Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Four-wave mixing driven by structured light in atomic media : optical mode transfer and spatial correlations

M. R. L. da Motta

Published Feb 5, 2024• 0 citations
OpenAlex

Abstract

In this work we present a series of results on four-wave mixing (FWM) processes induced by structured light in atomic media. We start with a theoretical study focusing on a cascade FWM process in rubidium vapor, generating a blue light field at 420 nm. In this setting, we show that in the extended-medium regime the Hermite-Gaussian basis presents a unique property of optical structure transfer. We then exploit this result to show that, by carefully tailoring the structure of the pump beams, one can obtain desired spatial modes with cylindrical and elliptical symmetries with high fidelity at the blue light output. Following that, we consider an experimental configuration where two degenerate FWM signals are generated in different directions of space by the same pump fields. In this setup, we present results in heated rubidium vapor evidencing the simultaneous conservation of orbital angular momentum (OAM) in the two FWM processes. We show that the two-channel setting allows to encode the OAM content of the input beams onto the OAM carried by the two FWM signals. Next, we explore the transverse mode dynamics in the context of optical modes contained in the so-called orbital angular momentum Poincaré sphere (PS). Defined in analogy with a general polarization state, this family of modes is parametrized in terms of polar and azimuthal angles. We show that the two FWM signals can also be described as belonging to Poincaré spheres, and that the angles on the output PS are related to those on the input PS by well-defined symmetries. The predicted FWM intensity profiles, as well as the consequences of the symmetry properties, are in good agreement with our experimental results. We also explore interesting scenarios, such as combinations of different PS modes and the fulfillment of one of the symmetry relations in each sphere independently, and restrictions that arise in the extended-medium regime. In the last part, we study the correlations between the light fields participating in the two-channel FWM configuration. Following our recent work on cold atoms, we investigate the correlations originating from the conversion of phase-noise to amplitude-noise as a result of the light-atom interaction, and discuss our attempts to discriminate transverse spatial dependencies on these correlations. Finally, we outline the quantum theory of FWM, exploring the multi-spatial-mode nature of the generated light state and the associated spatial correlations.

Related papers

Poincaré-sphere symmetries in four-wave mixing with orbital angular momentum

M. R. L. da Motta, G. B. Alves, Antonio Zelaquett Khoury +1 more

We explore a degenerate four-wave mixing process induced by transversely structured light beams in a rubidium vapor cell. In particular, we consider the nonlinear interaction driven by optical modes contained in the orbital angular momentum Poincar\'e sphere, which can be parametrized in terms of a polar and an azimuthal angle. In this context we investigate the transfer of spatial structure to two distinct four-wave mixing (FWM) signals, possessing different propagation directions in space. We show that under usual assumptions, the output fields can also be described by modes belonging to Poincar\'e spheres, and that the angles describing the input and output modes are related according to well-defined rules. Our experimental results show good agreement with the calculations, which predict intricate field structures and a transition of the FWM transverse profile between the near- and far-field regions.

arXiv:2308.11415•Physical Review A•Jan 11, 2024•3 citations

Four-wave mixing with hermite-gauss modes in rubidium vapor

Pedro Henrique Castro Magalhães [UNESP] Ferreira

In this work, we present an experimental study on the spatial profile of coherent light generated in a forward four-wave mixing (FWM) process. We are interested in investigating how the transverse structure of the incident beams, more specifically of the Hermite-Gauss (HG) modes, is transferred to the generated signal in this nonlinear process. For the experiment, we used a continuous wave diode laser to excite a sample of Rubidium atoms, on the ⁸⁵Rb D2 line, tuned to the frequency of the 5²S_(1/2) ( = 3) → 5²P_(3/2) transition. With a Spatial Light Modulator, we were able to split the laser beam in two and structure them in the desired modes. These two beams, A and B, with wave vectors kA and kB, and linear orthogonal polarizations, with quasi-copropagated configuration, were used to induce two FWM signals in the directions 2kA-kB and 2kB-kA. The spatial profile of incident beams and the two nonlinear signals were captured by a CMOS camera, and the regimes of a thin or extensive medium were investigated. We were able to obtain results for a combination of gaussian-HG beams, as well as HG-HG beams. The profiles obtained by computer simulation were compared with the experimental measurements. Our theoretical model relies on solving the paraxial equation of the generated field. It leads to the overlap integrals of the incident beams, which unfold into some interesting selection rules in the transversal plane, for the thin and extensive medium regimes, and in the longitudinal axis, only for the long medium regime. Although the extensive medium regime presents some additional selection rules, the experimental requirements are difficult to achieve in our system, among them, we highlight the Gouy phase matching. On the other hand, a good agreement between theory and experiment was observed in the thin medium regime.

