Quantum approaches relying on entangled photons have been recently proposed to increase the efficiency of optical measurements. We demonstrate here that, surprisingly, the use of classical light with entangled degrees of freedom can also bring outstanding advantages over conventional measurements in polarization metrology. Specifically, we show that radially polarized beams of light allow to perform real-time single-shot Mueller matrix polarimetry. Our results also indicate that quantum optical procedures requiring entanglement without nonlocality can be actually achieved in the classical optics regime.
Quantum approaches relying on entangled photons have been recently proposed to increase the efficiency of optical measurements. We demonstrate here that, surprisingly, the use of classical light with entangled degrees of freedom can also bring outstanding advantages over conventional measurements in polarization metrology. Specifically, we show that radially polarized beams of light allow to perform real-time single-shot Mueller matrix polarimetry. Our results also indicate that quantum optical procedures requiring entanglement without nonlocality can be actually achieved in the classical optics regime.
Quantum correlations are non-classical features of quantum systems that can be harnessed in new technologies. Nonlocality, a unique byproduct of the entanglement of more than one particle, can alter the causal sequence that is present in a classical measurement. In this work, we investigate a nonlocal form of Mueller polarimetry. In the classical method, light prepared in an initial state passes through a sample whose polarization properties are unknown, and the light's modified polarization state is subsequently measured. From a series of measurements, the Mueller matrix is obtained, which contains the polarization properties of the sample. In the nonclassical version of the technique presented here, the initial and final parts of this measurement were split into polarization projections on two polarization-entangled photons, but linked through quantum correlations in the post-selection process. We found the results with samples of known and unknown Mueller matrix using this approach to be equivalent to the classical ones. The nonlocal feature of the measurement can invert the causal order of preparation and measurement in the classical method. We present a study of its limitations when the entangled state of the photons is not the ideal one. From this work, we conclude that the technique is very resilient to imperfections in the quantum state of the photons, making it a feasible alternative to the classical method.
It takes some convincing to realize that light has a polarization degree of freedom, as our eyes are usually ignorant of light's polarization. Since overcoming this hurdle of intuition, polarization has become a fantastic resource that can be easily manipulated both physically and mathematically, opening the door to a wide variety of applications. We have only recently begun to appreciate how many more doors are opened by the quantum mechanical degrees of freedom inherent to optical polarization. One use of optical polarization is for polarimetry: measuring the changes in light's polarization after it interacts with a material is an excellent procedure for nondestructively probing the characteristics and composition of the intervening material. More sensitive measurements require brighter probe light; however, sufficiently intense light will begin to destroy the sample being probed. In this thesis, we seek to provide more sensitive polarimetry without resorting to bright beams of light. Tailoring the quantum properties of various states of light has been shown to increase their usefulness for other estimation protocols and we show how to extend this paradigm to quantum enhancements in polarimetry. We begin by finding the quantum states underlying classical polarization. Each particular set of classical polarization properties corresponds to a large variety of quantum states. Next, we establish quantum descriptions of classical polarization transformations corresponding to arbitrary Jones and Mueller matrices, including quantum mechanical insights into the distinction between processes that can and cannot be described by Jones matrices. We propose candidates for the most likely quantum states underlying classical decompositions into polarized and unpolarized fractions, carefully inspecting how these quantum states behave under polarization transformations. This language allows us to inspect quantum-enhanced sensing in the multiparameter context of polarimetry. We show the dramatic possibilities for quantum enhancements in any metrological scenario that is mathematically equivalent to a rotation, of which polarization rotations are a primary example; in contrast, we also show most attenuating and depolarizing polarization transformations to forbid such dramatic enhancements. Finally, we discuss polarization and its generalizations in the context of generating quantum entanglement via linear optics. These applications serve as mere examples of the usefulness promised by light’s quantum polarization degrees of freedom.
