The extensive field of driven quantum systems has seen numerous theoretical and experimental advances in recent years, with studies ranging from measurement techniques, over engineering of out-of-equilibrium phases of matter to considerations of active matter on the quantum level. In this thesis, we explore three timely directions of this body of research. First, we consider arrays of Josephson junctions, which have become highly tunable in experiments due to recent fabricational progress. Numerical calculations suggest that transverse magnetic fields induce a cascade of different vortex lattice states on the arrays. We find in this thesis that the measurement of the full resistivity tensor gives direct access to information about the vortex lattices. Motivated by a recent experiment, we further study an array of $ϕ_0$-junctions. We find that going beyond nearest neighbor coupling, the $ϕ_0$-shifts lead to an asymmetric pinning potential for the vortices which consequently facilitates a Josephson diode effect via vortex depinning. Second, we turn towards periodically driven spin chains. Motivated by a recent experiment on a quantum processor, we study the Floquet quantum Ising model in its fermionic formulation. Depending on the parameters, the model can host edge modes that are associated with a topological, equilibrium (Majorana zero modes) or out-of-equilibrium (Majorana pi modes) phase. In contrast to the equilibrium phase, we find that the edge modes in the out-of-equilibrium phase are characterized by remarkable resistance against parity-breaking perturbations, which we explain in terms of a stroboscopic perturbation theory. Following this, we study spin correlation functions of a Floquet time crystal. Here we find a connection of pairings in the spectrum of the Floquet operator to the defining period-2 spin correlations of the time-crystalline phase. Specifically, we can express the correlation functions in terms of the Fourier transform of the pairing distribution, which is approximately of log-normal form. We also discuss implications for the phase diagram of the time crystal. The third and final topic of this thesis is the emerging field of active quantum matter. We first state the general framework for a single active quantum particle, after which we consider the specific example of a spin-1/2 particle. We then show under which conditions the particle carries out active motion and demonstrate that the motion is characterized by genuine quantum features.
The extensive field of driven quantum systems has seen numerous theoretical and experimental advances in recent years, with studies ranging from measurement techniques, over engineering of out-of-equilibrium phases of matter to considerations of active matter on the quantum level. In this thesis, we explore three timely directions of this body of research. First, we consider arrays of Josephson junctions, which have become highly tunable in experiments due to recent fabricational progress. Numerical calculations suggest that transverse magnetic fields induce a cascade of different vortex lattice states on the arrays. We find in this thesis that the measurement of the full resistivity tensor gives direct access to information about the vortex lattices. Motivated by a recent experiment, we further study an array of ϕ0-junctions. We find that going beyond nearest neighbor coupling, the ϕ0-shifts lead to an asymmetric pinning potential for the vortices which consequently facilitates a Josephson diode effect via vortex depinning. Second, we turn towards periodically driven spin chains. Motivated by a recent experiment on a quantum processor, we study the Floquet quantum Ising model in its fermionic formulation. Depending on the parameters, the model can host edge modes that are associated with a topological, equilibrium (Majorana zero modes) or out-of-equilibrium (Majorana pi modes) phase. In contrast to the equilibrium phase, we find that the edge modes in the out-of-equilibrium phase are characterized by remarkable resistance against parity-breaking perturbations, which we explain in terms of a stroboscopic perturbation theory. Following this, we study spin correlation functions of a Floquet time crystal. Here we find a connection of pairings in the spectrum of the Floquet operator to the defining period-2 spin correlations of the time-crystalline phase. Specifically, we can express the correlation functions in terms of the Fourier transform of the pairing distribution, which is approximately of log-normal form. We also discuss implications for the phase diagram of the time crystal. The third and final topic of this thesis is the emerging field of active quantum matter. We first state the general framework for a single active quantum particle, after which we consider the specific example of a spin-1/2 particle. We then show under which conditions the particle carries out active motion and demonstrate that the motion is characterized by genuine quantum features.
