Entangled photons carry nontrivial quantum correlations that defy classical physics and provide new tools for monitoring quantum dynamics in molecules. The use of low-flux entangled photons in molecular spectroscopy has been proposed in the past to probe excited-state dynamics with enhanced temporal and spectral resolutions. However, these techniques have been challenging to implement experimentally since the resulting signal has a low signal-to-noise ratio. The signal strength can be boosted by using intense entangled-photon beams, where multiple pairs of entangled photons are present in the environment. This allows the molecule under study to interact with both entangled and unentangled photons, where the classical component of the spectroscopic signal stemming from the latter can mask the spectral features associated with the former. In this Letter, we show how the signal arising from unentangled photons can be eliminated when intense entangled-photon beams are used in two-dimensional electronic spectroscopy (2DES), and demonstrate the advantage of photonic entanglement.Entangled photons carry nontrivial quantum correlations that defy classical physics and provide new tools for monitoring quantum dynamics in molecules. The use of low-flux entangled photons in molecular spectroscopy has been proposed in the past to probe excited-state dynamics with enhanced temporal and spectral resolutions. However, these techniques have been challenging to implement experimentally since the resulting signal has a low signal-to-noise ratio. The signal strength can be boosted by using intense entangled-photon beams, where multiple pairs of entangled photons are present in the environment. This allows the molecule under study to interact with both entangled and unentangled photons, where the classical component of the spectroscopic signal stemming from the latter can mask the spectral features associated with the former. In this Letter, we show how the signal arising from unentangled photons can be eliminated when intense entangled-photon beams are used in two-dimensional electronic spectroscopy (2DES), and demonstrate the advantage of photonic entanglement.

Physical Review LettersNov 25, 20257 citations

Enhancing the absorption and energy transfer process via quantum entanglement

Xiao-Lan Zong, Wei Song, Jian Zhou +3 more

Quantum Information ProcessingMay 17, 20183 citations

Generation of maximally entangled states with subluminal Lorentz boosts

Veiko Palge, Jacob Dunningham

Recent work [J. Dunningham, V. Palge, and V. Vedral, Phys. Rev. A 80, 044302 (2009)] studied entanglement between the spin and momentum components of a single spin- $1/2$ particle and showed that maximal entanglement is obtained only when boosts approach the speed of light. Here we extend the boost scenario to general geometries and show that, intriguingly, maximal entanglement can be achieved with boosts less than the speed of light. Boosts approaching the speed of light may even decrease entanglement. We also provide a geometric explanation for this behavior.Recent work [J. Dunningham, V. Palge, and V. Vedral, Phys. Rev. A 80, 044302 (2009)] studied entanglement between the spin and momentum components of a single spin-$1/2$ particle and showed that maximal entanglement is obtained only when boosts approach the speed of light. Here we extend the boost scenario to general geometries and show that, intriguingly, maximal entanglement can be achieved with boosts less than the speed of light. Boosts approaching the speed of light may even decrease entanglement. We also provide a geometric explanation for this behavior.

arXiv:1207.5351Physical Review AApr 24, 201218 citations

Idler-free channel position finding

Jason L. Pereira, Leonardo Banchi, Quntao Zhuang +1 more

Entanglement is a powerful tool for quantum sensing, and entangled states can greatly boost the discriminative power of protocols for quantum illumination, quantum metrology, or quantum reading. However, entangled state protocols generally require the retention of an idler state, to which the probes are entangled. Storing a quantum state is difficult and so technological limitations can make protocols requiring quantum memories impracticable. One alternative is idler-free protocols that utilize nonclassical sources but do not require any idler states to be stored. Here we apply such a protocol to the task of channel position finding. This involves finding a target channel in a sequence of background channels, and has many applications, including quantum sensing, quantum spectroscopy, and quantum reading.Entanglement is a powerful tool for quantum sensing, and entangled states can greatly boost the discriminative power of protocols for quantum illumination, quantum metrology, or quantum reading. However, entangled state protocols generally require the retention of an idler state, to which the probes are entangled. Storing a quantum state is difficult and so technological limitations can make protocols requiring quantum memories impracticable. One alternative is idler-free protocols that utilize nonclassical sources but do not require any idler states to be stored. Here we apply such a protocol to the task of channel position finding. This involves finding a target channel in a sequence of background channels, and has many applications, including quantum sensing, quantum spectroscopy, and quantum reading.

arXiv:2010.10547Physical Review AApr 29, 202111 citations

Theoretical physics: Eyeing entanglement

NatureNov 1, 20080 citations

Recent work [J. Dunningham, V. Palge, and V. Vedral, Phys. Rev. A 80, 044302 (2009)] studied entanglement between the spin and momentum components of a single spin-

1/2

particle and showed that maximal entanglement is obtained only when boosts approach the speed of light. Here we extend the boost scenario to general geometries and show that, intriguingly, maximal entanglement can be achieved with boosts less than the speed of light. Boosts approaching the speed of light may even decrease entanglement. We also provide a geometric explanation for this behavior.