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LaserPhys Youth School-Conference

Frequency locking of three lasers to a single ULE-glass cavity for three-photon Rydberg excitation

Suliman Ghadeer

Published Jan 1, 2025• 0 citations
Publisher

Abstract

In this work, the description and implementation of a Pound-Drever-Hall (PDH) laser frequency stabilization system for a three-photon laser excitation scheme used to excite neutral rubidium-87 atoms to Rydberg states is presented. The three lasers (780 nm, 1367 nm, and 743 nm) are simultaneously frequency-locked to a single ultra-low-expansion (ULE) glass cavity. The first and second step lasers are locked to fixed frequencies, while the third step laser is frequency-swept during excitation to fine-tune the resonance. The setup demonstrates stable simultaneous locking of all three lasers and provides a foundation for enhanced stability and reduced linewidth in future implementations.

DOI
10.15862/83mnnpk25.41

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In this work, the description and implementation of a Pound-Drever-Hall (PDH) laser frequency stabilization system for a three-photon laser excitation scheme used to excite neutral rubidium-87 atoms to Rydberg states is presented. The three lasers (780 nm, 1367 nm, and 743 nm) are simultaneously frequency-locked to a single ultra-low-expansion (ULE) glass cavity. The first and second step lasers are locked to fixed frequencies, while the third step laser is frequency-swept during excitation to fine-tune the resonance. The setup demonstrates stable simultaneous locking of all three lasers and provides a foundation for enhanced stability and reduced linewidth in future implementations.
Quantum information processing using atomic qubits requires narrow linewidth lasers with long-term stability for high fidelity coherent manipulation of Rydberg states. In this paper, we report on the construction and characterization of three continuous-wave (CW) narrow linewidth lasers stabilized simultaneously to an ultra-high finesse Fabry-Perot cavity made of ultra-low expansion (ULE) glass, with a tunable offset-lock frequency. One laser operates at 852~nm while the two locked lasers at 1018~nm are frequency doubled to 509~nm for excitation of 133^{133}133Cs atoms to Rydberg states. The optical beatnote at 509~nm is measured to be 260(5)~Hz. We present measurements of the offset between the atomic and cavity resonant frequencies using electromagnetically induced transparency (EIT) for high-resolution spectroscopy on a cold atom cloud. The long-term stability is determined from repeated spectra over a period of 20 days yielding a linear frequency drift of ∼1\sim1∼1~Hz/s.
Abstract We present a self-assembled ultra-low expansion (ULE) cavity system designed for high-precision laser frequency stabilization. The cavity mirrors are bonded to the ULE spacer using a low thermal expansion adhesive, and the assembled cavity exhibits a finesse of nearly 3×1043 \times 10^{4}3×104. A custom-designed multilayer aluminum housing was developed to passively isolate the cavity from environmental fluctuations. Long-term performance characterization reveals a frequency drift of approximately 164 kHz per day.After locking a diode laser to the cavity using the Pound-Drever-Hall technique, we achieve a linewidth of approximately 19.4kHz19.4 \text{kHz}19.4kHz and a fractional frequency stability of6.4×10−136.4 \times 10^{-13}6.4×10−13 at 1 s.To validate the reliability of this frequency-stabilized laser system, we applied it to Rydberg excitation spectroscopy via trap-loss measurements of cold 87^{87}87Rb atoms. Compared to conventional wavelength meter locking, the cavity-stabilized system significantly improves spectral resolution, reducing the linewidth of the trap-loss spectrum from 34 MHz to 6 MHz. Our system offers a robust and cost-effective solution for high-resolution spectroscopy, with applications in coherent control of Rydberg atoms.
We describe the design, construction, and characterization of a medium-finesse Fabry-Perot cavity for simultaneous frequency stabilization of two lasers operating at 960 and 780 nm wavelengths, respectively. The lasers are applied in experiments with ultracold rubidium Rydberg atoms, for which a combined laser linewidth similar to the natural Rydberg linewidth (≈10 kHz) is desired. The cavity, with a finesse of ≈1500, is used to reduce the linewidth of the lasers to below this level. By using a spacer made of ultra low expansion (ULE) glass with active temperature stabilization, the residual frequency drift is limited to ≲1 MHz/day. The design optimizes for ease of construction, robustness, and affordability.
We propose and demonstrate an alternative method for spectral filtering and frequency stabilization of both 780-nm and 960-nm lasers using a high-finesse length-tunable cavity (HFLTC). Firstly, the length of HFLTC is stabilized to a commercial frequency reference. Then, the two lasers are locked to this HFLTC using the Pound–Drever–Hall (PDH) method which can narrow the linewidths and stabilize the frequencies of both lasers simultaneously. Finally, the transmitted lasers of HFLTC with each power up to about 100 μW, which act as seed lasers, are amplified using the injection locking method for single-atom Rydberg excitation. The linewidths of obtained lasers are narrowed to be less than 1 kHz, meanwhile the obtained lasers’ phase noise around 750 kHz are suppressed about 30 dB. With the spectrally filtered lasers, we demonstrate a Rabi oscillation between the ground state and Rydberg state of single-atoms in an optical trap tweezer with a decay time of (67 ± 37) μs, which is almost not affected by laser phase noise. We found that the maximum short-term laser frequency fluctuation of a single excitation lasers is at ∼3.3 kHz and the maximum long-term laser frequency drift of a single laser is ∼46 kHz during one month. Our work develops a stable and repeatable method to provide multiple laser sources of ultra-low phase noise, narrow linewidth, and excellent frequency stability, which is essential for high precision atomic experiments, such as neutral atom quantum computing, quantum simulation, quantum metrology, and so on.
We have proposed an artificial modulation-free Pound-Drever-Hall (PDH) method for laser frequency stabilization and demonstrated it via two-color polarization spectroscopy of Rydberg electromagnetically induced transparency (EIT) resonance in a room-temperature rubidium vapor. Due to the unique error signal profile, the conventional PDH method owns a large capture range in laser frequency locking. Here we manually construct a PDH error signal via a linear combination of polarization spectroscopies of the Rydberg EIT resonances without and with a magnetic field applied. The artificial modulation-free PDH error signal owns a subnatural linewidth dispersion curve as well as a large capture range with which we successfully stabilize the laser to an absolute atomic frequency reference in a long running time, immune to environmental fluctuation and even manmade impulse perturbation. This method can provide an absolute frequency reference based on atomic transition while keeping similar locking ability to provide corrections for frequency fluctuations over a broad bandwidth as the conventional PDH.
We demonstrate a three step laser stabilisation scheme for excitation to nP and nF Rydberg states in 85Rb, with all three lasers stabilised using active feedback to independent Rb vapour cells. The setup allows stabilisation to the Rydberg states 36P3/2 to 70P3/2 and 33F7/2 to 90F7/2, with the only limiting factor being the available third step laser power. We study the scheme by monitoring the three laser frequencies simultaneously against a self-referenced optical frequency comb. The third step laser, locked to the Rydberg transition, displays an Allan deviation of 30 kHz over 1 second and < 80 kHz over 1 hour. The scheme is very robust and affordable, and it would be ideal for carrying out a range of quantum information experiments.