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Quantum State Generation with Nonlinear Integrated Photonics: Conventional and Unconventional Approaches

Milica Banić

Published Jun 1, 2024• 0 citations
OpenAlex

Abstract

In this thesis we study the generation of non-classical states of light using nonlinear integrated photonics. We focus first on third-order parametric down-conversion (TOPDC), a process in which pump photons can be down-converted into photon triplets, and which could serve as a source of non-Gaussian states and tripartite discrete-variable entanglement. We investigate the possibility of implementing TOPDC in conventional integrated structures. By comparing the estimated triplet generation rates in a waveguide and a microring resonator, we establish that non-resonant structures appear to be a more promising platform for a near-term demonstration of TOPDC, due to the high generation bandwidth enhancing the rate of triplet generation. We estimate generation rates of ~10 triplets per second for a 1-cm-long waveguide driven by a 100 mW CW pump, a rate that is comparable to or higher than those quoted for other proposals. We then estimate the non-Gaussianity that might be expected in a supermode of the field generated by our sample structures. The predicted non-Gaussianity is negligible in both structures, for different reasons: The generation rate in the ring is too low, while the field generated by the waveguide is highly multimode. We conclude that although a simple SiN waveguide may be a suitable source for a first demonstration of optical TOPDC, the design will need to be improved significantly for observations of non-Gaussianity or tripartite entanglement in the generated light. Indeed, state generation protocols based on conventional spontaneous four-wave mixing sources and postselection appear to be more promising in the near term. We adopt this approach to design integrated sources of postselected multipartite states in a frequency bin encoding scheme. We introduce sources of W states and GHZ states, with kHz generation rates expected for picojoule pump pulses. This platform appears to be promising for the generation of more arbitrary states, including high-dimensional ones consisting of entangled qudits. We review a graph-based strategy that may be useful for designing other devices, and for understanding the limitations of this platform.

Related papers

Generation of photon pairs by stimulated emission in ring resonators

Milica Banić, Marco Liscidini, John E. Sipe

Third-order parametric downconversion (TOPDC) describes a class of nonlinear interactions in which a pump photon is converted into a photon triplet. This process can occur spontaneously or it can be stimulated by seeding fields. Here we show that stimulated TOPDC (StTOPDC) can be exploited for the generation of quantum correlated photon pairs. We model StTOPDC in a microring resonator, predicting observable pair generation rates in a microring engineered for third-harmonic generation, and we examine the peculiar features of this approach when compared with second-order spontaneous parametric downconversion and spontaneous four-wave mixing. We conclude that if the experimental difficulties associated with implementing StTOPDC can be overcome, it may soon be possible to demonstrate this process in resonant integrated devices.

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Tunable Quantum Optics in Index-Guiding Fibres

