This thesis investigates the cascaded photon interactions and spectral properties of a waveguide quantum electrodynamics system, with a focus on the interaction between spontaneous emission and a distant ensemble of laser-cooled Cesium atoms coupled to an optical nanofiber. We fabricate optical nanofibers with a diameter of approximately 400 nm using a tapering machine and integrate the nanofibers into the system in which the atoms in a magneto-optical trap interact with the nanofiber mode. We explore how spontaneous emission from a first atomic ensemble, reflected by a distant fiber Bragg grating mirror, interacts with a second ensemble, forming a cascaded configuration. Spectral measurements reveal broadening effects consistent with reabsorption and dephasing mechanisms. These effects are incorporated into theoretical models, yielding agreement with experimental observations and providing insight into non-Markovian dynamics. Additionally, we implement a two-color dipole trap and evaluate the coupling efficiency of trapped atoms to the optical nanofibers.
This thesis investigates the cascaded photon interactions and spectral properties of a waveguide quantum electrodynamics system, with a focus on the interaction between spontaneous emission and a distant ensemble of laser-cooled Cesium atoms coupled to an optical nanofiber. We fabricate optical nanofibers with a diameter of approximately 400 nm using a tapering machine and integrate the nanofibers into the system in which the atoms in a magneto-optical trap interact with the nanofiber mode. We explore how spontaneous emission from a first atomic ensemble, reflected by a distant fiber Bragg grating mirror, interacts with a second ensemble, forming a cascaded configuration. Spectral measurements reveal broadening effects consistent with reabsorption and dephasing mechanisms. These effects are incorporated into theoretical models, yielding agreement with experimental observations and providing insight into non-Markovian dynamics. Additionally, we implement a two-color dipole trap and evaluate the coupling efficiency of trapped atoms to the optical nanofibers.
We demonstrate the first experimental realization of cascaded resonance fluorescence over a 64-meter propagation delay time between two spatially and temporally independent ensembles of laser-cooled Cesium atoms coupled to an optical nanofiber. Spontaneously emitted photons from a strongly driven first ensemble are guided through a standard fiber, reflected by a fiber Bragg grating mirror, and interact with a second ensemble, producing a unidirectional two-node cascaded system. The cascaded fluorescence spectrum is broadened and blue-shifted relative to the original fluorescence spectrum. Our simple model reproduces the power broadening and the cascaded fluorescence spectrum, as well as the ratio of cascaded to original photon flux, giving insight into non-Markovian dynamics. Our results establish the longest-distance one-way cascaded atom-photon interface reported to date, providing a stepping stone towards a fiber-based platform for quantum networking.
We have recently demonstrated a new experimental platform for trapping and optically interfacing laser-cooled cesium atoms. The scheme uses a two-color evanescent field surrounding an optical nanofiber to localize the atoms in a one-dimensional optical lattice 200 nm above the nanofiber surface [1]. In order to use this fiber-coupled ensemble of trapped atoms for applications in the context of quantum communication and quantum information processing, non-classical states of the atomic spins have to be prepared and should live long enough to allow one to apply successive quantum gates. The close proximity of the trapped atoms to the nanofiber surface and the strong polarization gradients of nanofiber-guided light fields are potentially important sources of decoherence. Here, we present our latest experimental results on the coherence properties of atomic spins in our nanofiber-based trap. Using a microwave field to drive the clock transition, we determine inhomogeneous and homogeneous dephasing times by Ramsey and spin echo techniques, respectively. Our results constitute the first measurement of the coherence properties of atoms trapped in the vicinity of a nanofiber and represent a fundamental step towards establishing nanofiber-based traps for cold atoms as a building block in a quantum network.
Optical nanofibers provide a versatile platform for exploring strong light-matter interactions at the single-quantum level, a central goal of quantum optics. Their subwavelength diameter supports tightly confined guided modes with strong evanescent fields, enabling efficient coupling between photons and nearby atoms. By incorporating fiber Bragg gratings, nanofibers can form fully fiber-integrated high-finesse cavities, combining strong atom-photon coupling with efficient and low-loss optical input-output interfacing in the setting of cavity quantum electrodynamics (QED). In parallel, nanofiber systems naturally realize waveguide QED, where atoms interact strongly with propagating photons in a one-dimensional geometry. In this review, we introduce the underlying physical principles, summarize key experimental techniques and representative phenomena, and discuss prospects for applications in quantum information processing, quantum networks, and related quantum technologies.
