We demonstrate the first experimental realization of cascaded resonance fluorescence over a 64-meter propagation delay time between two spatially and temporally independent ensembles of laser-cooled Cesium atoms coupled to an optical nanofiber. Spontaneously emitted photons from a strongly driven first ensemble are guided through a standard fiber, reflected by a fiber Bragg grating mirror, and interact with a second ensemble, producing a unidirectional two-node cascaded system. The cascaded fluorescence spectrum is broadened and blue-shifted relative to the original fluorescence spectrum. Our simple model reproduces the power broadening and the cascaded fluorescence spectrum, as well as the ratio of cascaded to original photon flux, giving insight into non-Markovian dynamics. Our results establish the longest-distance one-way cascaded atom-photon interface reported to date, providing a stepping stone towards a fiber-based platform for quantum networking.
We demonstrate the first experimental realization of cascaded resonance fluorescence over a 64-meter propagation delay time between two spatially and temporally independent ensembles of laser-cooled Cesium atoms coupled to an optical nanofiber. Spontaneously emitted photons from a strongly driven first ensemble are guided through a standard fiber, reflected by a fiber Bragg grating mirror, and interact with a second ensemble, producing a unidirectional two-node cascaded system. The cascaded fluorescence spectrum is broadened and blue-shifted relative to the original fluorescence spectrum. Our simple model reproduces the power broadening and the cascaded fluorescence spectrum, as well as the ratio of cascaded to original photon flux, giving insight into non-Markovian dynamics. Our results establish the longest-distance one-way cascaded atom-photon interface reported to date, providing a stepping stone towards a fiber-based platform for quantum networking.
This thesis investigates the cascaded photon interactions and spectral properties of a waveguide quantum electrodynamics system, with a focus on the interaction between spontaneous emission and a distant ensemble of laser-cooled Cesium atoms coupled to an optical nanofiber. We fabricate optical nanofibers with a diameter of approximately 400 nm using a tapering machine and integrate the nanofibers into the system in which the atoms in a magneto-optical trap interact with the nanofiber mode. We explore how spontaneous emission from a first atomic ensemble, reflected by a distant fiber Bragg grating mirror, interacts with a second ensemble, forming a cascaded configuration. Spectral measurements reveal broadening effects consistent with reabsorption and dephasing mechanisms. These effects are incorporated into theoretical models, yielding agreement with experimental observations and providing insight into non-Markovian dynamics. Additionally, we implement a two-color dipole trap and evaluate the coupling efficiency of trapped atoms to the optical nanofibers.
Integrating the scalability of individually addressable arrays of optical-tweezer-trapped single atoms with the efficient light-matter interface provided by nanophotonic waveguides has been a long-standing challenge in quantum technologies based on atoms and photons. Here we realize a quantum interface between photons guided in an optical nanofiber with a diameter of 310 nm and an array of on average 155 individually addressable atoms. Using a spatial light modulator and an objective lens with NA = 0.45, single cesium atoms are trapped in a one-dimensional array of 200 optical tweezer spots with micrometer-scale trap sizes on the nanofiber. Individual atoms are addressed by spatially scanning an excitation laser beam, focused to a spot size comparable to that of the traps through the same objective lens, along the nanofiber. We confirm the single-atom nature of the individual trapping sites through photon-correlation measurements of the guided fluorescence, observing strong photon antibunching with g(2)(0)≈0.26. We measure trap lifetimes of a few hundred milliseconds, with a maximum value of 460 ms, at an atom-surface separation of 670 nm without active cooling, representing an order-of-magnitude improvement over previous nanofiber traps. This platform opens a new regime for atom-photon interfaces, paving the way for scalable distributed quantum computing and quantum networks, as well as for the exploration of collective radiative effects in waveguide QED with individually addressable atoms.