•Jul 27, 2023•0 citations

Four-Wave Mixing with Orbital Angular Momentum Transfer

Hana Warner

We explore the conservation of orbital angular momentum (OAM) in the four-wave mixing (FWM) process in hot rubidium vapor. Since most modern communication systems send data in pulses corresponding to bits, we can use OAM to encode more information in each pulse by assigning structure to each signal. Furthermore, because FWM can be used to generate entangled photon pairs, we can use this process to bring enhanced signal security. We experimentally studied FWM with a wide range of Laguerre-Gaussian modes and their superpositions and observed OAM transfer from the probe field to a generated Stokes field. By studying the output Stokes intensity and phase distributions, we confirm l mode (OAM) conservation for pure l and p modes, as well as for the superpositions of l and -l for the mode numbers up to l = 4, p = 4. We also found that p index is generally not conserved and its conservation is highly dependent on the relative sizes of the probe and pump beams in the Rb cell. We also identify parameters to improve FWM gain with OAM transfer and propose an analytical method for determining OAM p number.

•Jan 1, 2020•0 citations

Spatial-Multiplexed Four-Channel Optical Amplification via Multiple Four-Wave Mixing in a Double-Λ Atomic System

Xin Li, Dan Song, Yu-xia Fan +5 more

Optical amplification and spatial multiplexing technologies have important applications in quantum communication, quantum networks, and optical information processing. In this paper, based on the non-reciprocal amplification of a pair of co-propagating conjugate four-wave mixing (FWM) signals induced by a one-way pump field in a double-Λ-type hot atomic system, we demonstrate spatially multiplexed multiple FWM processes by introducing a counter-propagating collinear pump field. This configuration enables simultaneous amplification of bidirectional four-channel FWM signals. Furthermore, when the injected signal and pump beams are modulated to Laguerre-Gaussian beams carrying different optical orbital angular momentum (OAM), the OAM of the pump beam is transferred to each amplified field. Through the tilted lens method, we experimentally demonstrate that the OAM of the amplified signal light remains identical to that of the original injected signal light. In contrast, the OAM of the other three newly generated FWM fields is governed by the angular momentum conservation law of their respective FWM processes, which enables the precise manipulation of the OAM for the other generated amplified fields. Theoretical analysis of the dynamical transport equation for the density operator in light-matter interaction processes fully corroborates the experimental results. These findings establish a robust framework for developing OAM-compatible optical non-reciprocal devices based on complex structured light.

Nanomaterials•Jan 29, 2026•1 citation

Manipulation of Coherent Optical Phenomena and the Generation of Orbital Angular Momentum-Based Four-Wave Mixing Signal Using Structured Light

Samim Akhtar, Jayanta K. Saha, Md. Mabud Hossain

Abstract We study various coherent optical properties, e.g., two-photon electromagnetically induced transparency (EIT) and three-photon electromagnetically induced transparency and absorption (TPEIT/TPEIA), in a four-level ladder (Ξ)-type system of 87Rb atoms, where the probe and control fields are Gaussian-shaped laser beams and the pump field is structured laser beam. Additionally, the generated four-wave mixing (FWM) signal has been studied. Interestingly, it is found that the generated FWM signal is spatially structured along with the azimuthal phase, which carries the orbital angular momentum (OAM) of light. It is also observed that the coherent optical responses (EIT, TPEIT/TPEIA, and FWM signals) can be manipulated by utilizing the OAM number of the pump beam as a control knob.