Periodically driven quantum systems provide a versatile platform for engineering and exploring non-equilibrium states of matter that have no equilibrium counterparts– a field commonly re- ferred to as Floquet engineering. The research presented in this thesis addresses the microscopic interpretation of experimental spectroscopic signatures, the stability of these driven states in the presence of strong many-body interactions, and the emergence of novel forms of non-equilibrium criticality encoded in quantum entanglement. The first part of the thesis focuses on the interpretation of time- and angle-resolved photo- emission spectroscopy (tr-ARPES), the primary experimental tool for detecting Floquet–Bloch sidebands (FBs). The measured signal reflects interference between processes occurring both inside the material and in the vacuum. In particular, Floquet-dressed initial states coexist and interfere with Volkov-dressed final states arising from the laser-assisted photoelectric effect (LAPE). Their experimental identification requires careful comparison with theoretical predic- tions. Using graphene as a model Dirac material, we perform a systematic comparison between two theoretical frameworks: the first-order perturbative Born approximation (PB1) and time- dependent nonequilibrium Green’s functions (tdNEGF), and compare them with experimental results. We disentangle intrinsic Floquet states, LAPE, and their interference, and quantify how polarization, incidence angle, and near-surface screening shape the observed spectra. Our findings show that, once matrix elements are included, both methods capture qualitative trends, but tdNEGF is necessary to describe the full energy–momentum-resolved features, including hybridization gaps. While non-interacting systems exhibit well-defined FBs, interacting systems absorb energy and can evolve toward an infinite-temperature state. To study this competition between coherent driving and many-body heating, in the second part we consider a one-dimensional chain of interacting spinless fermions using exact diagonalization (ED) and matrix product state (MPS) methods. We compute time-dependent spectral functions and correlation measures, and compare the spectral width of the many-body excitation continuum with the driving frequency to define low- and high-frequency regimes. In our parameter regime, low-frequency driving leads to strong overlap between Floquet sectors, resulting in rapid heating and loss of coherence. For weakly populated continua, we find a transient timescale for the suppression of FBs. When the driving frequency exceeds the continuum width, FBs are well separated and long-lived. Thefinalpartofthethesisinvestigatesnon-equilibriumphenomenafromaninformation-theoretic perspective. Wereportanewclassofdynamicalphasetransitions,termedtemporalentanglement transitions (TET) characterized by non-analytic reorganizations of the entanglement spectrum, in a periodically driven transverse-field Ising chain. These transitions occur in the spectrum of the entanglement Hamiltonian and are signaled by dynamical spontaneous symmetry breaking, marked by the closure of the Schmidt gap and parity flips. These transitions remain invisible to conventional local observables. Finite-size scaling reveals that TET belong to a universality class with a correlation-length exponent ν = 1, mirroring equilibrium Ising universality despite their purely dynamical origin.
Recent advances in experimental condensed matter physics suggest a powerful new paradigm for the realization of exotic phases of quantum matter in the laboratory. Rather than conducting an exhaustive search for materials that realize these phases at low temperatures, it may be possible to design quantum systems that exhibit the desired properties. With the numerous advances made recently in the fields of cold atomic gases, superconducting qubits, trapped ions, and nitrogen-vacancy centers in diamond, it appears that we will soon have a host of platforms that can be used to put exotic theoretical predictions to the test. In this dissertation, I will highlight two ways in which theorists can interact productively with this fast-emerging field. \n \nFirst, there is a growing interest in driving quantum systems out of equilibrium in order to induce novel topological phases where they would otherwise never appear. In particular, systems driven by time-periodic perturbations—known as “Floquet systems”—offer fertile ground for theoretical investigation. This approach to designer quantum matter brings its own unique set of challenges. In particular, Floquet systems explicitly violate conservation of energy, providing no notion of a ground state. In the first part of my dissertation, I will present research that addresses this problem in two ways. First, I will present studies of open Floquet systems, where coupling to an external reservoir drives the system into a steady state at long times. Second, I will discuss examples of isolated quantum systems that exhibit signatures of topological properties in their finite-time dynamics. \n \nThe second part of this dissertation presents another way in which theorists can benefit from the designer approach to quantum matter; in particular, one can design analytically tractable theories of exotic phases. I will present an exemplar of this philosophy in the form of coupled-wire constructions. In this approach, one builds a topological state of matter from the ground up by coupling together an array of one-dimensional quantum wires with local interactions. I will demonstrate the power of this technique by showing how to build both Abelian and non-Abelian topological phases in three dimensions by coupling together an array of quantum wires.
