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Disquisitions on quantum-enhanced polarimetry

Aaron Z. Goldberg

Published Jun 1, 2021• 0 citations
OpenAlex

Abstract

It takes some convincing to realize that light has a polarization degree of freedom, as our eyes are usually ignorant of light's polarization. Since overcoming this hurdle of intuition, polarization has become a fantastic resource that can be easily manipulated both physically and mathematically, opening the door to a wide variety of applications. We have only recently begun to appreciate how many more doors are opened by the quantum mechanical degrees of freedom inherent to optical polarization. One use of optical polarization is for polarimetry: measuring the changes in light's polarization after it interacts with a material is an excellent procedure for nondestructively probing the characteristics and composition of the intervening material. More sensitive measurements require brighter probe light; however, sufficiently intense light will begin to destroy the sample being probed. In this thesis, we seek to provide more sensitive polarimetry without resorting to bright beams of light. Tailoring the quantum properties of various states of light has been shown to increase their usefulness for other estimation protocols and we show how to extend this paradigm to quantum enhancements in polarimetry. We begin by finding the quantum states underlying classical polarization. Each particular set of classical polarization properties corresponds to a large variety of quantum states. Next, we establish quantum descriptions of classical polarization transformations corresponding to arbitrary Jones and Mueller matrices, including quantum mechanical insights into the distinction between processes that can and cannot be described by Jones matrices. We propose candidates for the most likely quantum states underlying classical decompositions into polarized and unpolarized fractions, carefully inspecting how these quantum states behave under polarization transformations. This language allows us to inspect quantum-enhanced sensing in the multiparameter context of polarimetry. We show the dramatic possibilities for quantum enhancements in any metrological scenario that is mathematically equivalent to a rotation, of which polarization rotations are a primary example; in contrast, we also show most attenuating and depolarizing polarization transformations to forbid such dramatic enhancements. Finally, we discuss polarization and its generalizations in the context of generating quantum entanglement via linear optics. These applications serve as mere examples of the usefulness promised by light’s quantum polarization degrees of freedom.

