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Contribuições da coerência para a produção de entropia em processos quânticos

Mariana Afeche Cipolla

Published Sep 21, 2021• 0 citations
OpenAlex

Abstract

The thermodynamics of quantum processes is a recent field of study and it has been growing in recent years. Previously thought of as an emergent phenomenon for macroscopic systems, thermodynamics started being applied to quantum systems considering quantities such as heat and work as stochastics. The peculiarity of these systems is that, in addition to studying energetic resources, we must also take into account quantum informational resources such as entanglement and coherence. In this scenario, entropy becomes an important quantity, because in addition to being related to the irreversibility of a process, it can also be used as a measure of the amount of information in the system to which we have access. Entropy, unlike energy, is not a conserved quantity; that is, in a closed system, there is not only an entropy flow between it\'s parts, but also, in general, entropy production. According to the principle of Landauer [IBM Journal of Research and Development, vol. 5, no. 3, pp. 183191 (1961)], it is the entropy produced that causes the loss of information. Studying, then, the production of entropy becomes important for areas such as quantum computing, where you want to have control over information gains and losses. In quantum processes, entropy is produced due both to changes in the energy of the system and to fluctuations in coherence [Phys. Rev. E 99, 042105 (2019); npj Quantum Information 5, 23 (2019)], a purely quantum resource. In this project, we propose to study the statistics of entropy production due to coherence. For this, we will investigate two different splittings of the entropy production: the one proposed in [Phys. Rev. E, vol. 99, 042105 (2019); npj Quantum Information 5, 23 (2019)] and a most recent one proposed in [Phys. Rev. Research 2, 023377 (2020); New Journal of Physics 23, 063027 (2021)]. For simplicity, we will analyse a unitary quantum process, using the two-point measurement (TPM) scheme [Phys. Rev. E 75, 050102 (2007)]. We will apply both formalisms for two specific quantum systems: a macrospin model and the Lipkin-Meshkov-Glick (LMG) model [Nuclear Physics, vol. 62, no. 2, pp. 188 224 (1965)]. We will analyse, in these cases, how the distribution of coherence depends on parameters such as system dimension, temperature, evolution in time, etc.

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Coherence contributions to the entropy production in quantum processes

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•Sep 21, 2021•0 citations

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Sebastian Deffner

Thermodynamics is a phenomenological theory describing the energy conversion of work and heat. At its origins thermodynamics was developed in order to understand and improve heat engines. In conventional thermodynamics, however, only such processes are completely describable which are slow enough to keep the system of interest in an equilibrium state with its thermal environment at all times. On the contrary, all real physical processes are accompanied by non-equilibrium phenomena. These are mathematically described with the help of the irreversible entropy production, i.e. the dissipated work divided by the temperature of the bath. The second law of thermodynamics merely states that the irreversible entropy production is on average always positive. The modern trend of miniaturization, however, leads to smaller and smaller devices. On short length scales thermal noise as well as quantum fluctuations become important. Thus, usual thermodynamic quantities as work and heat acquire stochastic nature. Moreover, in the quantum regime a completely new theory had to be invented, since classical notions of work and heat are no longer valid. The present dissertation contributes to this prevailing field by the derivation of analytical expressions for the entropy production in open and closed quantum system far from thermal equilibrium. The theoretical treatment is motivated by an experimental point of view. The obtained results were derived from the reduced dynamics of the quantum mechanical system, which may be coupled to a thermal bath. To this end, it was dealt with methods and approaches of statistical physics, conventional thermodynamics, quantum information theory and the theory of open quantum systems. In this dissertation the most important physical systems are treated. First, an isolated system is considered before later on a heat bath is included. The limit of weak as well as of strong coupling are analyzed in detail. For isolated systems it turns out that a geometric approach is able to capture the thermodynamic properties, completely. To this end, the irreversible entropy production is sharply estimated from below by the angle between the real non-equilibrium state and the corresponding equilibrium one. Further, it is shown that the Heisenberg uncertainty relation for energy and time can be formulated more precisely in terms of that angle. As experimental system cold ion traps are introduced, in which the theoretical predictions can be verified. For weakly coupled systems, then, the irreversible entropy production is identified and a fluctuation theorem is derived by merely thermodynamic arguments. As experimental system we, again, propose the cold ion traps, where the heat bath can be simulated with the help of LASER light. In the limit of strong coupling a semiclassical description of the reduced quantum system is discussed. Again, an analytically exact expression for the entropy production and the corresponding fluctuation theorem is derived. A physical system, in which strong coupling to the environment can be analyzed, is given by Josephson junctions. This dissertation discusses the entropy production for isolated, weakly coupled, and overdamped quantum systems. For these physical regimes analytical relation are derived and experimental systems proposed, with which the predictions can be verified.