Superconductivity in its various manifestations has been stimulating both experimental and theoretical progress in condensed-matter physics for more than a hundred years. The remarkable property of electrons to pair up and form quasi-particles gives rise to a plethora of phenomena featuring important practical applications not only in science, but, for instance, also in medicine and metrology. Recently, new directions in investigating this fascinating subject emerged, such as superconductivity out-of equilibrium and topological superconductors. Providing experimental evidence for enhanced superconducting correlations in optically pumped copper oxides at temperatures far above the equilibrium transition temperature, the first issue caused considerable excitement. On the other hand, topological superconductors are believed to provide realizations of highly fault-tolerant qubits by means of hosting non-Abelian quasi-particles, which can be the building blocks of scalable quantum computers. Experimentally verifying the emergence of these Majorana edge modes, exotic quasi-particles in heterostructures consisting of a conventional superconductor and semiconductors or topological insulators, is one of the most urgent questions to be answered right now. Both subjects cannot be accounted for with analytically solvable approximations only, and also provide very challenging numerical problems. We implemented a matrix-product state (MPS) based toolkit exploiting U(1) symmetries, providing a flexible and efficient platform to study these complex systems. In order to efficiently simulate out-of equilibrium setups we studied, compared, and developed time-evolution algorithms for MPS enabling us to choose the most suitable method for a given task. We also developed a new framework to represent operators in an enlarged Hilbert space so that benefits from conserving U(1) symmetries can also be exploited in systems that originally break such symmetries (projected purification). Using this method we could efficiently model mesoscopic phenomena such as a charging energy controlled by a gate electrode without further approximations. Equipped with this techniques we studied out-of equilibrium spectral functions to explore how to identify superconducting correlations more reliably on ultra-short timescales. We found conclusive evidence that in particular two-particle spectral functions yield excellent probes for the formation of a (quasi-)condensate out-of equilibrium. Furthermore, we also investigated the question whether in a particular model system there is the possibility of true long-range order out-of equilibrium by studying correlation matrices and the scaling of their eigenvalues. Here, we observe a change in the algebraic decay of the correlations, even though the extrapolated order parameter is still zero within the error bounds. Furthermore, we also investigated the effects of coupling a superconductor-semiconductor heterostructure, which is subject to an in-plane magnetic field and a charging energy controlled by a gate voltage, to normal leads. In the context of experimentally verifying the existence of Majorana edge modes, such systems are believed to be the most promising and recent studies seem to underline this expectation. However, in order to consistently analyze the experimental data, the effects of quantum fluctuations caused by hybridization of the heterostructure with the leads have to be understood. Here, only perturbative limits are available so far, i.e., the weak and strong tunneling limit, while the experimentally relevant regime is expected to be somewhere inbetween. We aimed to fill this gap using the projected purification method to calculate the ground state phase diagram over a wide parameter regime. Our results indicate that the experimental situation is much more involved than what is predicted from perturbative analysis.
The study of quantum dynamics is an increasingly important aspect of atomic, molecular and optical physics, as well as condensed-matter physics and other disciplines. It is essential in order to understand non-equilibrium phenomena which do not fit within the framework of equilibrium thermodynamics, such as many-body localization, dynamical quantum phase transitions, and non-equilibrium steady states in driven-dissipative systems. However, the exact calculation of dynamical observables is extremely difficult in general for several reasons, which makes it challenging for theoretical predictions and analyses to keep pace with rapidly advancing experiments. In this thesis I use and develop several computational methods to investigate the dynamics of quantum many-body systems, with the two goals of better understanding the evolution of local observables and correlation functions in spin and Fermion systems as well as creating and testing more effective numerical methods for solving quantum dynamics problems. I explore quantum dynamics by using Hamiltonian parameter quenches in several commonly-used models in AMO physics and elsewhere: the Fermi-Hubbard model, the XXZ model, and the transverse-Ising model. The first represents a system of short-range interacting Fermions, while the latter two represent spin systems with different spin-spin couplings and magnetic field terms. All of these models can be realized in current experiments. First, I derive an exact solution for an extreme interaction quench in the Fermi-Hubbard model, from a strongly-interacting initial state to a noninteracting final Hamiltonian. From this result I show that there are nontrivial transient connected correlations, despite the fact that the system has very high temperature and a noninteracting Hamiltonian. Those features would suppress such correlations in equilibrium, but the dynamical correlations are still significant. Then, I develop and examine two numerical methods for solving dynamics of the spin expectation values and correlation functions in the transverse-Ising and XXZ models. Both methods rely on approximating a thermodynamically large system with a much smaller and more computationally tractable cluster of lattice sites, or a series of clusters. The first method is a dynamical numerical linked cluster expansion (NLCE). NLCEs have already been used successfully on systems in thermodynamic equilibrium, and I extended the technique to directly compute the dynamics of an observable after a quantum quench. I review the general NLCE method, describe my dynamical variant of it, and compute the quench dynamics of spin and correlation observables in the transverse-Ising and XXZ models. The second method, which I term the adaptive-boundary cluster method, relies on recently refined bounds on information propagation in quantum systems to choose a cluster of lattice sites that minimizes the finite size error bound of a dynamical computation. I briefly review these bounds, and describe a new algorithm which uses them to construct a cluster whose boundary is chosen according to a related error estimate. Such an adaptive-boundary cluster has the property that there exists a computable upper bound on the finite size error of observables measured at the cluster center, and this error bound is nearly minimal when compared to that of other clusters of the same size. I then compute the quench dynamics of spin and correlation observables in the transverse-Ising model using the adaptive boundary clusters. I apply this method to both uniform and strongly disordered systems. To evaluate the effectiveness of both dynamical NLCE and adaptive-boundary clusters, I compare the results obtained using them to results from a standard and general purpose numerical method: exact solvers applied a rectangular cluster with periodic boundary conditions. Both of the new methods usually converge faster and are more accurate than the standard method for comparable cluster sizes. This thesis illustrates that choosing numerical methods which take advantage of the geometric and entanglement structure of the initial state and Hamiltonian can substantially enhance our ability to study quantum dynamics, by reducing the computational cost of numerically exact solutions. I conclude with a discussion of various avenues for future research to build on this work.
