The extraordinary success of quantum mechanics and its formalism has been established thanks to countless experiments with microscopic systems. Nevertheless, it is still not clear whether and when the quantum world ends, allowing for the emergence of classical phenomena. The extension of quantum properties to macroscopic system gives rise to paradoxes, as the well-known Schrödinger’s cat example. Among the alternatives to quantum mechanics, collapse models propose an objective modification of standard quantum theory to restore macrorealism at large scale. They predict a loss of coherence when scaling towards macroscopic systems, due to a spontaneous collapse mechanism included into the dynamics through non-linear stochastic modifications of the Schrödinger equation. Assessing and characterizing these models is a noteworthy endeavour in the exploration of the quantum-to-classical transition. The overarching goal of this Thesis is to address some of these fundamental issues, by exploring the concept of macrorealism and probing collapse models, making use of optomechanical setups. To answer the question whether a system has a quantum or classical dynamics, we will propose a theoretical test of Leggett-Garg inequalities, as tool to probe the macrorealism of an optomechanical system. We will investigate collapse models through the study of the dynamics of an optomechanical cavity, looking for signatures in the noise spectrum. Further, we will use the hypothesis testing framework and quantum metrology tools to distinguish dynamical channels encoding the presence or the lack of the collapse. Our findings show a violation of Leggett-Garg inequalities, suggesting that the demarcation line of the quantum domain can be pushed further to include larger systems. Our approaches for testing collapse models provide novel methodologies to better discriminate these effects and the results represent another step forward in the attempt of gaining a better understanding of the foundations of physics.
The extraordinary success of quantum mechanics and its formalism has been established thanks to countless experiments with microscopic systems. Nevertheless, it is still not clear whether and when the quantum world ends, allowing for the emergence of classical phenomena. The extension of quantum properties to macroscopic system gives rise to paradoxes, as the well-known Schrödinger’s cat example. Among the alternatives to quantum mechanics, collapse models propose an objective modification of standard quantum theory to restore macrorealism at large scale. They predict a loss of coherence when scaling towards macroscopic systems, due to a spontaneous collapse mechanism included into the dynamics through non-linear stochastic modifications of the Schrödinger equation. Assessing and characterizing these models is a noteworthy endeavour in the exploration of the quantum-to-classical transition. The overarching goal of this Thesis is to address some of these fundamental issues, by exploring the concept of macrorealism and probing collapse models, making use of optomechanical setups. To answer the question whether a system has a quantum or classical dynamics, we will propose a theoretical test of Leggett-Garg inequalities, as tool to probe the macrorealism of an optomechanical system. We will investigate collapse models through the study of the dynamics of an optomechanical cavity, looking for signatures in the noise spectrum. Further, we will use the hypothesis testing framework and quantum metrology tools to distinguish dynamical channels encoding the presence or the lack of the collapse. Our findings show a violation of Leggett-Garg inequalities, suggesting that the demarcation line of the quantum domain can be pushed further to include larger systems. Our approaches for testing collapse models provide novel methodologies to better discriminate these effects and the results represent another step forward in the attempt of gaining a better understanding of the foundations of physics.
