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Optics Communications

Generation of photon pairs in time-lapse entangled quantum states by spontaneous four-wave mixing in nonlinear fiber-optic ring resonators

W.F. da Silva, J.L.S. Lima, A. F. G. F. Filho, Kleber Zuza Nobrega, M.M. Freire, A.S.B. Sombra

Published Mar 19, 2026• 0 citations
Publisher

Abstract

Quantum entanglement has been an extremely active field of research, both theoretically and experimentally. Studies on entanglement are fundamental to improving our basic understanding of quantum mechanics. As our understanding of the phenomenon grows, so does interest in using it to advance various technological fields: communications, computing, and sensing, to name just a few. It is now known that entangled photon pairs can be generated through a process known as Spontaneous Four-Wave Mixing (SFWM). In this paper, we report the generation of entangled photon pairs in time intervals by spontaneous four-wave mixing in a nonlinear fiber optic ring resonator. The requirements for efficient SFWM are quite similar to those for classical FWM, but they require even greater precision, especially for quantum applications. To achieve a measurable pair generation rate, a high-intensity pump laser is essential. The nonlinear medium must have high nonlinearity and confinement. This technique is compatible with contemporary fiber, enabling compact, low-cost, and scalable implementations such as quantum memories.

DOI
10.1016/j.optcom.2026.133125

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Quantum entanglement has been an extremely active field of research, both theoretically and experimentally. Studies on entanglement are fundamental to improving our basic understanding of quantum mechanics. As our understanding of the phenomenon grows, so does interest in using it to advance various technological fields: communications, computing, and sensing, to name just a few. It is now known that entangled photon pairs can be generated through a process known as Spontaneous Four-Wave Mixing (SFWM). In this paper, we report the generation of entangled photon pairs in time intervals by spontaneous four-wave mixing in a nonlinear fiber optic ring resonator. The requirements for efficient SFWM are quite similar to those for classical FWM, but they require even greater precision, especially for quantum applications. To achieve a measurable pair generation rate, a high-intensity pump laser is essential. The nonlinear medium must have high nonlinearity and confinement. This technique is compatible with contemporary fiber, enabling compact, low-cost, and scalable implementations such as quantum memories.
In recent years, there has been a spurring research interest growing on photonics integrated circuits as the way to scale up quantum communications. In particular, building a reliable integrated source of entangled photons is one of the main challenges remaining for commercial exploitation in quantum sensing and metrology. Therefore, advances in design of integrated sources of entangled photons is a necessary and crucial task to be performed for miniaturization and cost-effectiveness. Microring resonators are one of the most promising candidates to generate entangled photons via nonlinear interactions, especially Spontaneous Four-Wave Mixing (SFWM). But fabrication limitations in reproducibility of high-quality resonators mandate the use of active devices. Here we present the results of preparing the excitation pulse with different spectral, intensity and dispersion parameters to optimize the quantum efficiency in passive devices after fabrication. Different numerical methods such as Finite Difference Time Domain (FDTD) and Split-Step Fourier Method (SSFM) are used to reproduce the nonlinear propagation, interplay with dispersion and losses. Exploiting the degree of freedom of the excitation pulse can bring more energy efficient and passive devices as quantum entangled pair sources in an integrated chip. Considerations on different degrees of entanglement are also discussed for applications in quantum sensing and quantum metrology.
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Entangled photons have acted as a workhorse in many quantum technologies, including cryptography, imaging, sensing, and computation. With the growing demands of quantum technology, the entangled photon pair sources are required to be compact and integrable. For the last few years, the field of quantum optics in the nanoscale has demonstrated photon pair generation in ’flat’ optics such as thin layers, Van der Waals crystals, micro-, nano-antennas, and metasurfaces. The word ’flat’ is used because such optical platforms have sub-wavelength thicknesses. Due to the short travel length inside the sources, they can possess multiple functions that their bulky counterparts cannot have. This doctoral thesis addresses photon pair generation in ’flat’ optics via second- and third-order nonlinear processes, which are spontaneous parametric down-conversion (SPDC) and spontaneous four-wave mixing (SFWM). The main aims of the thesis are to understand how the photon pair generation is realized via SPDC and SFWM on subwavelength-scale platforms, and to make a bridge between photon pair generation via two nonlinear processes under the presence of optical resonances. The thesis covers two experimental parts related to SPDC and SFWM, and one future expectation of the SFWM in metamaterials. The first part of the thesis addresses one of the multi-functionalities that has recently been reported: the emission direction control of the photon pairs. A 150 nm-thick gallium phosphide (GaP) metasurface is used as a source. The metasurface supports a quasi-bound state in the continuum (quasi-BIC) resonance, enhancing the electric field inside the material. I generate the entangled photons through the SPDC process. The generated photons are in two different wavelengths under the given pump wavelength: signal photon at the resonance, and idler photon out of the resonance. The photon pair generation rate is enhanced by 66 times compared to the unpatterned GaP slab since the vacuum field in the signal mode is enhanced by the resonance. The generated photons obey the transmission spectrum of the metasurface. As a result, the signal photons at resonance are mostly reflected, and the idler photons are transmitted after generation. This result is the first work of photon demultiplexing by a metasurface. The second part of the thesis covers the photon pair generation through SFWM in thin nonlinear films. Silicon-rich silicon nitride (SiN) layers are selected as the sources. The layers have an intriguing characteristic that the third-order nonlinear susceptibility (chi-3) differs with the nitrogen doping rate. I generate the photon pairs through chi-3 variant SiN layers. The thicknesses of the samples are all sub-wavelength level, having a few hundred nanometers. Time-energy correlation measurements are conducted for all samples, and the second-order correlation functions (g(2)(0)) are calculated. The maximum g(2)(0) of the samples exceeds 2. Interestingly, I observed two-photon interference effects between photon pairs generated in the layers and the fused-silica substrate, which allows me to estimate the chi-3 values of the samples by knowing the reference: chi-3 value of the substrate. The last part of the thesis introduces designs of metasurfaces and possible experimental schemes for photon pair generation through SFWM. Yet, due to its weak light-matter interaction in third-order nonlinear processes, the photon pair generation through SFWM has not been observed in metasurfaces. However, it is fairly possible to enhance the vacuum fields at the output photon modes and generate photon pairs because preliminary work in unpatterned slabs has already been observed in this thesis. Finally, I introduce a fabricated metasurface. It needs improvements, but it is quite promising for the ongoing project.
Four-wave mixing in optical fibers has been proven to have many applications within processing of classical optical signals. In addition, recent developments in multimode fibers have made it possible to achieve the necessary phase-matching for efficient four-wave mixing over a very wide bandwidth. Thus, the combination of multimode fiber optics and four-wave mixing is very attractive for various applications. This is especially the case for applications in quantum communication, for example in photon-pair generation. This is the subject of this work, where we discuss the impact of fluctuations in core radius on the quality of the heralded single-photon states and demonstrate experimental results of intermodal spontaneous four-wave mixing for photon-pair generation.
Silicon micro-ring resonators have been demonstrated to be potential “on- chip” efficient sources of time-energy entangled photons. In these devices, photon pairs are generated by spontaneous four-wave-mixing (SFWM), an elastic scattering event involving two pump photons that results in the generation of an idler and a signal photon. The mass production of such integrated devices for quantum optic experiment requires the implementation of fast and reliable techniques to monitor the emitted two-photon state as well as the device performances. In this work we show that the joint spectral density of photon pairs that would be generated by SFWM in a silicon ring resonator can be measured with unprecedented resolution and speed, improving of several orders of magnitudes the results of traditional approaches based on coincidence measurements.