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The spontaneous decay of a pump photon into a tripartite entangled photon state (photon triplets) has been extensively studied in theory. Observation of these photon triplets at optical frequencies is of interest for fundamental science and future applications of quantum optics, such as quantum computing and quantum cryptography. This decay is known as spontaneous third-order parametric down-conversion (TOPDC). Experimentally, TOPDC has not been demonstrated in the optical frequency domain. TOPDC is enabled by the third-order nonlinearity of the material in which the interaction takes place. In optical fibres, the effective nonlinearity of the glass is increased manifold. The reason for this is the long light-matter interaction length and the tight confinement of light in the waveguide. Optical fibres are therefore the ideal platform for the observation of TOPDC, provided that phase matching can be achieved. In this thesis, the use of submicrometre fibre tapers is studied in the context of TOPDC, both in experiment and theory. Comparing different fibre-based TOPDC sources, fibre tapers rank among the highest in terms of expected triplet generation rate. At the same time, the background noise generated in these fibres is very low, which leads to a high expected three-photon coincidence-to-accidental ratio (CAR) on the order of 7000. In the experiments related to TOPDC, the precision of manufacturing fibre tapers is studied. A novel gas-based mechanism for dispersion tuning is demonstrated. Without this mechanism the manufacturing precision of the fibre tapers would not suffice to observe TOPDC in an experiment. The tuning mechanism is demonstrated using third-harmonic generation, which is the inverse process of TOPDC. The resonant third-harmonic radiation generated around 460nm can be tuned at a rate of −0.118nm/bar. This is achieved by introducing pressurised argon in the taper environment. The background noise from fibre tapers is characterised. The effect of the tuning mechanism on the three-photon-state and the signal-to-noise ratio is studied in theory. In another part of the thesis, gas-filled suspended-core fibres (SCFs) are used as a spectrally tunable source of entangled photon pairs (biphotons). Generation of biphotons via spontaneous four-wave mixing (FWM) in fibres offers great advantages over the generation in bulk crystals, which is the commonly employed technique. The most important advantages are the excellent control of the spatial mode structure, the extra degrees of freedom for dispersion design and the possibility to integrate the fibres into existing networks. Yet, fibre biphoton sources lack the convenient spectral tunability of crystal-based sources. Introducing pressurised gas into the hollow channels of the SCF is demonstrated to be a convenient and broadband spectral tuning mechanism. The FWM-sidebands can be continuously tuned at a rate of −0.3 THz/bar, in the quantum and in the seeded scenario. A high two-photon-CAR exceeding 10000 is measured for the biphoton state, and the frequency entangled joint-spectral intensity is measured. Finally, seeded FWM is used to characterise the core size of high-NA submicrometre fibres to a nanometre precision. If ultrafast pulses are used instead of nanosecond pulses, this will present a non-destructive and high precision characterisation technique for such fibres. The results of this work present an important step towards realising TOPDC at optical frequencies in the near future. The experimental realisation of a broadly tunable biphoton source combines the convenient tuning mechanism found in crystal-based sources with the advantages of fibre-based biphoton generation. Such tunable fibre biphoton sources can therefore be competitive with crystal-based systems for quantum optics applications.

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Non-Hermitian quantum and classical integrated nonlinear photonics

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Integrated optical quantum circuits based on photonic waveguiding structures are increasingly gaining attention as a possible solution for scalable quantum technologies with important applications to quantum simulations. Quantum communication provides secure information transmission, but the distance over which quantum states of light can be distributed without significant disturbance is limited due to inescapable losses and noise in optical elements. Loss is the greatest challenge facing the implementation of integrated photonic technologies, and it is inescapable in experimental reality. In recent years there is a rise of interest in structures with spatially inhomogeneous losses. Light propagation in waveguiding structures with spatially distributed sections of loss can be used for implementation of quantum plasmonic circuits, which are able to strongly confine light to sub-wavelength dimensions, as well as for parity-time (PT) symmetric structures, with phase transition associated with PT-symmetry breaking, which opens new possibilities for light manipulation. The PhD thesis contains research on the controllable classical and quantum dynamics of optical frequency conversion processes in quadratically nonlinear photonic integrated circuites in the presence of losses. Namely, I discuss spontaneous parametric down-conversion (SPDC), sum-frequency generation (SFG) and optical parametric amplification (OPA) in nonlinear structures governed by non-Hermition Hamiltonians. I explore the fundamental features of multi-photon generation in integrated nonlinear waveguides. I have been shown that arrays of coupled nonlinear waveguides can serve as a robust integrated platform for the generation of entangled photon states with nonclassical spatial correlations through spontaneous parametric down-conversion (SPDC), and that the operation of such quantum circuit is tolerant even to relatively high losses. Furthermore, I have studied the bi-photon multimode quantum emission tomography in waveguide structures with spatially inhomegeneous losses. The PhD thesis also covers the research on the effect of these losses in waveguide couplers possessing parity-time (PT) symmetry. I have identified an anti-PT spectral symmetry of a parametric amplifier based on those couplers. Finally, I describe the single-photon conversion to a photon pair, and identify opportunities for the efficient enhancement of this process.

•Jan 1, 2016•0 citations

An Integrated Approach to Third-order Parametric Down-conversion

Milica Banić, Marco Liscidini, John E. Sipe

We propose an integrated platform for the deterministic generation of non-Gaussian states by third-order parametric down-conversion. We suggest an approach to its experimental demonstration by photon triplet detection, predicting a rate up to 100 Hz.