An open problem in modern physics is why microscopic quantum objects can be at two places at once (i.e. a superposed quantum state) while macroscpoic classical object never show such a behaviour. Collapse models provides a quantitative answer for this problem and explain how macroscopic classical world emerges out of microscopic quantum world. A universal noise field is postulated in collapse models, inducing appropriate Brownian- motion corrections to standard quantum dynamics. The strength of collapse-driven Brownian fluctuations depend on: (i) the parameters characterizing the system (e.g., mass, size, density), and (ii) two phenomenological parameters defining the statistical properties of the collapse noise. The collapse-driven Brownian motion works such that microscopic systems behave quantum mechanically, while macroscopic objects are classical. At the intermediate mesocopic scale, collapse models predict deviations from standard quantum predictions. This issue has been subject of experimental tests. All experiments to date have been at the scales where collapse effects are negligible for all practical purposes. However, recent experimental progress in revealing quantum features of larger objects, increases the hope for testing at unprecedented scales where collapse models can be falsified. Current experiments are mainly focused on the preparation of macroscopic systems in a spatial quantum superposition state. The collapse effects would then manifest as loss of visibility in the observed inference pattern. However, one needs a quantum interference with single particles of mass ∼ 10 10 amu for a decisive test of collapse models. Creating such massive superpositionsis quite challenging, and beyond currectstate-of-the-art. Quite recently, an alternative approach has been proposed where the collapse manifests in the fluctuating properties of light interacting with the quantum system. The great advantage of this new approach is that here there is no need for the preparation of a quantum superposed state. It has been discussed that promising results can be revealed in the spectrum of light interacting with a radiation pressure-driven mechanical oscillator in a cavity optomechanics setting. Here, we review the theoretical modelling of the above optomechenical proposal. We discuss how collapse-driven Brownian motion modifies the spectrum. We quantify the collapse effect and explain how it depends on the parameters of the mechanical oscillator (e.g., mass, density, geometry).
While quantum theory has been tested to an incredible degree on microscopic scales, quantum effects are seldom observed in our everyday macroscopic world. The curious results of applying quantum mechanics to macroscopic objects are perhaps best illustrated by Erwin Schrödinger's famous thought experiment, where a cat can be put into a superposition state of being both dead and alive. Obviously, these quantum predictions are in stark contradiction to our common experience. Even with plenty of theoretical explanations put forward to explain this discrepancy, a large number of questions about the frontier between the quantum and the classical world remain unanswered. To distinguish between classical and quantum behavior, two fundamental concepts inherent to classical physics have been established over the years: The world view of local realism limits the power of classical experiments to establish correlations over space, while the world view of macroscopic realism (or macrorealism) restricts temporal correlations. Necessary conditions for both world views have been formulated in the form of Bell and Leggett-Garg inequalities, and Bell inequalities have been shown to be violated by quantum mechanics through increasingly conclusive experiments. Furthermore, many challenging steps towards convincing violations of macrorealism have been taken in a number of recent experiments. In the first part of this thesis, conditions for macrorealism are analyzed in detail. Two necessary conditions for macrorealism, the original Leggett-Garg inequality and the recently proposed no-signaling in time condition, are presented. It is then shown that a combination of no-signaling in time conditions is not only necessary but also sufficient for the existence of a macrorealistic description. Finally, an operational formulation of no-signaling in time, in terms of positive-operator valued measurements and Hamiltonians, is derived. In the next part, we argue that these results lead to a suitable definition of classical behavior. In particular, we provide a formalism to judge the classicality of measurements and time evolutions. We then proceed to apply it to a number of exemplary measurement operators and Hamiltonians. Finally, we argue for the importance of spontaneously realized Hamiltonians in our intuition of classical behavior. Next, differences between local realism and macrorealism are analyzed. For this purpose, the probability polytopes for spatially and temporally separated experiments are compared, and a fundamental difference in the power of quantum mechanics to build both types of correlations is discovered. This result shows that Fine's theorem, which states that a set of Bell inequalities is necessary and sufficient for local realism, is not transferable to macrorealism. Thus, (Leggett-Garg) inequalities are in principle not well-suited for tests of macrorealism, as they can never form a necessary and sufficient condition, and unnecessarily restrict the violating parameter space. No-signaling in time is both better suited and more strongly motivated from the underlying physical theory. In the final part of this thesis, a concrete experimental setup for implementing quantum experiments with macroscopic objects is proposed. It consists of a superconducting micro-sphere in the Meißner state, which is levitated by magnetic fields. Through its expelled magnetic field, the sphere's center-of-mass motion couples to a superconducting quantum circuit. Properly tuned, ground state cooling can be realized, since the sphere's motion is extremely well isolated from the surrounding environment. This setup therefore is a promising candidate for the observation of quantum effects in macroscopic systems.