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The thermodynamics of quantum processes is a recent field of study and it has been growing in recent years. Previously thought of as an emergent phenomenon for macroscopic systems, thermodynamics started being applied to quantum systems considering quantities such as heat and work as stochastics. The peculiarity of these systems is that, in addition to studying energetic resources, we must also take into account quantum informational resources such as entanglement and coherence. In this scenario, entropy becomes an important quantity, because in addition to being related to the irreversibility of a process, it can also be used as a measure of the amount of information in the system to which we have access. Entropy, unlike energy, is not a conserved quantity; that is, in a closed system, there is not only an entropy flow between it's parts, but also, in general, entropy production. According to the principle of Landauer [IBM Journal of Research and Development, vol. 5, no. 3, pp. 183191 (1961)], it is the entropy produced that causes the loss of information. Studying, then, the production of entropy becomes important for areas such as quantum computing, where you want to have control over information gains and losses. In quantum processes, entropy is produced due both to changes in the energy of the system and to fluctuations in coherence [Phys. Rev. E 99, 042105 (2019); npj Quantum Information 5, 23 (2019)], a purely quantum resource. In this project, we propose to study the statistics of entropy production due to coherence. For this, we will investigate two different splittings of the entropy production: the one proposed in [Phys. Rev. E, vol. 99, 042105 (2019); npj Quantum Information 5, 23 (2019)] and a most recent one proposed in [Phys. Rev. Research 2, 023377 (2020); New Journal of Physics 23, 063027 (2021)]. For simplicity, we will analyse a unitary quantum process, using the two-point measurement (TPM) scheme [Phys. Rev. E 75, 050102 (2007)]. We will apply both formalisms for two specific quantum systems: a macrospin model and the Lipkin-Meshkov-Glick (LMG) model [Nuclear Physics, vol. 62, no. 2, pp. 188 224 (1965)]. We will analyse, in these cases, how the distribution of coherence depends on parameters such as system dimension, temperature, evolution in time, etc.
Thermodynamics is a phenomenological theory describing the energy conversion of work and heat. At its origins thermodynamics was developed in order to understand and improve heat engines. In conventional thermodynamics, however, only such processes are completely describable which are slow enough to keep the system of interest in an equilibrium state with its thermal environment at all times. On the contrary, all real physical processes are accompanied by non-equilibrium phenomena. These are mathematically described with the help of the irreversible entropy production, i.e. the dissipated work divided by the temperature of the bath. The second law of thermodynamics merely states that the irreversible entropy production is on average always positive. The modern trend of miniaturization, however, leads to smaller and smaller devices. On short length scales thermal noise as well as quantum fluctuations become important. Thus, usual thermodynamic quantities as work and heat acquire stochastic nature. Moreover, in the quantum regime a completely new theory had to be invented, since classical notions of work and heat are no longer valid. The present dissertation contributes to this prevailing field by the derivation of analytical expressions for the entropy production in open and closed quantum system far from thermal equilibrium. The theoretical treatment is motivated by an experimental point of view. The obtained results were derived from the reduced dynamics of the quantum mechanical system, which may be coupled to a thermal bath. To this end, it was dealt with methods and approaches of statistical physics, conventional thermodynamics, quantum information theory and the theory of open quantum systems. In this dissertation the most important physical systems are treated. First, an isolated system is considered before later on a heat bath is included. The limit of weak as well as of strong coupling are analyzed in detail. For isolated systems it turns out that a geometric approach is able to capture the thermodynamic properties, completely. To this end, the irreversible entropy production is sharply estimated from below by the angle between the real non-equilibrium state and the corresponding equilibrium one. Further, it is shown that the Heisenberg uncertainty relation for energy and time can be formulated more precisely in terms of that angle. As experimental system cold ion traps are introduced, in which the theoretical predictions can be verified. For weakly coupled systems, then, the irreversible entropy production is identified and a fluctuation theorem is derived by merely thermodynamic arguments. As experimental system we, again, propose the cold ion traps, where the heat bath can be simulated with the help of LASER light. In the limit of strong coupling a semiclassical description of the reduced quantum system is discussed. Again, an analytically exact expression for the entropy production and the corresponding fluctuation theorem is derived. A physical system, in which strong coupling to the environment can be analyzed, is given by Josephson junctions. This dissertation discusses the entropy production for isolated, weakly coupled, and overdamped quantum systems. For these physical regimes analytical relation are derived and experimental systems proposed, with which the predictions can be verified.