We have recently demonstrated a new experimental platform for trapping and optically interfacing laser-cooled cesium atoms. The scheme uses a two-color evanescent field surrounding an optical nanofiber to localize the atoms in a one-dimensional optical lattice 200 nm above the nanofiber surface [1]. In order to use this fiber-coupled ensemble of trapped atoms for applications in the context of quantum communication and quantum information processing, non-classical states of the atomic spins have to be prepared and should live long enough to allow one to apply successive quantum gates. The close proximity of the trapped atoms to the nanofiber surface and the strong polarization gradients of nanofiber-guided light fields are potentially important sources of decoherence. Here, we present our latest experimental results on the coherence properties of atomic spins in our nanofiber-based trap. Using a microwave field to drive the clock transition, we determine inhomogeneous and homogeneous dephasing times by Ramsey and spin echo techniques, respectively. Our results constitute the first measurement of the coherence properties of atoms trapped in the vicinity of a nanofiber and represent a fundamental step towards establishing nanofiber-based traps for cold atoms as a building block in a quantum network.
Summary form only given. Reversible light-matter interfaces are crucial elements in quantum optics and quantum information networks. In particular, the coupling of one-dimensional bosonic nanoscale waveguides and cold atoms appears as a promising pathway to build strong light-matter interaction thanks to the tight transverse confinement of light.Recently, our group has developed an interface where light, tightly guided by a subwavelength-diameter optical fiber (nanofiber), strongly interacts with atoms near its vicinity. In this case, a single atom close to the surface can absorb a non-negligible fraction of the guided light, as the effective area of the mode is comparable with the atomic cross-section. Moreover, using this configuration, it is possible to generate an in-fiber dipole trap for atoms in the vicinity of the waveguide. Using this all-fibered interface we have recently demonstrated the realization of an optical memory at the single photon level [1]. Here, we will describe the most recent result using this new interface: the observation of a large Bragg reflection off a 1D optical lattice [2]. The ability to control photon transport in 1D waveguides coupled to spin systems would allow for novel quantum network capabilities and many-body effects emerging from long-range interactions.
Tapered optical fibers with a nanofiber waist are versatile tools for interfacing light and matter. In this context, laser-cooled atoms trapped in the evanescent field surrounding the optical nanofiber are of particular interest: They exhibit both long ground-state coherence times and efficient coupling to fiber-guided fields. Here, we demonstrate electromagnetically induced transparency, slow light, and the storage of fiber-guided optical pulses in an ensemble of cold atoms trapped in a nanofiber-based optical lattice. We measure a slow-down of light pulses to group velocities of 50 m/s. Moreover, we store optical pulses at the single photon level and retrieve them on demand in the fiber after 2 microseconds with an overall efficiency of (3.0 +/- 0.4) %. Our results show that nanofiber-based interfaces for cold atoms have great potential for the realization of building blocks for future optical quantum information networks.
Fluorescence of atoms has been the subject of interest in quantum optical measurementsfor many years. The atomic fluorescence is routinely used as a tool to detectatoms, to generate photons and to generate non-classical states of light. One of thewidely used methods to investigate the atomic fluorescence is laser-induced fluorescencespectroscopy. This thesis presents the development of optical nanofibers as atool for the measurement of fluorescence spectrum of atoms.Optical nanofibers are ultrathin optical fibers, with diameters less than the propagationwavelength of the fiber, with a silica core and a vacuum clad. Such opticalnanofibers can support only the single propagating guided-mode. The guided-modesof the nanofiber is confined in the transverse direction of the nanofiber and a partof the propagating field lies outside the fiber, in the evanescent region of the fiber.The mode density of the electromagnetic field is modified by the nanofiber. Due tothe modification of mode density, the spontaneous emission of atoms is modified bythe optical nanofibers and the confinement of the guided-modes results in a strongchanneling of spontaneous emission of atoms into the guided-modes of the nanofiber.Such a property of nanofibers can be used to study fluorescence