•Jan 1, 2023•0 citations
In this thesis we study the generation of non-classical states of light using nonlinear integrated photonics. We focus first on third-order parametric down-conversion (TOPDC), a process in which pump photons can be down-converted into photon triplets, and which could serve as a source of non-Gaussian states and tripartite discrete-variable entanglement. We investigate the possibility of implementing TOPDC in conventional integrated structures. By comparing the estimated triplet generation rates in a waveguide and a microring resonator, we establish that non-resonant structures appear to be a more promising platform for a near-term demonstration of TOPDC, due to the high generation bandwidth enhancing the rate of triplet generation. We estimate generation rates of ~10 triplets per second for a 1-cm-long waveguide driven by a 100 mW CW pump, a rate that is comparable to or higher than those quoted for other proposals. We then estimate the non-Gaussianity that might be expected in a supermode of the field generated by our sample structures. The predicted non-Gaussianity is negligible in both structures, for different reasons: The generation rate in the ring is too low, while the field generated by the waveguide is highly multimode. We conclude that although a simple SiN waveguide may be a suitable source for a first demonstration of optical TOPDC, the design will need to be improved significantly for observations of non-Gaussianity or tripartite entanglement in the generated light. Indeed, state generation protocols based on conventional spontaneous four-wave mixing sources and postselection appear to be more promising in the near term. We adopt this approach to design integrated sources of postselected multipartite states in a frequency bin encoding scheme. We introduce sources of W states and GHZ states, with kHz generation rates expected for picojoule pump pulses. This platform appears to be promising for the generation of more arbitrary states, including high-dimensional ones consisting of entangled qudits. We review a graph-based strategy that may be useful for designing other devices, and for understanding the limitations of this platform.
Third-order parametric downconversion (TOPDC) describes a class of nonlinear interactions in which a pump photon is converted into a photon triplet. This process can occur spontaneously or it can be stimulated by seeding fields. Here we show that stimulated TOPDC (StTOPDC) can be exploited for the generation of quantum correlated photon pairs. We model StTOPDC in a microring resonator, predicting observable pair generation rates in a microring engineered for third-harmonic generation, and we examine the peculiar features of this approach when compared with second-order spontaneous parametric downconversion and spontaneous four-wave mixing. We conclude that if the experimental difficulties associated with implementing StTOPDC can be overcome, it may soon be possible to demonstrate this process in resonant integrated devices.
The spontaneous decay of a pump photon into a tripartite entangled photon state (photon triplets) has been extensively studied in theory. Observation of these photon triplets at optical frequencies is of interest for fundamental science and future applications of quantum optics, such as quantum computing and quantum cryptography. This decay is known as spontaneous third-order parametric down-conversion (TOPDC). Experimentally, TOPDC has not been demonstrated in the optical frequency domain. TOPDC is enabled by the third-order nonlinearity of the material in which the interaction takes place. In optical fibres, the effective nonlinearity of the glass is increased manifold. The reason for this is the long light-matter interaction length and the tight confinement of light in the waveguide. Optical fibres are therefore the ideal platform for the observation of TOPDC, provided that phase matching can be achieved. In this thesis, the use of submicrometre fibre tapers is studied in the context of TOPDC, both in experiment and theory. Comparing different fibre-based TOPDC sources, fibre tapers rank among the highest in terms of expected triplet generation rate. At the same time, the background noise generated in these fibres is very low, which leads to a high expected three-photon coincidence-to-accidental ratio (CAR) on the order of 7000. In the experiments related to TOPDC, the precision of manufacturing fibre tapers is studied. A novel gas-based mechanism for dispersion tuning is demonstrated. Without this mechanism the manufacturing precision of the fibre tapers would not suffice to observe TOPDC in an experiment. The tuning mechanism is demonstrated using third-harmonic generation, which is the inverse process of TOPDC. The resonant third-harmonic radiation generated around 460nm can be tuned at a rate of −0.118nm/bar. This is achieved by introducing pressurised argon in the taper environment. The background noise from fibre tapers is characterised. The effect of the tuning mechanism on the three-photon-state and the signal-to-noise ratio is studied in theory. In another part of the thesis, gas-filled suspended-core fibres (SCFs) are used as a spectrally tunable source of