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Teoria da produção de entropia de Wehrl para sistemas quânticos fora do equilíbrio

Bruno O. Goes

Published Apr 16, 2020• 0 citations
OpenAlex

Abstract

The physics of systems out of equilibrium is a topic of great interest, mainly due to the possibility of exploring phenomena that can not be observed in equilibrium systems. Driven-dissipative phase transitions open the opportunity of studying phases with no classical counterparts, and these can be experimentally realized in quantum optical platforms. Since these transitions occur in systems kept out of equilibrium, they are characterized by a finite entropy production rate. However, due to technical difficulties regarding the zero temperature limit and the non-gaussianity of such models, very little is known about how entropy production behaves around criticality. Using a quantum phase-space method, based on the Husimi Q-function, we put forth a framework that allows for the complete characterization of the entropy production in driven-dissipative transitions. This new theoretical framework is tailored specifically to describe photon loss dissipation, which is effectively a zero temperature process for which the standard theory of entropy production breaks down. It makes no assumptions about Gaussianity about the model or the state. It works for both, steady-states as well as the dynamics and as an application, we study both situations in the paradigmatic driven-dissipative Kerr model, which presents a discontinuous phase transition. For general driven-dissipative critical systems, where one can define a thermodynamic limit, we find that the entropy production rate and flux naturally split into two contributions: an extensive one and a contribution due to quantum fluctuations only. Moreover, we identify a contribution to the entropy production due to unitary dynamics, and we find that the behavior of this contribution at the non-equilibrium steady-state (NESS) matches the behavior of entropy production rate observed in classical systems. The quantum contributions are found to diverge at the critical point.

