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Role of disorder and low-density in correlated low-dimensional systems

Morpurgo, Giacomo Arturo Maria

Published Jan 1, 2025• 0 citations
Publisher

Abstract

In this thesis, we study the effects of both disorder and low carrier density in low-dimensional systems, employing a variety of analytical and numerical methods. The work is structured in two main parts, each addressing a distinct research direction. The first part focuses on the impact of disorder in one-dimensional and quasi-one dimensional systems. Using tools such as bosonization, renormalization group techniques, and exact diagonalization, we investigate two key aspects. First, we explore how specific spatial correlations in the disorder affect the properties of the metallic-insulating transition in a one-dimensional system, uncovering significant deviations from the behaviour typically associated with uncorrelated disorder. Second, we examine the effects of different types of disorder on a quasi-one-dimensional singlet superconductor, where we recover Anderson’s theorem under certain conditions and observe a competition between disorder and interactions. The second part of the thesis examines magneto-transport in two-dimensional, locally correlated materials. Using a microscopic quantum theory, we demonstrate pronounced deviations of the Hall constant and the conductivities of the system from their semiclassical predictions, in regimes where the Fermi energy is no longer the dominant energy scale.

DOI
10.13097/archive-ouverte/unige:189073

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In this thesis, we study the effects of both disorder and low carrier density in low-dimensional systems, employing a variety of analytical and numerical methods. The work is structured in two main parts, each addressing a distinct research direction. The first part focuses on the impact of disorder in one-dimensional and quasi-one dimensional systems. Using tools such as bosonization, renormalization group techniques, and exact diagonalization, we investigate two key aspects. First, we explore how specific spatial correlations in the disorder affect the properties of the metallic-insulating transition in a one-dimensional system, uncovering significant deviations from the behaviour typically associated with uncorrelated disorder. Second, we examine the effects of different types of disorder on a quasi-one-dimensional singlet superconductor, where we recover Anderson’s theorem under certain conditions and observe a competition between disorder and interactions. The second part of the thesis examines magneto-transport in two-dimensional, locally correlated materials. Using a microscopic quantum theory, we demonstrate pronounced deviations of the Hall constant and the conductivities of the system from their semiclassical predictions, in regimes where the Fermi energy is no longer the dominant energy scale.
Topic of the thesis is a theoretical description of the ultracold atomic gases in one- and two-dimensional optical lattices in the presence of the disorder leading to the Anderson localization. The disorder is created by interaction of the main fraction of atoms with the second immobilized fraction distributed randomly over the lattice. In low-dimensional systems there is no transition from the Anderson localized to the conducting phase, although in the presence of correlations a discrete set of extended states can exist. The first part of the thesis is devoted to properties of such states. In the finite size lattices, the presence of those states results in the appearance of `windows of transport' -- energy ranges, in which the localization length is longer than the system size.The analytical method of determining the extended states energies for correlations of generalized NNN-mers type is presented, along with a proof that indeed those states are extended in the infinite system. Subsequently, the way of experimental creation of this type of correlations is proposed, as well as the technique of generation of the disorder in the tunneling amplitudes, which significantly enhances tunability of the proposed energy filters. The second part of the thesis describes the method which allows to simulate a specific type of the disorder: random magnetic field. Systems of such a class, created in a two dimensional lattice using simultaneous fast periodic modulation of the lattice height and interactions with immobilized species, may allow in future to investigate the range of topics from the condensed matter physics, for example fractional quantum Hall effect at half-filling. In the thesis, the most interesting features observed upon investigation of such systems are presented. Especially, the anomalously low localization length for correlated disorder is explained.