The transition from the quantum to the classical realm remains one of the most profound open questions in physics. While quantum theory predicts the existence of macroscopic superpositions, their apparent absence in the everyday world is attributed either to environmental decoherence or to an intrinsic mechanism for wave-function collapse. This work presents a quantitative and experimentally grounded framework for distinguishing these possibilities. We propose a levitated optomechanical platform capable of generating controllable Schrodinger-cat states in the center of mass motion of a dielectric nanosphere. A comprehensive master equation incorporates gas collisions, black-body radiation, and photon-recoil noise, establishing a calibrated environmental baseline. The Continuous Spontaneous Localization (CSL) model is embedded within the same framework, predicting a characteristic saturation of the decoherence rate with superposition size and a quadratic scaling with mass. A Bayesian inference protocol is outlined to discriminate collapse induced excess decoherence from environmental noise. Together these elements provide a concrete experimental blueprint for a decisive test of quantum linearity, either revealing new physics beyond standard quantum mechanics or setting the most stringent bounds to date on objective-collapse parameters.
This thesis investigates three aspects of nonclassicality. The first aspect is macroscopic quantumness, a field which considers the properties of macroscopic superpositions. The various measures of macroscopicity are reviewed. An optomechanical system is described which enables us to study nonclassicality in macroscopic mechanical oscillators. We analyse the impact of different measurement settings on the macroscopicity of the mirror and the Wigner functions of the mechanical state. The same system is also considered under open system dynamics. The second nonclassical concept is the violation of macrorealism. It is shown that a two-level system can violate the Leggett-Garg inequality, thereby demonstrating that the assumptions of macrorealism do not hold. Similar dynamics are then replicated in a macroscopic mechanical system through the use of a hybrid optomechanical system in which an atom interacts with the mechanical oscillator through an optical mode. Mechanical damping is then factored into the dynamics to examine its effect on the violation of the Leggett-Garg inequality for different parameter ranges. The third is nonclassical correlations. Quantum discord and quantum entanglement are defined and several measures are explained. Entanglement distribution via separable states is introduced and then built on by adding imperfections to the operations in the protocol. It is found that the protocol is still successful in spite of the errors in the operations, both when they are unitary and non-unitary. We also develop a method of generating entanglement between two bosons through mediation with two spin systems. Through this system we demonstrate the creation of both entangled coherent states and NOON states.
The field of cavity optomechanics is based on the coupling of optical cavities to mechanical degrees of freedom. Over the past two decades, it has led to remarkable and surprising discoveries. A cavity optomechanical system enabled the first observation of gravitational waves, a discovery awarded with the 2017 Nobel prize, confirming Einstein's 100-year-old prediction. It was also a cavity optomechanical system that has for the first time enabled ground state cooling of the motion of an object containing ~1012 atoms, and entanglement of mechanical oscillators of similar size. Moreover, cavity optomechanical systems have facilitated significant progress in precision-sensing technologies, with diverse applications such as biosensing, magnetometry, and many more.But this may only be the beginning. The field is still in its early days and experimental capabilities are improving fast. For instance, cavity optomechanical systems have the potential to test predicted signatures of quantum gravity such as modifications to the canonical commutator, short-distance modifications to Newtonian gravity, dark matter and dark energy, and even extra dimensions. In this sense, they form an economical platform with a short experimental turnover time, that can compete in its predictive power with mega-scale, multi-billion-dollar experiments such as the Large Hadron Collider.This thesis is dedicated to utilizing cavity optomechanics to explore the maybe most challenging and unexplored frontier in quantum mechanics: The dynamics of macroscopic quantum systems. Quantum physics, since its discovery in the early 20th century, has revolutionized our understanding of the microworld, but has long been thought to apply exclusively to extremely small objects. However, over the past decades, ever-larger quantum systems have emerged in laboratories around the world. On one hand, these are collective, macroscopic quantum phenomena such as superfluidity, superconductivity, and Bose-Einstein condensation. On the other hand, they are quantum states of relatively massive mechanical objects. While our understanding of the interplay of quantum mechanical and classical systems has greatly improved over the past decades, as described by theories of decoherence and open quantum systems, many basic questions about macroscopic quantum systems still remain unanswered. Quantum fluids such as Bose-Einstein condensates and superfluid helium are inherently hard to understand due to their complex dynamics, and difficult to probe experimentally due to the weakness of their interactions with the environment and their fragile nature. This is especially true in the strongly-interacting regime, which is, for instance, found in superfluid helium.Another long-standing, unanswered set of questions in quantum mechanics is related to the quantum measurement problem. What constitutes a quantum measurement? What happens if we engineer a quantum state that is large enough to be, in principle, part of our everyday world? What if we attempt to create a quantum superposition of a living being? Do the laws of physics even permit either of these scenarios?Cavity optomechanics is a unique and powerful platform to investigate macroscopic quantum systems. The extreme sensitivity of cavity optomechanical sensors in readout of mechanical motion makes them susceptible to minute quantum effects. The strong coupling between single photons and phonons in these systems allows engineering and measurement of quantum states of mechanical systems. Furthermore, most cavity optomechanical experiments are cryo-compatible and small in size, which allows integration with other quantum systems to be analyzed, such as superfluid helium.