To understand in detail the relation between unitary quantum theory that describes our world at the microscopic scale and thermodynamics, which was long believed only to apply to macroscopic objects, is one of the most interesting and long-standing problems in physics. Recently, this problem has received renewed attention, in particular from the community of quantum information theory, but also from the field of statistical mechanics, inspired from stochastic thermodynamics. These results suggest that thermodynamics is also relevant for individual quantum systems, provided that they can be brought into contact with thermal baths. In this thesis, I use recently developed tools to provide new results both on fundamental questions, but also on questions which are of practical relevance for potential miniaturized thermal machines. In terms of fundamental questions, the results in this thesis contribute to understanding how the basic laws of thermodynamics and statistical mechanics can be understood directly from unitary quantum mechanics. In particular, I discuss and answer the following questions: i) How can we quantify the third law of thermodynamics using information theoretic methods? ii) How can we quantify the "thermodynamic value" of a state-transition in quantum systems? iii) How can we axiomatically characterize the non-equilibrium free energy and relative entropy? iv) How can we justify statistical ensembles from an operational perspective, without having to introduce either some probability measures or an information theoretic entropy measure? v) How can we understand the equilibration of closed quantum systems, how long does it take and how difficult is it to avoid? In the second part of the thesis I discuss in detail how experimental restrictions, which become important at the quantum scale, influence the ultimate thermodynamic bounds for thermal machines. In particular, the results in this thesis provide thermodynamic bounds on work-extraction and efficiencies of thermal machines in situations where 1.) an experimenter only has limited field strengths available, 2.) an experimenter cannot control the interactions between particles, but external fields arbitrarily well, and 3.) situations in which a small quantum system can only be strongly coupled to heat baths. These bounds are tight and I provide explicit examples illustrating the different behaviours. Finally, I come back to a classic problem in statistical physics: The emergence of spontaneous symmetry breaking. Here, I provide general and rigorous new results that show how symmetry-breaking stationary states emerge from fluctuations in order parameters in dissipative lattice models.
We define and analyse the concept of entanglement production during the evolution of a general quantum mechanical dissipative system. While it is important to minimise entropy production in order to achieve thermodynamical efficiency, maximising the rate of change of entanglement is important in quantum information processing. Quantitative relations are obtained between entropy and entanglement productions, under specific assumptions detailed in the text. We apply these to the processes of dephasing and decay of correlations between two initially entangled qubits. Both the Master equation treatment as well as the higher Hilbert space analysis are presented. Our formalism is very general and contains as special cases many reported individual instance of entanglement dynamics, such as, for example, the recently discovered notion of the sudden death of entanglement.
We formulate a stochastic description of entropy production in scattering theory for coherent transport. We distinguish between the information entropy change due to partial knowledge of the leads' state and the thermodynamic entropy change due to the equilibration of each lead with its bath. By employing a two-point measurement scheme, we access the stochastic entropy production at these different stages of the process, as well as the statistics of generic transport quantities. When restricted to particle or energy transport, our approach reproduces the Landauer-Büttiker formulas. The possibility to consider more general quantities such as the entropy currents and their fluctuations, provides a systematic connection between stochastic thermodynamics and coherent transport.
Landauer's principle sets fundamental thermodynamical constraints for classical and quantum information processing, thus affecting not only various branches of physics, but also of computer science and engineering. Despite its importance, this principle was only recently experimentally considered for classical systems. Here we employ a nuclear magnetic resonance set-up to experimentally address the information to energy conversion in a quantum system. Specifically, we consider a three nuclear spins [Formula: see text] (qubits) molecule-the system, the reservoir and the ancilla-to measure the heat dissipated during the implementation of a global system-reservoir unitary interaction that changes the information content of the system. By employing an interferometric technique, we were able to reconstruct the heat distribution associated with the unitary interaction. Then, through quantum state tomography, we measured the relative change in the entropy of the system. In this way, we were able to verify that an operation that changes the information content of the system must necessarily generate heat in the reservoir, exactly as predicted by Landauer's principle. The scheme presented here allows for the detailed study of irreversible entropy production in quantum information processors.