Understanding the effects of disorder in quantum many-body systems is one of the central challenges of contemporary statistical physics. Its interplay with interactions and quantum fluctuations profoundly modifies the nature of quantum states and their dynamics, giving rise to phenomena such as localization, ergodicity breaking, and the emergence of complex collective behavior. This thesis presents new results on two classes of disordered quantum systems. The first part is devoted to the study of the many-body localization transition, a paradigmatic example of disorder-induced ergodicity breaking. The critical properties of the transition are investigated using a numerical renormalization-group approach, establishing a connection between its scaling behavior and that of the Anderson localization transition on tree-like graphs. The second part focuses on the zero-temperature quantum spin-glass phase of the two-dimensional bond-disordered Heisenberg model. Combining large-scale numerical simulations with a semiclassical expansion, evidence is provided for the existence of the spin-glass phase. The effective model governing the semiclassical fluctuations is further analyzed to characterize the low-energy excitation spectrum and its localization properties. Finally, the weak-disorder regime is investigated and its implications for the ferromagnetic phase are discussed. Overall, the results presented in this thesis contribute to the understanding of the effects of disorder in interacting quantum many-body systems, encompassing both localization phenomena and the collective behavior of disordered quantum magnets.
Disorder and interactions both play crucial roles in quantum transport. Decades ago, Mott showed that electron-electron interactions can lead to insulating behavior in materials that conventional band theory predicts to be conducting. Soon thereafter, Anderson demonstrated that disorder can localize a quantum particle through the wave interference phenomenon of Anderson localization. Although interactions and disorder both separately induce insulating behavior, the interplay of these two ingredients is subtle and often leads to surprising behavior at the periphery of our current understanding. Modern experiments probe these phenomena in a variety of contexts (e.g. disordered superconductors, cold atoms, photonic waveguides, etc.); thus, theoretical and numerical advancements are urgently needed. In this thesis, we report progress on understanding two contexts in which the interplay of disorder and interactions is especially important. The first is the so-called “dirty” or random boson problem. In the past decade, a strong-disorder renormalization group (SDRG) treatment by Altman, Kafri, Polkovnikov, and Refael has raised the possibility of a new unstable fixed point governing the superfluid-insulator transition in the one-dimensional dirty boson problem. This new critical behavior may take over from the weak-disorder criticality of Giamarchi and Schulz when disorder is sufficiently strong. We analytically determine the scaling of the superfluid susceptibility at the strong-disorder fixed point and connect our analysis to recent Monte Carlo simulations by Hrahsheh and Vojta. We then shift our attention to two dimensions and use a numerical implementation of the SDRG to locate the fixed point governing the superfluid-insulator transition there. We identify several universal properties of this transition, which are fully independent of the microscopic features of the disorder. The second focus of this thesis is the interplay of localization and interactions in systems with high energy density (i.e., far from the usual low energy limit of condensed matter physics). Recent theoretical and numerical work indicates that localization can survive in this regime, provided that interactions are sufficiently weak. Stronger interactions can destroy localization, leading to a so-called many-body localization transition. This dynamical phase transition is relevant to questions of thermalization in isolated quantum systems: it separates a many-body localized phase, in which localization prevents transport and thermalization, from a conducting (“ergodic”) phase in which the usual assumptions of quantum statistical mechanics hold. Here, we present evidence that many-body localization also occurs in quasiperiodic systems that lack true disorder.
Since the advent of high-TcT_cTc​ cuprate superconductors in 1986, strongly correlated electron systems have attracted much attention. Since the cuprates are essentially two-dimensional, low-dimensional systems have moved into the focus of condensed-matter theory. From a theoretical point of view, one-dimensional systems are of particular interest because there are exact numerical and analytical methods which permit detailed studies and deep insights into the many-body problem. In the first part of this thesis, using the numerically exact methods Exact Diagonalization and the Density-Matrix Renormalization Group (DMRG), we investigate the properties of the Tomonaga–Luttinger liquid which is the generic metallic state of matter in one dimension. In particular, we concentrate on the investigation of the so-called Tomonaga–Luttinger liquid parameter which determines the critical exponent α\alphaα for the density of states near the Fermi energy. Experimental results for some quasi one-dimensional materials report α≳1\alpha \gtrsim 1α≳1, which would imply Kρ≲0.17K_\rho \lesssim 0.17Kρ​≲0.17, a value which cannot be reconciled with the bare Hubbard model where KρH≥0.5K_\rho^H \geq 0.5KρH​≥0.5, i.e., αH≲1/8\alpha^H \lesssim 1/8αH≲1/8. We develop new accurate numerical methods to obtain KρK_\rhoKρ​ and investigate how to obtain such small values for KρK_\rhoKρ​ for slightly doped charge-density-wave insulators. In the second part of this thesis, using the Thermodynamic Bethe Ansatz (TBA) as exact analytical method, we investigate the one-dimensional Hubbard model in the spindisordered regime, which is characterized by the temperature being much larger than the magnetic energy scale but small compared to the Mott–Hubbard gap. Our study is motivated by the controversy about the Mott–Hubbard insulator in infinite dimensions whose ground state is also spin-disordered. In this system the determination of the precise value of the critical interaction strength Uc where the Mott–Hubbard gap closes is still unsolved. Therefore, we provide an example of a Hubbard-type model with a disordered spin background which can be solved exactly. The thermodynamics of our model can be understood in terms of gapped charged excitations with an effective dispersion which are decoupled form the spin degrees of freedom; the latter contribute only entropically. An interpretation of this regime in terms of a putative interacting-electron system at zero temperature leads to a metal-insulator transition at a finite interaction strength above which the gap opens linearly. Our exact results indicate that the strong-coupling expansion of the ground-state energy cannot be used to locate UcU_cUc​. However, the strong-coupling expansion of the gap permits a reliable extrapolation of the critical interaction strength.
