In this thesis, we theoretically investigate exotic quantum phenomena underlying periodically-driven systems.We discuss three distinct systems, noninteracting Dirac systems, lattice systems with a strong repulsive interaction, and lattice systems with a strong attractive interaction.We reveal various novel phenomena underlying these systems, and provide clear understanding of them.Periodically-driven systems, i.e., systems with a discrete time-translational symmetry, are described by the Floquet formalism, which maps the time-dependent Hamiltonian to a static "photon-dressed Hamiltonian".While a perturbative expansion of this Hamiltonian from the limit of high driving frequency has clarified various novel phenomena peculiar to periodically-driven systems, such an approach suffers from serious heating or damage when it is applied to realistic condensed matters.In this thesis, we focus on a lower-frequency regime, especially when the heating should be suppressed due to the small driving amplitude or an energy gap larger than the driving frequency.There, the high-frequency expansion cannot capture the relevant physics, so that we first formulate various perturbative expansions for three distinct regimes, i.e., high-frequency, small-amplitude, and strong-coupling regimes.We apply the small-amplitude expansion to two-and three-dimensional Dirac electrons driven by a circularly-polarized light to explore their behavior in the lowfrequency regime.We find an emergence of infinite numbers of topological gaps for the former and Weyl nodes for the latter.We also discuss how a regularization of the model affects this topological structure.We then introduce a strong repulsive interaction, and discuss behaviors of spins using the strong-coupling expansion.We predict an emergence of scalar spin chirality when a circularly-polarized light is illuminated, and discuss possible applications to photo-induced chiral spin liquids, and optical probing of spin chirality.Finally we turn to a strong attractive interaction to discuss the fate of the ordinary s-wave superconductivity under the periodic driving.We demonstrate an emergence of long sought-after η-pairing superconductivity, first as a ground state of the photon-dressed Hamiltonian, and then as a consequence of a dynamical phase transition in an isolated system such as an optical lattice system.
In this thesis, we theoretically investigate exotic quantum phenomena underlying periodically-driven systems.We discuss three distinct systems, noninteracting Dirac systems, lattice systems with a strong repulsive interaction, and lattice systems with a strong attractive interaction.We reveal various novel phenomena underlying these systems, and provide clear understanding of them.Periodically-driven systems, i.e., systems with a discrete time-translational symmetry, are described by the Floquet formalism, which maps the time-dependent Hamiltonian to a static "photon-dressed Hamiltonian".While a perturbative expansion of this Hamiltonian from the limit of high driving frequency has clarified various novel phenomena peculiar to periodically-driven systems, such an approach suffers from serious heating or damage when it is applied to realistic condensed matters.In this thesis, we focus on a lower-frequency regime, especially when the heating should be suppressed due to the small driving amplitude or an energy gap larger than the driving frequency.There, the high-frequency expansion cannot capture the relevant physics, so that we first formulate various perturbative expansions for three distinct regimes, i.e., high-frequency, small-amplitude, and strong-coupling regimes.We apply the small-amplitude expansion to two-and three-dimensional Dirac electrons driven by a circularly-polarized light to explore their behavior in the lowfrequency regime.We find an emergence of infinite numbers of topological gaps for the former and Weyl nodes for the latter.We also discuss how a regularization of the model affects this topological structure.We then introduce a strong repulsive interaction, and discuss behaviors of spins using the strong-coupling expansion.We predict an emergence of scalar spin chirality when a circularly-polarized light is illuminated, and discuss possible applications to photo-induced chiral spin liquids, and optical probing of spin chirality.Finally we turn to a strong attractive interaction to discuss the fate of the ordinary s-wave superconductivity under the periodic driving.We demonstrate an emergence of long sought-after η-pairing superconductivity, first as a ground state of the photon-dressed Hamiltonian, and then as a consequence of a dynamical phase transition in an isolated system such as an optical lattice system.