of atoms around thenanofiber.Optical nanofibers are prepared by the adiabatic tapering of single-mode opticalfibers. Our experiments are performed by overlapping cold Cesium atoms, from amagneto-optical trap (MOT), with the optical nanofiber and observing the fluorescencethrough the guided-modes of the nanofiber. The nanofiber suppresses with highprobability any coupling of scattering light from the excitation laser into the guidedmodesand high coupling efficiency of fluorescence into the guided-modes enables us tomeasure the fluorescence spectrum of atoms present around the nanofiber with a goodsignal-to-noise ratio. In this thesis, we demonstrate the measurement of laser inducedfluorescence (LIF) emission spectra of strongly driven atoms using optical nanofibers.For the fluorescence emission spectrum measurements, we develop and demonstrate anew sensitive and high resolution method consisting of optical heterodyne techniqueand photon correlation spectroscopy. The key point of the method is to extract theinformation of first-order field correlation function from the measured second-orderintensity correlation function. The Fourier transform of the field correlation functionthen gives the fluorescence emission spectrum.The atoms emitting fluorescence in the guided-modes of the nanofiber lie very closeto the nanofiber surface and are subjected to atom-surface interactions. It has beenreported in earlier experiments on nanofiber, that such surface interactions can bemodified by irradiating the MOT-atoms overlapped with the nanofiber with UV lasers.After such irradiations, MOT-atoms are kept from falling into the surface-potentialand behave almost like free-space atoms around the nanofiber. We first perform ourfluorescence spectra measurements under this free-atom conditions. The observedexcitation spectrum lineshape shows a free-atom like Lorentzian behavior, with avery small tail in the red-detuned side (red-tail). The red-tail has been attributedto photoassociation process, due to atoms making transition from free ground statesto bound excited states of the surface potential. Under this conditions, the emissionspectra measured for on-resonant and off-resonant excitations show the well-knownthree-peak Mollow-triplet spectrum of free-space two-level atoms. The observationconfirms that the near surface atoms behave like free-space atoms. Also, the quantitativeagreement between the observed spectra with the theoretical calculationsdemonstrates the validity of the optical nanofiber method for measuring fluorescenceemission spectrum of atoms.As mentioned above, since we are observing near-surface atoms, fluorescence measurementsbased on optical nanofibers may become a unique tool to probe atomsurfaceinteractions. In earlier experiments using nanofiber, signatures of atomsurfaceinteraction have been observed in the excitation spectrum of atoms, in theform of a broad red-tail. The lineshape of the excitation spectrum is understood as aresult of a process where atoms approaching the nanofiber surface fall into the shallowsurface potential, forming long-range atom-surface bound states. In this thesis,we have systematically investigated the evolution of the lineshape of the excitationspectrum from a Lorentzian shape to a broad red-tail condition. The evolution of thespectrum lineshape has been attributed to the changing nanofiber surface condition.The spectrum shape is found to depend on the flux of background Cs-atoms. Wespeculate that this might be due to the adsorption of hot background atoms ontothe nanofiber surface, which changes the surface condition of the nanofiber locallyand helps in loading of cold MOT-atoms into the shallow surface potential. We havefound that the effect of UV laser irradiation is to photoionize the MOT-atoms, andthe generated photoelectrons might help in the desorption of adsorbed atoms on thesurface. We discuss the roles of adsorption and desorption of atoms on the surfaceconditions. We have shown that such changing surface condition can be controlledby adjusting the hot background atom flux and the UV laser intensity. Under suchcontrolled surface condition, we have measured the emission spectrum. The observedemission spectrum under the broad red-tail condition can be explained only by includingthe surface interactions. We also discuss qualitatively the phonon-mode densityfor nanofiber at room temperature and the phonon-mediated decay of atoms in thesurface potential.This work may open up the way for using optical nanofibers as a tool to investigatethe laser-induced fluorescence spectrum of strongly driven atoms, and to study atomsurfaceinteractions. In the future, we hope to create optical dipole traps around thenanofibers by introducing trap laser lights through the guided-modes and performfluorescence measurements of these trapped atoms.