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It takes some convincing to realize that light has a polarization degree of freedom, as our eyes are usually ignorant of light's polarization. Since overcoming this hurdle of intuition, polarization has become a fantastic resource that can be easily manipulated both physically and mathematically, opening the door to a wide variety of applications. We have only recently begun to appreciate how many more doors are opened by the quantum mechanical degrees of freedom inherent to optical polarization. One use of optical polarization is for polarimetry: measuring the changes in light's polarization after it interacts with a material is an excellent procedure for nondestructively probing the characteristics and composition of the intervening material. More sensitive measurements require brighter probe light; however, sufficiently intense light will begin to destroy the sample being probed. In this thesis, we seek to provide more sensitive polarimetry without resorting to bright beams of light. Tailoring the quantum properties of various states of light has been shown to increase their usefulness for other estimation protocols and we show how to extend this paradigm to quantum enhancements in polarimetry. We begin by finding the quantum states underlying classical polarization. Each particular set of classical polarization properties corresponds to a large variety of quantum states. Next, we establish quantum descriptions of classical polarization transformations corresponding to arbitrary Jones and Mueller matrices, including quantum mechanical insights into the distinction between processes that can and cannot be described by Jones matrices. We propose candidates for the most likely quantum states underlying classical decompositions into polarized and unpolarized fractions, carefully inspecting how these quantum states behave under polarization transformations. This language allows us to inspect quantum-enhanced sensing in the multiparameter context of polarimetry. We show the dramatic possibilities for quantum enhancements in any metrological scenario that is mathematically equivalent to a rotation, of which polarization rotations are a primary example; in contrast, we also show most attenuating and depolarizing polarization transformations to forbid such dramatic enhancements. Finally, we discuss polarization and its generalizations in the context of generating quantum entanglement via linear optics. These applications serve as mere examples of the usefulness promised by light’s quantum polarization degrees of freedom.
Measuring the polarization states of light and their variations, a process known as polarimetry, is essential to modern metrology, especially within the field of optical rotation. However, enhancing the precision of such measurements by improving the detectors is challenging, primarily due to the limitation in photoelectric response. By contrast, the scheme of quantum polarimetry has shown that exploiting correlated particles as the probe can provide an enhancement in the precision. Inspired by the scheme, by introducing correlations among classical light beams, we demonstrate that the precision of polarimetry focused on optical rotation can be enhanced. This conclusion is supported by both our theoretical analysis and experimental results. And we call it correlated optical polarimetry. Because the correlated beams we consider are spatially separable, a distributed optical rotation polarimetry scheme is given, which can be applied for the detection of spatially distributed but homogeneous objects. Our results show that the maximal improvements of the precision scales are proportional to the square root of the probe number, and we verify the results by experiments when the probe number is 2, 4, and 6. The scaling of precision improvements mathematically resembles the transition from shot-noise scaling to Heisenberg scaling in quantum metrology, but works for a classical light detection system. Hence, it helps enhance the traditional light-based polarization measure and other relevant practical applications.
Conventional polarimetry, including schemes leveraging entangled light, characterizes optical samples through linear transformations of polarization states. We introduce a two-photon probing approach in which both photons of an entangled pair interact with the same depolarizing medium simultaneously. In this regime, the transformation of the two-photon polarization correlations becomes quadratic in the Mueller matrix, enabling access to second-order polarization information beyond conventional polarimetry. We develop a theoretical framework linking the Mueller matrix to the evolution of the two-photon polarization correlation tensor and show that depolarization induces quadratic degradation of entanglement and state purity. Experiments using polarization-entangled photon pairs transmitted through controlled scattering media confirm the predicted response and reveal enhanced sensitivity to polarization scrambling compared with single-photon probing. These results establish two-photon probing as a higher-order quantum polarimetric modality for characterizing polarization channels.
Quantum approaches relying on entangled photons have been recently proposed to increase the efficiency of optical measurements. We demonstrate here that, surprisingly, the use of classical light with entangled degrees of freedom can also bring outstanding advantages over conventional measurements in polarization metrology. Specifically, we show that radially polarized beams of light allow to perform real-time single-shot Mueller matrix polarimetry. Our results also indicate that quantum optical procedures requiring entanglement without nonlocality can be actually achieved in the classical optics regime.
The insights offered by quantum mechanics to the field of optical metrology are many-fold, with non-classical states of light themselves used to make sensors that surpass the sensitivity of sensors using classical states of light. Unfortunately, this advantage, referred to often as "super-sensitivity" is notoriously fragile, and even the slightest experimental imperfections may greatly reduce the efficacy of the non-classical sensors, sometimes completely obviating their advantage. In my thesis I have shown that the performance of an otherwise ideal two-photon interferometer, which exploits entanglement between photons to make super-sensitive measurements of phase, is crippled by the slightest introduction of decoherence between modes of the interferometer. I have shown further that such drastic reduction in sensitivity can also appear in classical measurement problems, specifically that the recently developed methods of estimating the separation between a pair of point sources are rendered less effective when the ideal assumption of complete spatial incoherence is relaxed. Towards overcoming these and other issues, I have designed new configurations that use ancillary optical degrees of freedom, a tool-set that has recently garnered much interest in the field of quantum optics. In the context of two-photon interferometry, I have shown that by coupling polarization to the spatial-structure of the two photon state used to probe phase it is possible to obviate the need for a reference phase, even in the context of decoherence and imperfections in the interferometer. In the context of two-point resolution, I have developed an anisotropic imaging system that performs the function of an image-inversion interferometer and is inherently stable, offering an attractive implementation of recently developed methods of sub-Rayleigh imaging. I have further shown both theoretically and experimentally that the same anisotropic image-inversion interferometer is useful in measuring spatially encoded phases, both in the context of classical illumination as well as quantum-aided two-photon super-sensing. In both cases, the ability to perform interferometric measurements of the spatial structure of an electric field without splitting beam paths forms a bridge between conception and implementation of precision-sensing measurement strategies. Finally, I have shown that binary interferometric method based on the common-path anisotropic imaging system that I introduced, are able to measure both phase gradients and transverse beam tilts with a sensitivity beating conventional systems that are used both commercially and in research laboratories.
Abstract Classical polarimetry is a well-established discipline with diverse applications across different branches of science. The burgeoning interest in leveraging quantum resources to achieve highly sensitive measurements has spurred researchers to elucidate the behavior of polarized light within a quantum mechanical framework, thereby fostering the development of a quantum theory of polarimetry. In this work, drawing inspiration from polarimetric investigations in biological tissues, we investigate the precision limits of polarization rotation angle estimation about a known rotation axis, in a quantum polarimetric process, comprising three distinct quantum channels. The rotation angle to be estimated is induced by the retarder channel on the Stokes vector of the probe state. The diattenuator and depolarizer channels, acting on the probe state, can be thought of as effective noise processes. We explore the precision constraints inherent in quantum polarimetry by evaluating the quantum Fisher information for probe states of significance in quantum metrology, namely NOON, Kings of Quantumness, and Coherent states. The effects of the noise channels as well as their ordering is analyzed on the estimation error of the rotation angle to characterize practical and optimal quantum probe states for quantum polarimetry. Furthermore, we propose an experimental framework tailored for NOON state quantum polarimetry, aiming to bridge theoretical insights with empirical validation.