We construct a systematic high-frequency expansion for periodically driven quantum systems based on the Brillouin-Wigner (BW) perturbation theory, which generates an effective Hamiltonian on the projected zero-photon subspace in the Floquet theory, reproducing the quasienergies and eigenstates of the original Floquet Hamiltonian up to desired order in $1/\ensuremath{\omega}$, with $\ensuremath{\omega}$ being the frequency of the drive. The advantage of the BW method is that it is not only efficient in deriving higher-order terms, but even enables us to write down the whole infinite series expansion, as compared to the van Vleck degenerate perturbation theory. The expansion is also free from a spurious dependence on the driving phase, which has been an obstacle in the Floquet-Magnus expansion. We apply the BW expansion to various models of noninteracting electrons driven by circularly polarized light. As the amplitude of the light is increased, the system undergoes a series of Floquet topological-to-topological phase transitions, whose phase boundary in the high-frequency regime is well explained by the BW expansion. As the frequency is lowered, the high-frequency expansion breaks down at some point due to band touching with nonzero-photon sectors, where we find numerically even more intricate and richer Floquet topological phases spring out. We have then analyzed, with the Floquet dynamical mean-field theory, the effects of electron-electron interaction and energy dissipation. We have specifically revealed that phase transitions from Floquet-topological to Mott insulators emerge, where the phase boundaries can again be captured with the high-frequency expansion.
Controlling and manipulating complex many-body quantum systems will be a key ingredient \nfor the development of next-generation technologies. While the realisation of a \nuniversal quantum machine is still out of reach, in recent years experimental systems of \nultracold atoms have already evolved into a vivid field of research for quantum simulation. \nCrucially, such systems even allow for the successful quantum engineering of targeted \nmany-body systems by means of coherent periodic driving. The essential properties of \nthese Floquet systems encompass two main aspects: fast driving facilitates the simulation \nof effective static systems, and interactions lead to unique heating effects as energy is only \nconserved modulo the driving frequency. Within this thesis we theoretically study both \nof these aspects in respective model systems. \nIn part I of this thesis, we investigate the dynamics of excitations of a bosonic Mott \ninsulator in a designed one-dimensional Floquet system. Here, periodic driving in combination \nwith breaking all mirror symmetries of the system can induce directed motion of \nparticles. In the limit of small excitation densities, the effectively non-interacting quantum \nratchet determines the motion of holes and doublons in the Mott insulator and can in fact \nbe used to manipulate the dynamics of such. This little quantum machine can also be \nused to drive particles against an external force, where transport is possible but requires \nthe fulfilment of a commensurability condition for long times. \nIn part II, we discuss the role of interactions for periodically driven systems by means \nof a Floquet version of the Boltzmann equation. Starting from the Keldysh approach, \nwe develop this semiclassical formalism based on a clear separation of time scales. The \nresult is a description of the dynamics and the scattering of Floquet quasiparticles in \nsuch systems. Here, the property of discrete energy violation is naturally encoded in our \nformalism predicting the heating of interacting Floquet systems to infinite temperatures in \nthe long-time limit. As a first application of this approach, we investigate a cold atom setup \nrealising the Haldane model by means of periodic shaking. While homogeneous systems \nheat up globally, a confining potential evokes thermoelectric transport effects resulting \nfrom spatially dependent heating characteristics. Moreover, we show that the interplay \nof intrinsic heating, macroscopic diffusion and non-trivial topological properties of the \nHaldane model lead to an anomalous Floquet-Nernst effect, which describes anomalous \nparticle transport as the result of developing temperature gradients. \nIn part III, we elaborate on the quantum simulator aspect of ultracold atoms by providing \na theoretical framework for a possible simulation of a topological edge state in a \none-dimensional optical lattice. In this case, the one-dimensional Dirac equation with \nspatially varying mass is important, which captures the topological properties of a corresponding \nsystem of the BDI symmetry class. We analytically discuss such system and \ninvestigate the role of mean-field interaction effects. We also identify the emergence of \ndynamical instabilities in a realisation with bosonic atoms.