Driving a quantum system periodically in time can profoundly alter its long-time correlations and give rise to exotic quantum states of matter. The complexity of the combination of many-body correlations and dynamic manipulations has the potential to uncover a whole field of new phenomena, but the theoretical and numerical understanding becomes extremely difficult. We now propose a promising numerical method by generalizing the density matrix renormalization group to a superposition of Fourier components of periodically driven many-body systems using Floquet theory. With this method we can study the full time-dependent quantum solution in a large parameter range for all evolution times, beyond the commonly used high-frequency approximations. Numerical results are presented for the isotropic Heisenberg antiferromagnetic spin-1/2 chain under both local(edge) and global driving for spin-spin correlations and temporal fluctuations. As the frequency is lowered, we demonstrate that more and more Fourier components become relevant and determine strong length- and frequency-dependent changes of the quantum correlations that cannot be described by effective static models.
The main topic of this thesis is the study of many-body effects in strongly correlated one- or quasi one-dimensional condensed matter systems. These systems are characterized by strong quantum and thermal fluctuations, which make mean-field methods fail and demand for a fully numerical approach. Fortunately, a numerical method exist, which allows to treat unusually large one -dimensional system at very high precision. This method is the density-matrix renormalization group method (DMRG), introduced by Steve White in 1992. Originally limited to the study of static problems, time-dependent DMRG has been developed allowing one to investigate non-equilibrium phenomena in quantum mechanics. In this thesis I present the solution of three conceptionally different problems, which have been addressed using mostly the Krylov-subspace version of the time-dependent DMRG. My findings are directly relevant to recent experiments with ultracold atoms, also carried out at LMU in the group of Prof. Bloch. The first project aims the ultimate goal of atoms in optical lattices, namely, the possibility to act as a quantum simulator of more complicated condensed matter system. The underline idea is to simulate a magnetic model using ultracold bosonic atoms of two different hyperfine states in an optical superlattice. The system, which is captured by a two-species Bose-Hubbard model, realizes in a certain parameter range the physics of a spin-1/2 Heisenberg chain, where the spin exchange constant is given by second order processes. Tuning of the superlattice parameters allows one to controlling the effect of fast first order processes versus the slower second order ones. The analysis is motivated by recent experiments, %\cite{Folling2007,Trotzky2008} where coherent two-particle dynamics with ultracold bosonic atoms in isolated double wells were detected. My project investigates the coherent many-particle dynamics, which takes place after coupling the double well. I provide the theoretical background for the next step, the observation of coherent many-particle dynamics after coupling the double wells. The tunability between the Bose-Hubbard model and the Heisenberg model in this setup could be used to study experimentally the differences in equilibration processes for non-integrable and Bethe ansatz integrable models. It turns out that the relaxation in the Heisenberg model is connected to a phase averaging effect, which is in contrast to the typical scattering driven thermalization in nonintegrable models In the second project I study a many-body generalization of the original Landau-Zener formula. This formula gives the transition probability between the two states of a quantum mechanical two-level system, where the offset between the two levels is varying linearly in time. In a recent experiment this framework has been extended to a many-body system consisting of pairwise tunnel-coupled one-dimensional Bose liquids. It was found that the tunnel coupling between the tubes and the intertube interactions strongly modify the original Landau-Zener picture. After a introduction to the two-level and the three-level Landau-Zener problem I present my own results for the quantum dynamics of the microscopic model and the comparison to the experimental results. I have calculated both Landau-Zener sweeps as well as the time-evolution after sudden quenches of the energy offset. A major finding is that for sufficiently large initial density quenches can be efficiently used to create quasi-thermal states of arbitrary temperatures. The third project is more mathematical and connects the fields of quantum computation and of quantum information. Here, the main purpose is to analyse systematically the effects of decoherence on maximally entangled multi-partite states, which arise typically during quantum computation processes. The bigger the number of entangled qubits the more fragile is its entanglement under the influence decoherence. As starting point I consider first two entangled qubits, whereby one qubit interacts with an arbitrary environment. For this particular case I have derived a factorization law for the disentanglement. Next, I calculate the decrease of entanglement of two , three and four entangled qubits, general W- and general GHZ-state, coupled to a global spin-1/2 bath or several independent spin-1/2 baths , one for each qubit. Although there is no appropriate entanglement measure for three and more qubits, it turns out that this decrease is directly related to the increase of entanglement between the central system and the bath. This implies the formation of a much bigger multipartite entangled network. Thus, using the von Neumann entropy and the Wootters concurrence, I derive a simple upper bound for the bath-induced entanglement breaking power of the initially maximally entangled multi-partite states.