We study the competition between disorder and singlet superconductivity in a quasi-one-dimensional (1D) system. We investigate the applicability of the Anderson theorem, namely that time-reversal conserving (nonmagnetic) disorder does not impact the critical temperature, by opposition to time-reversal breaking disorder (magnetic). To do so, we examine a quasi-1D system of spin 1/2 fermions with attractive interactions and forward scattering disorder using field theory (bosonization). By computing the superconducting critical temperature ( T c ), we find that, for nonmagnetic disorder, the Anderson theorem also holds in the quasi-1D geometry. In contrast, magnetic disorder has an impact on the critical temperature, which we investigate by deriving renormalization group equations describing the competition between disorder and interactions. Computing the critical temperature as a function of disorder strength, we observe different regimes depending on the strength of interactions. We discuss possible platforms where this can be observed in cold atoms and condensed matter. Published by the American Physical Society 2024
This dissertation examines the impact of long-range interactions in lattice models of low-dimensional strongly correlated systems with a focus on their relevance to anomalous electronic transport. Traditionally, the Hubbard model forms the basis of theoretical and numerical investigations of strongly correlated quantum matter. This effective model constitutes the simplest model of electronic correlation and relies on an approximation that truncates electron-electron interactions to a local, on-site potential. While this approximation has proved valid in several instances, certain unexplained phenomena in correlated materials challenge us to develop new perspectives and approaches.In the first part of this thesis, we discuss the historical motivation for our current work from both a theoretical and an experimental viewpoint. In particular, we cover the discovery of bad metallic transport and the associated breakdown of Boltzmann theory of electron transport. We further review examples of strongly correlated systems that exhibit bad metallic transport and other exotic phenomena that suggest the possibility of poorly screened electronic interactions acting as a common microscopic mechanism. This general feature justifies the development of a theoretical framework that is capable of examining long-range interactions in a controlled, systematic manner.Motivated by this, we analyze a long-range interacting lattice model for spinless electrons in two dimensions via exact diagonalization on a finite cluster in real space. As this method is susceptible to finite-size errors, we discuss at length its implementation and technical details designed specifically to reduce these errors, namely the use of twisted boundary conditions and the Ewald summation. We determine the phase diagram at zero temperature and demonstrate that the long-range interactions act as a source of self-generated disorder that drives the development of a strongly correlated pseudogap phase, in a manner reminiscent of the classical Efros-Shklovskii Coulomb gap. Furthermore, we establish that this phenomenon is independent of lattice geometry, a fact that represents the broad potential of long-range interactions in giving rise to a novel form of strongly correlated behavior.Following our zero-temperature study, we address the question of whether this self-generated disorder can survive in the presence of thermal fluctuations and local Coulomb repulsion (Hubbard terms) relevant in Mott systems, a situation closer to those in experimental systems. By means of classical Monte Carlo calculations, we show that not only does the self-generated disorder survive, but that it also acts as a microscopic mechanism that generates bad metallic transport. Upon further investigation, we determine that the long-range interactions, in combination with quantum fluctuations, cause a transient localization of the charge carriers, thereby suppressing the conductivity values below those predicted in conventional Boltzmann theory, as observed experimentally.In conclusion, we have established that long-range interactions in electronic models act as a microscopic mechanism that is capable of causing exotic phenomena in numerous materials. We conclude that a proper treatment of both quantum fluctuations and long-range interactions should next be studied with the finite temperature Lanczos method, which will act as a bridge between our exact diagonalization and Monte Carlo studies. Overall, this dissertation emphasizes the capability of long-range interactions to produce novel phenomena and elicits further thought-provoking questions concerning the interplay with Mott-Hubbard physics and external disorder, crucial in metallic systems.