Periodically driven quantum systems provide a versatile platform for engineering and exploring non-equilibrium states of matter that have no equilibrium counterparts– a field commonly re- ferred to as Floquet engineering. The research presented in this thesis addresses the microscopic interpretation of experimental spectroscopic signatures, the stability of these driven states in the presence of strong many-body interactions, and the emergence of novel forms of non-equilibrium criticality encoded in quantum entanglement. The first part of the thesis focuses on the interpretation of time- and angle-resolved photo- emission spectroscopy (tr-ARPES), the primary experimental tool for detecting Floquet–Bloch sidebands (FBs). The measured signal reflects interference between processes occurring both inside the material and in the vacuum. In particular, Floquet-dressed initial states coexist and interfere with Volkov-dressed final states arising from the laser-assisted photoelectric effect (LAPE). Their experimental identification requires careful comparison with theoretical predic- tions. Using graphene as a model Dirac material, we perform a systematic comparison between two theoretical frameworks: the first-order perturbative Born approximation (PB1) and time- dependent nonequilibrium Green’s functions (tdNEGF), and compare them with experimental results. We disentangle intrinsic Floquet states, LAPE, and their interference, and quantify how polarization, incidence angle, and near-surface screening shape the observed spectra. Our findings show that, once matrix elements are included, both methods capture qualitative trends, but tdNEGF is necessary to describe the full energy–momentum-resolved features, including hybridization gaps. While non-interacting systems exhibit well-defined FBs, interacting systems absorb energy and can evolve toward an infinite-temperature state. To study this competition between coherent driving and many-body heating, in the second part we consider a one-dimensional chain of interacting spinless fermions using exact diagonalization (ED) and matrix product state (MPS) methods. We compute time-dependent spectral functions and correlation measures, and compare the spectral width of the many-body excitation continuum with the driving frequency to define low- and high-frequency regimes. In our parameter regime, low-frequency driving leads to strong overlap between Floquet sectors, resulting in rapid heating and loss of coherence. For weakly populated continua, we find a transient timescale for the suppression of FBs. When the driving frequency exceeds the continuum width, FBs are well separated and long-lived. Thefinalpartofthethesisinvestigatesnon-equilibriumphenomenafromaninformation-theoretic perspective. Wereportanewclassofdynamicalphasetransitions,termedtemporalentanglement transitions (TET) characterized by non-analytic reorganizations of the entanglement spectrum, in a periodically driven transverse-field Ising chain. These transitions occur in the spectrum of the entanglement Hamiltonian and are signaled by dynamical spontaneous symmetry breaking, marked by the closure of the Schmidt gap and parity flips. These transitions remain invisible to conventional local observables. Finite-size scaling reveals that TET belong to a universality class with a correlation-length exponent ν = 1, mirroring equilibrium Ising universality despite their purely dynamical origin.
Periodically-driven (Floquet) quantum systems are ubiquitous in science and technology. For example, when a laser illuminates a material or an AC voltage is applied to a device, the system is well-described by a time-periodic Hamiltonian. In recent years, periodic driving has been proposed, not just as a tool to excite and probe devices, but actually as a mechanism of engineering new phases of matter, some of which have no equilibrium analog. However, with this promise comes a serious problem. Intuitively, if energy is injected into and distributed throughout a system, it is no surprise that it tends to heat up indefinitely to infinite temperature. In this thesis, we study the mechanisms of heating, i.e. the process of thermalization, in Floquet systems and propose methods to control them. Specifically, for non-interacting Floquet systems that are coupled to external bosonic and fermionic baths (e.g. laser-driven electrons in a semiconductor that interact with phonons and an external lead), we classify the relevant scattering processes that contribute to cooling/heating in the Floquet bands and suggest methods to suppress heating via bandwidth-restrictions on the baths. We find that is possible, with appropriate dissipative engineering, to stabilize a controlled incompressible nonequilibrium steady-state resembling a ground state - a state we term the "Floquet insulator." We extend this analysis to include short-range interactions that contribute additional heating processes and show, under the same framework, that heating can be controlled with dissipation. In the process, we develop a simple effective model for the Floquet band densities that captures the essence of all the Floquet scattering processes and that is useful for ballparking experimentally-relevant estimates of heating. Next, we turn our attention to strongly-interacting closed Floquet systems and study how heating emerges through a proliferation of resonances. We find a novel integrable point governing the strong-interaction limit of the Floquet system and examine the breakdown of integrability via the proliferation of resonances. We observe two distinct scaling regimes, attributed to non-thermal and thermal behavior, and discover a power-law scaling of the crossover between them as a function of system size. The lingering ergodicity-breaking effects of the conserved quantities in the vicinity (in parameter space) of the integrable point at finite size is a phenomena we term "near-integrability." These results suggest that small quantum systems, which are accessible currently in many platforms (e.g. trapped ions, cold atoms, superconducting devices), intrinsically host non-thermal states that one may be able to utilize to avoid heating. Furthermore, our results suggest a "dual" interpretation, in the thermodynamic limit, that a periodically-driven system exhibits prethermalization as a power-law in interaction strength.