Optomechanics has made great strides in theory and experiments over the past decade, which culminated in the first direct detection of gravitational waves in 2015 by LIGO. This thesis explores how optomechanics can be used to test fundamental physics other than the theory of general relativity. Our emphasis will be on falsifiable theories (ultimately, only experiments can decide whether a theory is correct) that address two outstanding issues in quantum mechanics: the measurement problem, and reconciling quantum mechanics with the theory of general relativity. In particular, we show that the space experiment LISA pathfinder places aggressive bounds on two objective collapse models, which are non-linear stochastic modifications of the Schroedinger equation that can resolve the measurement problem. Moreover, we show that state-of-the-art torsion pendulum experiments can test the Schroedinger-Newton theory, which is the non-relativistic limit of a non-linear theory combining quantum mechanics with a fundamentally classical spacetime. Along the way, we propose how to resolve two major difficulties with determining the predictions of non-linear quantum mechanics in an actual experiment. First, we cannot use the density matrix formalism in non-linear quantum mechanics and so we have to suggest and justify a particular ensemble for the thermal bath. Separating out quantum and classical fluctuations helped us propose a reasonable ensemble. Second, most researchers believe that deterministic non-linear quantum mechanics must violate the no-signaling condition. We show this isn't necessarily the case because different interpretations of quantum mechanics make different predictions in non-linear quantum mechanics. We propose an interpretation, the causal-conditional prescription, that doesn't violate causality by noticing that once we fix an initial state, the evolution of a system under many non-linear theories is equivalent to evolution under a linear Hamiltonian with feedback. The mapping allows us to leverage the tools of quantum control, and it tells us that if the non-linear parameters of a non-linear Hamiltonian respond causally (i.e. with an appropriate delay) to measurement results, then the theory can be made causal. We also contribute to the theory of quantum optomechanics. We introduce two new bases that one can view environment modes with. In linear optomechanics a system interacts with an infinite number of bath modes. We show that the interaction can be reduced to one with finite degrees of freedom. Moreover, at any particular time, the system is correlated with only a finite number of bath modes. We show that if we make the assumption that we can measure any commuting environment modes, then this basis allows us to understand the one-shot quantum Cramer-Rao bound in a simple way, and allows us to sweep large parameter regimes and so find promising optomechanics topologies for quantum state preparation tasks that we can then analyze without the assumption of being able to measure any observable of the environment. We also use this basis to show that when we are interested in the conditional dynamics of a test mass, we can only adiabatically eliminate a lossy cavity when we measure the optomechanical system at a slow enough rate. Finally, we develop an analytic filter for obtaining the state of a generic optomechanical system that interacts linearly with its environment and is driven by Gaussian states, and where the outgoing light is measured with a non-linear photon-counting measurement. We hope that our work will help researchers explore optomechanics topologies that make use of photon counters.