In this thesis, I present the realization of a fiber-optical interface using optically trapped cesium atoms, which is an efficient tool for coupling light and atoms. The basic principle of the presented scheme relies on the trapping of neutral cesium atoms in a two-color evanescent field surrounding a nanofiber. The strong confinement of the fiber guided light, which also protrudes outside the nanofiber, provides strong confinement of the atoms as well as efficient coupling to near-resonant light propagating through the fiber. In chapter 1, the necessary physical and mathematical background describing the propagation of light in an optical fiber is presented. The exact solution of Maxwell’s equations allows us to model fiber-guided light fields which give rise to the trapping potentials and the atom-light coupling in the close vicinity of a nanofiber. Chapter 2 gives the theoretical background of light-atom interaction. A quantum mechanical model of the light-induced shifts of the relevant atomic levels is reviewed, which allows us to quantify the perturbation of the atomic states due to the presence of the trapping light-fields. The experimental realization of the fiber-based atom trap is the focus of chapter 3. Here, I analyze the properties of the fiber-based trap in terms of the confinement of the atoms and the impact of several heating mechanisms. Furthermore, I demonstrate the transportation of the trapped atoms, as a first step towards a deterministic delivery of individual atoms. In chapter 4, I present the successful interfacing of the trapped atomic ensemble and fiber-guided light. Three different approaches are discussed, i.e., those involving the measurement of either near-resonant scattering in absorption or the emission into the guided mode of the nanofiber. In the analysis of the spectroscopic properties of the trapped ensemble we find good agreement with the prediction of theoretical model discussed in chapter 2. In addition, I introduce a non-destructive scheme for the interrogation of the atoms states, which is sensitive to phase shifts of far-detuned fiber-guided light interacting with the trapped atoms. The inherent birefringence in our system, induced by the atoms, changes the state of polarization of the probe light and can be thus detected via a Stokes vector measurement.
New effects can arise in quantum physics when there is strong coupling, either between atoms and light or between different quantum systems. This thesis examines an optical nanofiber atom trap as a mediator of atom-light interactions and a potential element of a hybrid quantum system. The evanescent field around the sub-wavelength waist of an optical nanofiber possesses a small mode area that increases the cooperativity between atoms and the mode, in a manner analogous to traditional cavity QED. We demonstrate trapping of 87Rb atoms with an optical nanofiber, confining hundreds of atoms with typical trap lifetimes of tens of milliseconds. We then employ single photon counting techniques to study untrapped ensembles of cold atoms around the nanofiber. A first experiment uses intensity autocorrelations of resonance fluorescence emitted into the nanofiber mode to observe a transition from classical to nonclassical photon statistics. Measuring the correlations on longer timescales reveals the motion of atoms through the optical mode, and we develop a correspondence between the transit time and atomic cloud temperature. A second experiment measures Purcell enhancement of spontaneous emission of atoms near the nanofiber by correlating their fluorescence with a known trigger event. The spontaneous decay rate of an atom near a dielectric is modified by the induced dipole and by a change in the modes of the vacuum electromagnetic field. Our observed enhancement of 6.5±0.9% over the free-space rate matches well with what one finds from mode simulations in our system.
Summary form only given. Reversible light-matter interfaces are crucial elements in quantum optics and quantum information networks. In particular, the coupling of one-dimensional bosonic nanoscale waveguides and cold atoms appears as a promising pathway to build strong light-matter interaction thanks to the tight transverse confinement of light.Recently, our group has developed an interface where light, tightly guided by a subwavelength-diameter optical fiber (nanofiber), strongly interacts with atoms near its vicinity. In this case, a single atom close to the surface can absorb a non-negligible fraction of the guided light, as the effective area of the mode is comparable with the atomic cross-section. Moreover, using this configuration, it is possible to generate an in-fiber dipole trap for atoms in the vicinity of the waveguide. Using this all-fibered interface we have recently demonstrated the realization of an optical memory at the single photon level [1]. Here, we will describe the most recent result using this new interface: the observation of a large Bragg reflection off a 1D optical lattice [2]. The ability to control photon transport in 1D waveguides coupled to spin systems would allow for novel quantum network capabilities and many-body effects emerging from long-range interactions.