this platform in an attempt to study the order parameter of its intrinsic superconducting phase. The nature of the order parameter in this material remains an open question, as both topological and superconducting phases can exist, possibly simultaneously. This work thus demonstrates a unique use of superconducting resonators beyond quantum information applications.