Physics of Wave Phenomena•Aug 1, 2025•0 citations

Spiral Bandwidth of Four-Wave Mixing in Rubidium Vapour

Rachel F. Offer, Dalius Stulga, Erling Riis +2 more

Atomic vapours are an experimentally simple and efficient system in which to study nonlinear wave mixing. We study a four-wave mixing (FWM) process in rubidium vapour which efficiently converts 780 and 776 nm light to 420 nm and 5.2 μm fields. In particular, we quantitatively investigate the transfer of orbital angular momentum (OAM) between the FWM fields. OAM, and structured light more generally, is an important research tool for optical manipulation, imaging and communication. Phase-matched nonlinear processes are both longitudinally and transversely phase coherent, and therefore OAM, which is associated with spiral phase fronts, must be conserved between the pump and generated fields. This makes wave mixing an ideal tool for frequency conversion and generation of a variety of OAM states for use in both classical and quantum communication.

Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)•Jun 1, 2019•0 citations
In this work we present a series of results on four-wave mixing (FWM) processes induced by structured light in atomic media. We start with a theoretical study focusing on a cascade FWM process in rubidium vapor, generating a blue light field at 420 nm. In this setting, we show that in the extended-medium regime the Hermite-Gaussian basis presents a unique property of optical structure transfer. We then exploit this result to show that, by carefully tailoring the structure of the pump beams, one can obtain desired spatial modes with cylindrical and elliptical symmetries with high fidelity at the blue light output. Following that, we consider an experimental configuration where two degenerate FWM signals are generated in different directions of space by the same pump fields. In this setup, we present results in heated rubidium vapor evidencing the simultaneous conservation of orbital angular momentum (OAM) in the two FWM processes. We show that the two-channel setting allows to encode the OAM content of the input beams onto the OAM carried by the two FWM signals. Next, we explore the transverse mode dynamics in the context of optical modes contained in the so-called orbital angular momentum Poincaré sphere (PS). Defined in analogy with a general polarization state, this family of modes is parametrized in terms of polar and azimuthal angles. We show that the two FWM signals can also be described as belonging to Poincaré spheres, and that the angles on the output PS are related to those on the input PS by well-defined symmetries. The predicted FWM intensity profiles, as well as the consequences of the symmetry properties, are in good agreement with our experimental results. We also explore interesting scenarios, such as combinations of different PS modes and the fulfillment of one of the symmetry relations in each sphere independently, and restrictions that arise in the extended-medium regime. In the last part, we study the correlations between the light fields participating in the two-channel FWM configuration. Following our recent work on cold atoms, we investigate the correlations originating from the conversion of phase-noise to amplitude-noise as a result of the light-atom interaction, and discuss our attempts to discriminate transverse spatial dependencies on these correlations. Finally, we outline the quantum theory of FWM, exploring the multi-spatial-mode nature of the generated light state and the associated spatial correlations.
We explore a degenerate four-wave mixing process induced by transversely structured light beams in a rubidium vapor cell. In particular, we consider the nonlinear interaction driven by optical modes contained in the orbital angular momentum Poincar\'e sphere, which can be parametrized in terms of a polar and an azimuthal angle. In this context we investigate the transfer of spatial structure to two distinct four-wave mixing (FWM) signals, possessing different propagation directions in space. We show that under usual assumptions, the output fields can also be described by modes belonging to Poincar\'e spheres, and that the angles describing the input and output modes are related according to well-defined rules. Our experimental results show good agreement with the calculations, which predict intricate field structures and a transition of the FWM transverse profile between the near- and far-field regions.
In this work, we present an experimental study on the spatial profile of coherent light generated in a forward four-wave mixing (FWM) process. We are interested in investigating how the transverse structure of the incident beams, more specifically of the Hermite-Gauss (HG) modes, is transferred to the generated signal in this nonlinear process. For the experiment, we used a continuous wave diode laser to excite a sample of Rubidium atoms, on the ⁸⁵Rb D2 line, tuned to the frequency of the 5²S_(1/2) ( = 3) → 5²P_(3/2) transition. With a Spatial Light Modulator, we were able to split the laser beam in two and structure them in the desired modes. These two beams, A and B, with wave vectors kA and kB, and linear orthogonal polarizations, with quasi-copropagated configuration, were used to induce two FWM signals