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arXiv:1711.02645 · Journal of the Optical Society of America B

Sub-kilohertz excitation lasers for quantum information processing with Rydberg atoms

Remy Legaie, Craig Picken, Jonathan D. Pritchard

Published Mar 21, 2018• 35 citations
arXivHTMLPDF

Abstract

Quantum information processing using atomic qubits requires narrow linewidth lasers with long-term stability for high fidelity coherent manipulation of Rydberg states. In this paper, we report on the construction and characterization of three continuous-wave (CW) narrow linewidth lasers stabilized simultaneously to an ultra-high finesse Fabry-Perot cavity made of ultra-low expansion (ULE) glass, with a tunable offset-lock frequency. One laser operates at 852~nm while the two locked lasers at 1018~nm are frequency doubled to 509~nm for excitation of $^{133}$Cs atoms to Rydberg states. The optical beatnote at 509~nm is measured to be 260(5)~Hz. We present measurements of the offset between the atomic and cavity resonant frequencies using electromagnetically induced transparency (EIT) for high-resolution spectroscopy on a cold atom cloud. The long-term stability is determined from repeated spectra over a period of 20 days yielding a linear frequency drift of $\sim1$~Hz/s.

DOI
10.1364/josab.35.000892

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physics.atom-phCross-listedarXiv:2603.22080•Mar 24, 2026
Quantum information processing using atomic qubits requires narrow linewidth lasers with long-term stability for high fidelity coherent manipulation of Rydberg states. In this paper, we report on the construction and characterization of three continuous-wave (CW) narrow linewidth lasers stabilized simultaneously to an ultra-high finesse Fabry-Perot cavity made of ultra-low expansion (ULE) glass, with a tunable offset-lock frequency. One laser operates at 852nm while the two locked lasers at 1018nm are frequency doubled to 509nm for excitation of 133^{133}133Cs atoms to Rydberg states. The optical beatnote at 509nm is measured to be 260(5)~Hz. We present measurements of the offset between the atomic and cavity resonant frequencies using electromagnetically induced transparency (EIT) for high-resolution spectroscopy on a cold atom cloud. The long-term stability is determined from repeated spectra over a period of 20 days yielding a linear frequency drift of ∼1\sim1∼1~Hz/s.
We describe the design, construction, and characterization of a medium-finesse Fabry-Perot cavity for simultaneous frequency stabilization of two lasers operating at 960 and 780 nm wavelengths, respectively. The lasers are applied in experiments with ultracold rubidium Rydberg atoms, for which a combined laser linewidth similar to the natural Rydberg linewidth (≈10 kHz) is desired. The cavity, with a finesse of ≈1500, is used to reduce the linewidth of the lasers to below this level. By using a spacer made of ultra low expansion (ULE) glass with active temperature stabilization, the residual frequency drift is limited to ≲1 MHz/day. The design optimizes for ease of construction, robustness, and affordability.
We demonstrate a method to simultaneously suppress the linewidths and stabilize the long-term frequency drifts of both 780-nm and 960-nm lasers to the 10-kHz level. We first use an iodine frequency stabilization laser as a frequency reference to stabilize the length of a tunable high-finesse transfer cavity (THFTC). Then two slave lasers of 780 nm and 960 nm are locked to this THFTC. In this way, the linewidths of slave lasers are suppressed to the order of 10 kHz, which are measured by delayed self-heterodyne measurements. Meanwhile, the long-term frequency drifts are stabilized to be less than 22 kHz for 10 h. With the locked lasers, we realize the coherent Rydberg excitation of a single Rb87 atom and keep the exciting stable and repeatable for 10 h, which is essential for Rydberg-mediated single-atom quantum information processing. This dual-laser frequency stabilization and transfer method can also be used in other high-resolution experiments in atomic physics, precision metrology, and molecular spectroscopy.