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The physics of systems out of equilibrium is a topic of great interest, mainly due to the possibility of exploring phenomena that can not be observed in equilibrium systems. Driven-dissipative phase transitions open the opportunity of studying phases with no classical counterparts, and these can be experimentally realized in quantum optical platforms. Since these transitions occur in systems kept out of equilibrium, they are characterized by a finite entropy production rate. However, due to technical difficulties regarding the zero temperature limit and the non-gaussianity of such models, very little is known about how entropy production behaves around criticality. Using a quantum phase-space method, based on the Husimi Q-function, we put forth a framework that allows for the complete characterization of the entropy production in driven-dissipative transitions. This new theoretical framework is tailored specifically to describe photon loss dissipation, which is effectively a zero temperature process for which the standard theory of entropy production breaks down. It makes no assumptions about Gaussianity about the model or the state. It works for both, steady-states as well as the dynamics and as an application, we study both situations in the paradigmatic driven-dissipative Kerr model, which presents a discontinuous phase transition. For general driven-dissipative critical systems, where one can define a thermodynamic limit, we find that the entropy production rate and flux naturally split into two contributions: an extensive one and a contribution due to quantum fluctuations only. Moreover, we identify a contribution to the entropy production due to unitary dynamics, and we find that the behavior of this contribution at the non-equilibrium steady-state (NESS) matches the behavior of entropy production rate observed in classical systems. The quantum contributions are found to diverge at the critical point.
Driven-dissipative phase transitions are currently a topic of intense research due to the prospect of experimental realizations in quantum optical setups. The most paradigmatic model presenting such a transition is the Kerr model, which predicts the phenomenon of optical bistability, where the system may relax to two different steady states for the same driving condition. These states, however, are inherently out-of-equilibrium and are thus characterized by the continuous production of irreversible entropy, a key quantifier in thermodynamics. In this paper, we study the dynamics of the entropy production rate in a quench scenario of the Kerr model, where the external pump is abruptly changed. This is accomplished using a recently developed formalism, based on the Husimi QQQ-function, which is particularly tailored for driven-dissipative and non-Gaussian bosonic systems, Goes et al. [Phys. Rev. Res. 2, 013136 (2020)]. Within this framework, the entropy production can be split into two contributions, one being extensive with the drive and describing classical irreversibility, and the other being intensive and directly related to quantum fluctuations. The latter, in particular, is found to reveal the high degree of nonadiabaticity for quenches between different metastable states.
Phase transitions represent fundamental transformations of matter, characterized by abrupt changes in macroscopic properties and often associated with singular behavior at critical points. While equilibrium aspects of phase transitions, particularly universal critical exponents and scaling laws, are well-understood, the non-equilibrium processes occurring near criticality, especially the production of entropy, remain a rich area of investigation. This paper explores the intricate relationship between critical entropy production and the emergence of scaling laws in systems undergoing phase transitions. We delve into how the rate of entropy production diverges or exhibits anomalous scaling near critical points, reflecting the system's attempts to dissipate energy and respond to external perturbations as it approaches a state of macroscopic change. By integrating concepts from non-equilibrium thermodynamics, statistical mechanics, and renormalization group theory, we aim to elucidate the underlying mechanisms that govern entropy generation in these critical regimes. We discuss theoretical frameworks that predict universal scaling behaviors for entropy production rates, analogous to those observed for equilibrium order parameters and susceptibilities. The implications of these scaling laws extend beyond theoretical physics, offering insights into complex systems, far-from-equilibrium dynamics, and the efficiency of energy conversion processes in critical environments. Our analysis highlights the critical entropy production as a unique signature of non-equilibrium dynamics during phase transitions, providing a deeper understanding of the interplay between fluctuations, dissipation, and universality near points of instability.
We study finite-time driving across second-order dissipative quantum phase transitions described by Lindblad dynamics. We show that the nonadiabatic entropy production, which quantifies deviations from the instantaneous nonequilibrium steady state, exhibits universal power-law scaling with the ramp duration in analogy to the Kibble-Zurek mechanism for closed systems. This establishes the universality of irreversible dissipation induced by driving an open quantum system near criticality. Furthermore, in systems described by bosonic Gaussian states, our scaling laws predict that the nonadiabatic entropy production is independent of driving speed to leading order, revealing a distinctive feature of Gaussian dissipative quantum phase transitions. We validate these analytical predictions in the thermodynamic limit of the driven-dissipative Dicke model and via finite-size scaling in the open Kerr model. Our results establish a general framework for understanding universal nonequilibrium response and thermodynamic irreversibility in critical open quantum systems.
This thesis is about the theory of open quantum many-body physics with a particular focus on driven-dissipative photonic and spin lattices. After a review of the main physical platforms and theoretical concepts, we describe our original results. In Chapter 2, we present a theory of the single-mode Kerr model with a time-dependent pump. This model describes a single-mode optical cavity with a third-order optical nonlinearity. In the regime of parameters where the semiclassical analysis shows bistability, we find that a dynamic hysteresis loop appears in the exact solution. The hysteresis area as a function of the sweep time shows a double power-law decay where the second exponent is independent of the system parameters. We show how these effects are related to the emergence of a dissipative phase transition. We also describe concisely the experimental results which have recently confirmed such theoretical predictions. In Chapter 3, we present the corner-space renormalization method. In order to obtain the steady-state density matrix of the lattice, we solve the Lindblad master equation in a subspace of the Hilbert space (the "corner"). The states spanning the corner space are selected iteratively using eigenvectors of the density matrix of smaller lattice systems, merging in real space two lattices at each iteration and selecting M pairs of states by maximizing their joint probability. The accuracy of the results is then improved by increasing the dimension M of the corner space until convergence is reached. The method has been benchmarked on a two-dimensional Bose-Hubbard model with coherent driving. The strength and limitations of the method are critically discussed.In Chapter 4, we investigate a dissipative phase transition in the two-dimensional anisotropic Heisenberg XYZ model. Using the corner-space renormalization method we present a finite-size analysis of steady-state observables. In particular, we show the critical behaviour of the magnetic susceptibility, the entropy growth and the entanglement witnesses, providing a first evaluation of the critical exponents characterizing the transition. A study of the dynamics of finite-size systems is also consistent with a critical slowing down. For comparison, we present the corresponding analysis for one-dimensional arrays, showing the absence of criticality due to the reduced dimension.In Chapter 5, we explore the non-equilibrium photonic phases of a dissipative Bose-Hubbard model with incoherent pumping of coupled two-level systems. Within a Gutzwiller mean-field approach, we determine the steady-state phase diagram of the system. We predict a second-order phase transition between an incompressible Mott-like phase and a coherent delocalized phase.
By considering a solvable driven-dissipative quantum model, we demonstrate that continuous phase transitions in dissipative systems may occur without an accompanying symmetry breaking. As such, the underlying mechanism for this type of transition is qualitatively different from that of continuous equilibrium phase transitions. In our model, the transition is solely a result of the interplay between Hamiltonian and dissipative dynamics and manifests as a nonanalyticity in the steady state ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\ensuremath{\rho}}}_{\mathrm{ss}}$ in the thermodynamic limit. Based on knowledge from critical classical models we suggest that this behavior derives from a rounding of a first-order phase transition into a continuous one due to large environment-induced fluctuations. Despite being conceptually different from the traditional continuous transitions, we show that expectations of local observables can still be characterized by a set of critical exponents.