in the directions 2kA-kB and 2kB-kA. The spatial profile of incident beams and the two nonlinear signals were captured by a CMOS camera, and the regimes of a thin or extensive medium were investigated. We were able to obtain results for a combination of gaussian-HG beams, as well as HG-HG beams. The profiles obtained by computer simulation were compared with the experimental measurements. Our theoretical model relies on solving the paraxial equation of the generated field. It leads to the overlap integrals of the incident beams, which unfold into some interesting selection rules in the transversal plane, for the thin and extensive medium regimes, and in the longitudinal axis, only for the long medium regime. Although the extensive medium regime presents some additional selection rules, the experimental requirements are difficult to achieve in our system, among them, we highlight the Gouy phase matching. On the other hand, a good agreement between theory and experiment was observed in the thin medium regime.
We explore the conservation of orbital angular momentum (OAM) in the four-wave mixing (FWM) process in hot rubidium vapor. Since most modern communication systems send data in pulses corresponding to bits, we can use OAM to encode more information in each pulse by assigning structure to each signal. Furthermore, because FWM can be used to generate entangled photon pairs, we can use this process to bring enhanced signal security. We experimentally studied FWM with a wide range of Laguerre-Gaussian modes and their superpositions and observed OAM transfer from the probe field to a generated Stokes field. By studying the output Stokes intensity and phase distributions, we confirm l mode (OAM) conservation for pure l and p modes, as well as for the superpositions of l and -l for the mode numbers up to l = 4, p = 4. We also found that p index is generally not conserved and its conservation is highly dependent on the relative sizes of the probe and pump beams in the Rb cell. We also identify parameters to improve FWM gain with OAM transfer and propose an analytical method for determining OAM p number.
Optical amplification and spatial multiplexing technologies have important applications in quantum communication, quantum networks, and optical information processing. In this paper, based on the non-reciprocal amplification of a pair of co-propagating conjugate four-wave mixing (FWM) signals induced by a one-way pump field in a double-Λ-type hot atomic system, we demonstrate spatially multiplexed multiple FWM processes by introducing a counter-propagating collinear pump field. This configuration enables simultaneous amplification of bidirectional four-channel FWM signals. Furthermore, when the injected signal and pump beams are modulated to Laguerre-Gaussian beams carrying different optical orbital angular momentum (OAM), the OAM of the pump beam is transferred to each amplified field. Through the tilted lens method, we experimentally demonstrate that the OAM of the amplified signal light remains identical to that of the original injected signal light. In contrast, the OAM of the other three newly generated FWM fields is governed by the angular momentum conservation law of their respective FWM processes, which enables the precise manipulation of the OAM for the other generated amplified fields. Theoretical analysis of the dynamical transport equation for the density operator in light-matter interaction processes fully corroborates the experimental results. These findings establish a robust framework for developing OAM-compatible optical non-reciprocal devices based on complex structured light.
Abstract We study various coherent optical properties, e.g., two-photon electromagnetically induced transparency (EIT) and three-photon electromagnetically induced transparency and absorption (TPEIT/TPEIA), in a four-level ladder (Ξ)-type system of 87Rb atoms, where the probe and control fields are Gaussian-shaped laser beams and the pump field is structured laser beam. Additionally, the generated four-wave mixing (FWM) signal has been studied. Interestingly, it is found that the generated FWM signal is spatially structured along with the azimuthal phase, which carries the orbital angular momentum (OAM) of light. It is also observed that the coherent optical responses (EIT, TPEIT/TPEIA, and FWM signals) can be manipulated by utilizing the OAM number of the pump beam as a control knob.
Atomic vapours are an experimentally simple and efficient system in which to study nonlinear wave mixing. We study a four-wave mixing (FWM) process in rubidium vapour which efficiently converts 780 and 776 nm light to 420 nm and 5.2 μm fields. In particular, we quantitatively investigate the transfer of orbital angular momentum (OAM) between the FWM fields. OAM, and structured light more generally, is an important research tool for optical manipulation, imaging and communication. Phase-matched nonlinear processes are both longitudinally and transversely phase coherent, and therefore OAM, which is associated with spiral phase fronts, must be conserved between the pump and generated fields. This makes wave mixing an ideal tool for frequency conversion and generation of a variety of OAM states for use in both classical and quantum communication.