Abstract We present a self-assembled ultra-low expansion (ULE) cavity system designed for high-precision laser frequency stabilization. The cavity mirrors are bonded to the ULE spacer using a low thermal expansion adhesive, and the assembled cavity exhibits a finesse of nearly 3×1043 \times 10^{4}3×104. A custom-designed multilayer aluminum housing was developed to passively isolate the cavity from environmental fluctuations. Long-term performance characterization reveals a frequency drift of approximately 164 kHz per day.After locking a diode laser to the cavity using the Pound-Drever-Hall technique, we achieve a linewidth of approximately 19.4kHz19.4 \text{kHz}19.4kHz and a fractional frequency stability of6.4×10−136.4 \times 10^{-13}6.4×10−13 at 1 s.To validate the reliability of this frequency-stabilized laser system, we applied it to Rydberg excitation spectroscopy via trap-loss measurements of cold 87^{87}87Rb atoms. Compared to conventional wavelength meter locking, the cavity-stabilized system significantly improves spectral resolution, reducing the linewidth of the trap-loss spectrum from 34 MHz to 6 MHz. Our system offers a robust and cost-effective solution for high-resolution spectroscopy, with applications in coherent control of Rydberg atoms.
We propose and demonstrate an alternative method for spectral filtering and frequency stabilization of both 780-nm and 960-nm lasers using a high-finesse length-tunable cavity (HFLTC). Firstly, the length of HFLTC is stabilized to a commercial frequency reference. Then, the two lasers are locked to this HFLTC using the Pound–Drever–Hall (PDH) method which can narrow the linewidths and stabilize the frequencies of both lasers simultaneously. Finally, the transmitted lasers of HFLTC with each power up to about 100 μW, which act as seed lasers, are amplified using the injection locking method for single-atom Rydberg excitation. The linewidths of obtained lasers are narrowed to be less than 1 kHz, meanwhile the obtained lasers’ phase noise around 750 kHz are suppressed about 30 dB. With the spectrally filtered lasers, we demonstrate a Rabi oscillation between the ground state and Rydberg state of single-atoms in an optical trap tweezer with a decay time of (67 ± 37) μs, which is almost not affected by laser phase noise. We found that the maximum short-term laser frequency fluctuation of a single excitation lasers is at ∼3.3 kHz and the maximum long-term laser frequency drift of a single laser is ∼46 kHz during one month. Our work develops a stable and repeatable method to provide multiple laser sources of ultra-low phase noise, narrow linewidth, and excellent frequency stability, which is essential for high precision atomic experiments, such as neutral atom quantum computing, quantum simulation, quantum metrology, and so on.
In this work, the description and implementation of a Pound-Drever-Hall (PDH) laser frequency stabilization system for a three-photon laser excitation scheme used to excite neutral rubidium-87 atoms to Rydberg states is presented. The three lasers (780 nm, 1367 nm, and 743 nm) are simultaneously frequency-locked to a single ultra-low-expansion (ULE) glass cavity. The first and second step lasers are locked to fixed frequencies, while the third step laser is frequency-swept during excitation to fine-tune the resonance. The setup demonstrates stable simultaneous locking of all three lasers and provides a foundation for enhanced stability and reduced linewidth in future implementations.
We present a standalone frequency-offset locking system for controlling narrow-linewidth lasers using off-the-shelf electronic components. We lock two frequency-doubled 1560 nm lasers to a stable primary laser operating at 780 nm via their optical beat note. This radio-frequency beat note is fed through a broadband variable divider, a frequency-to-voltage converter, and a proportional-integrator controller to lock each follower laser to a tunable offset frequency relative to the primary. This architecture provides a large capture range (>1> 1>1 GHz), fast response times (<1< 1<1 ms), and high linearity. We achieve a frequency resolution of 1.9 kHz and a short-term fractional frequency instability 10−11/τ(s)10^{-11}/\sqrt{τ\rm (s)}10−11/τ(s)​ at 780 nm without the need for a dedicated, precise clock reference. We perform high-resolution spectroscopy of cold 87^{87}87Rb atoms to demonstrate the tunability and precision of our locking system. We designed the system to be modular and extensible, making it applicable to a wide variety of atomic physics experiments, including laser cooling, spectroscopy, and quantum sensing with atoms, ions, and molecules.