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Physical Review A

Superradiant Raman scattering with rubidium atoms in an optical cavity: Dynamical dispersive coupling and AC Stark shift effect

Huihui Yu, Gang Chen, Chongxin Shan, Yuan Zhang

Published Feb 25, 2026• 0 citations
Publisher
DOI
10.1103/81q3-zyjk

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Superradiant Raman scattering of Rubidium atoms has been explored in the experiment [Nature 484, 78 (2012)] to prove the concept of the superradiant laser, which attracts significant attentions in quantum metrology due to the expected ultra-narrow linewidth down to millihertz. To better understand the physics involved in this experiment, we have developed a quantum master equation theory by treating the Rubidium atoms as three-level systems, and coupling them with a dressed laser and an optical cavity. Our simulations show different superradiant Raman scattering pulses for the systems within the crossover and strong coupling regime, and the shifted and broader spectrum of the steady-state Raman scattering. Thus, our studies provide a unified view on the superradiant Raman scattering pulses, and an alternative explanation to the broad spectrum of the steady-state Raman scattering, as observed in the experiment. In future, our theory can be readily applied to study other interesting phenomena relying on the superradiant Raman scattering, such as magnetic field sensing, real-time tracking of quantum phase, Dicke phase transition of non-equilibrium dynamics and so on.
For the two-photon ac Stark effect in Raman-Ramsey configuration, such as the Raman clock, and pulsed CPT clock configuration, an interference phenomenon of two-photon ac Stark effect is predicted. Here we report this new physical phenomenon, the interference of two-photon ac Stark effect in two-zone Raman-Ramsey interactions, which is general in any Raman-Ramsey spectroscopy. In particular, for an atomic beam Raman clock configuration, the ac Stark shift will present an interference fringe caused by the separated oscillatory-field interaction when the shift fields interact with atoms at two zones. On the center of dispersion shape of normal ac-Stark shift, an interference pattern appeared when the scale of frequency detuning is expanded.
The theory of stimulated Raman scattering has been treated at various levels of sophistication from plane-wave steady-state models through 3-D transient quantum-electrodynamic calculations.1 Many physical effects, such as pump depletion, dispersion, level degeneracy, ac Stark shift, and parametric coupling of Stokes and anti-Stokes light, can be important in experimental setups. We describe a recently developed computer code which treats these effects in detail. The code is based on integration of the coupled Maxwell-Bloch equations of quantum optics. We discuss numerical predictions of the code relating to these effects and present applications to experimental investigations such as Raman beam cleanup and transient amplification.2