This thesis reports on the realization of Floquet topological systems with ultracold atoms in an optical honeycomb lattice. Using periodically driven quantum systems, topological phases of matter can be simulated by an effective, static Hamiltonian related to the time-evolution at integer multiples of the driving period, which is known as Floquet engineering. However, periodic driving can also give rise to genuinely time-dependent settings without static counterparts. One example is the anomalous Floquet phase in two dimensions, in which all bulk bands have a Chern number of zero but nevertheless robust chiral edge modes appear, which would be precluded by the bulk-edge correspondence in a static system. In an optical honeycomb lattice, anomalous Floquet systems can be created by continuous, periodic modulation of the laser intensities. This driving scheme results in different topological regimes, three of which are investigated, including the anomalous Floquet phase and a Haldane-like phase. Periodically driven systems feature periodic quasienergies and can be characterized in terms of winding numbers, which count the number of chiral edge modes in each quasienergy gap. By interferometric measurements of the quasienergy gaps between the first two Floquet bands, the topological phase transitions, emerging as gap closings, are located. For periodically driven systems, a modified bulk-edge correspondence can be formulated. In particular, the change of the winding number at a phase transition is related to the sign change of the local Berry curvature. The Berry curvature at the gap closing points is probed by Hall deflection measurements to obtain the winding numbers in each of the topological regimes, revealing the existence of chiral edge modes also in a setting with smooth boundaries as used in the experiments. The measured quasienergy gaps and transverse deflections are quantitatively well described by a numerical calculation of the Floquet bandstructure that includes coupling to higher bands during the driving period. To derive the spectrum of the modulated lattice in a geometry with edges, a tight-binding description of the system is discussed. Circular phase modulation of the honeycomb lattice can also give rise to an anomalous Floquet system when inversion symmetry is broken. The topological phase diagrams and the experimental feasibility are compared for both modulation schemes. Due to the vanishing Chern numbers, the bulk states in the anomalous Floquet regime can be fully localized by a disorder potential. This could prevent heating in interacting, periodically driven systems, resulting in a many-body localized bulk coexisting with thermalizing edge states. The experimental realization of disorder and strong interactions, as well as independent probes of the edge states are investigated. Bloch band geometry can be extended to multiband systems, using Wilson lines. The possible symmetry protection of their eigenvalues is discussed, along with measurements in the optical honeycomb lattice. Moreover, the onset of heating in weakly-interacting, periodically driven systems, triggered by parametric instabilities, is studied experimentally in a one-dimensional lattice.
Abstract Non-equilibrium engineering is becoming a seminal way for realising novel quantum phases that are unimaginable in equilibrium. In particular, Floquet theory applied to quantum mechanics revealed that we can even control the band topology in semimetallic/insulating systems, while the straightforward application to topological superconductivity fails for typical superconductors because the supercondicting gap function does not couple to the electromagnetic field in a direct manner. Here we show that we can overcome this difficulty by taking account of correlation effects. Namely, we study how a d-wave superconductivity is changed when illuminated by circularly-polarised light (CPL) in the repulsive Hubbard model in the strong-coupling regime. We adopt the Floquet formalism for the Gutzwiller-projected effective Hamiltonian with the time-periodic Schrieffer-Wolff transformation. We find that CPL induces a topological superconductivity with a d + id pairing, which arises from the chiral spin coupling and the three-site term generated by the CPL. The latter term remains significant even for low frequencies and low intensities of the CPL. This is clearly reflected in the obtained phase diagram against the laser intensity and temperature for various frequencies red-detuned from the Hubbard U, with the transient dynamics also examined. The phenomenon revealed here can open a novel, dynamical way to induce a topological superconductivity.