entangled photon pairs (biphotons). Generation of biphotons via spontaneous four-wave mixing (FWM) in fibres offers great advantages over the generation in bulk crystals, which is the commonly employed technique. The most important advantages are the excellent control of the spatial mode structure, the extra degrees of freedom for dispersion design and the possibility to integrate the fibres into existing networks. Yet, fibre biphoton sources lack the convenient spectral tunability of crystal-based sources. Introducing pressurised gas into the hollow channels of the SCF is demonstrated to be a convenient and broadband spectral tuning mechanism. The FWM-sidebands can be continuously tuned at a rate of −0.3 THz/bar, in the quantum and in the seeded scenario. A high two-photon-CAR exceeding 10000 is measured for the biphoton state, and the frequency entangled joint-spectral intensity is measured. Finally, seeded FWM is used to characterise the core size of high-NA submicrometre fibres to a nanometre precision. If ultrafast pulses are used instead of nanosecond pulses, this will present a non-destructive and high precision characterisation technique for such fibres. The results of this work present an important step towards realising TOPDC at optical frequencies in the near future. The experimental realisation of a broadly tunable biphoton source combines the convenient tuning mechanism found in crystal-based sources with the advantages of fibre-based biphoton generation. Such tunable fibre biphoton sources can therefore be competitive with crystal-based systems for quantum optics applications.
The main goal of this thesis is to study nonlinear photonic devices from the perspective of generation of non-classical states of light through the process of parametric down-conversion, also considering practical aspects. Periodically-poled waveguides as well as relatively new Bragg reflection waveguides are studied as a promising bright sources for integrated platforms. Possible limitations by imperfections of fabrication process are considered as well. More common bulk crystals are also used to generate more complex entangled states and fields, whose correlations properties are studied not only at single-photon level, but also in a mesoscopic domain.
We demonstrate that genuine multipartite entangled states can be generated using frequency bin encoding in integrated photonic platforms. We introduce a source of four-photon GHZ states and a source of three-photon W states. We predict generation rates on the order of 104{10}^{4}104 Hz for a silicon microring source with milliwatt pump powers. These results, along with the versatility and scalability of integrated structures, identify this as a promising approach for the generation of higher-dimensional and larger entangled states.
Integrated optical quantum circuits based on photonic waveguiding structures are increasingly gaining attention as a possible solution for scalable quantum technologies with important applications to quantum simulations. Quantum communication provides secure information transmission, but the distance over which quantum states of light can be distributed without significant disturbance is limited due to inescapable losses and noise in optical elements. Loss is the greatest challenge facing the implementation of integrated photonic technologies, and it is inescapable in experimental reality. In recent years there is a rise of interest in structures with spatially inhomogeneous losses. Light propagation in waveguiding structures with spatially distributed sections of loss can be used for implementation of quantum plasmonic circuits, which are able to strongly confine light to sub-wavelength dimensions, as well as for parity-time (PT) symmetric structures, with phase transition associated with PT-symmetry breaking, which opens new possibilities for light manipulation. The PhD thesis contains research on the controllable classical and quantum dynamics of optical frequency conversion processes in quadratically nonlinear photonic integrated circuites in the presence of losses. Namely, I discuss spontaneous parametric down-conversion (SPDC), sum-frequency generation (SFG) and optical parametric amplification (OPA) in nonlinear structures governed by non-Hermition Hamiltonians. I explore the fundamental features of multi-photon generation in integrated nonlinear waveguides. I have been shown that arrays of coupled nonlinear waveguides can serve as a robust integrated platform for the generation of entangled photon states with nonclassical spatial correlations through spontaneous parametric down-conversion (SPDC), and that the operation of such quantum circuit is tolerant even to relatively high losses. Furthermore, I have studied the bi-photon multimode quantum emission tomography in waveguide structures with spatially inhomegeneous losses. The PhD thesis also covers the research on the effect of these losses in waveguide couplers possessing parity-time (PT) symmetry. I have identified an anti-PT spectral symmetry of a parametric amplifier based on those couplers. Finally, I describe the single-photon conversion to a photon pair, and identify opportunities for the efficient enhancement of this process.