Measuring the polarization states of light and their variations, a process known as polarimetry, is essential to modern metrology, especially within the field of optical rotation. However, enhancing the precision of such measurements by improving the detectors is challenging, primarily due to the limitation in photoelectric response. By contrast, the scheme of quantum polarimetry has shown that exploiting correlated particles as the probe can provide an enhancement in the precision. Inspired by the scheme, by introducing correlations among classical light beams, we demonstrate that the precision of polarimetry focused on optical rotation can be enhanced. This conclusion is supported by both our theoretical analysis and experimental results. And we call it correlated optical polarimetry. Because the correlated beams we consider are spatially separable, a distributed optical rotation polarimetry scheme is given, which can be applied for the detection of spatially distributed but homogeneous objects. Our results show that the maximal improvements of the precision scales are proportional to the square root of the probe number, and we verify the results by experiments when the probe number is 2, 4, and 6. The scaling of precision improvements mathematically resembles the transition from shot-noise scaling to Heisenberg scaling in quantum metrology, but works for a classical light detection system. Hence, it helps enhance the traditional light-based polarization measure and other relevant practical applications.
We present a method to determine the Mueller matrix of a sample using polarization-entangled photon pairs. One of the photons of a pair goes through a sample and is then subject to a polarization projection measurement. The other photon, which does not go through the sample, is also subject to a polarization projection. The measured quantum correlations are equivalent to polarimetry measurements, where the initial state of the photon going through the sample is determined by the polarization projection on the entangled partner that does not go through the sample. The correspondence with the classical system is acausal because quantum measurements apply to distinct Hilbert spaces. We tested this method with standard optical elements finding excellent agreement with the expectations. Thus it can be used as an alternative to classical Mueller polarimetry for conditions that would be challenging to do otherwise.
Conventional polarimetry, including schemes leveraging entangled light, characterizes optical samples through linear transformations of polarization states. We introduce a two-photon probing approach in which both photons of an entangled pair interact with the same depolarizing medium simultaneously. In this regime, the transformation of the two-photon polarization correlations becomes quadratic in the Mueller matrix, enabling access to second-order polarization information beyond conventional polarimetry. We develop a theoretical framework linking the Mueller matrix to the evolution of the two-photon polarization correlation tensor and show that depolarization induces quadratic degradation of entanglement and state purity. Experiments using polarization-entangled photon pairs transmitted through controlled scattering media confirm the predicted response and reveal enhanced sensitivity to polarization scrambling compared with single-photon probing. These results establish two-photon probing as a higher-order quantum polarimetric modality for characterizing polarization channels.
We explore the concepts of coherence and entanglement as they apply to both the classical and quantum natures of light. In the classical domain, we take inspiration from the tools and concepts developed in foundational quantum mechanics and quantum information science to gain a better understanding of classical coherence theory of light with multiple degrees of freedom (DoFs). First, we use polarization and spatial parity DoFs to demonstrate the notion of classical entanglement, and show that Bell's measure can serve as a useful tool in distinguishing between classical optical coherence theory. Second, we establish a methodical yet versatile approach called 'optical coherency matrix tomography' for reconstructing the coherency matrix of an electromagnetic beam with multiple DoFs. This technique exploits the analogy between this problem in classical optics and that of tomographically reconstructing the density matrix associated with multipartite quantum states in quantum information science. Third, we report the first experimental measurements of the 4 x 4 coherency matrix associated with an electromagnetic beam in which polarization and a spatial DoF are relevant, ranging from the traditional two-point Young's double slit to spatial parity and orbital angular momentum modes. In the quantum domain, we use the modal structure of classical fields to develop qubits and structure Hilbert spaces for use in quantum information processing. Advancing to three-qubit logic gates is an important step towards the success of optical schemes for quantum computing. We experimentally implement a variety of two- and three- qubit, linear and deterministic, single-photon, controlled, quantum logic gates using polarization and spatial parity qubits. Lastly, we demonstrate the implementation of two-qubit single-photon logic using polarization and orbital angular momentum qubits.