Metamaterials are artificially designed materials to exhibit properties not available in natural materials by engineering the constituting elements at sub-wavelength scales, enabling unique interactions of matter with electromagnetic waves or coupling modes of electromagnetic waves. Examples of such novel optics phenomenons include negative index of refraction, cloaking, and super-resolution imaging. The study of superconducting metamaterials operating in the microwave frequency domain has recently generated significant interest in the framework of quantum technologies due to a wide range of direct applications, e.g., exploration of novel quantum optics phenomena, non-destructive quantum sensing, quantum-limited amplification, quantum information processing, and quantum illumination. In contrast to their normal metal and semiconducting counterparts, superconducting metamaterials offer some unique advantages. The most relevant of these for Josephson junction based metamaterials are low losses, flux quantization, and Josephson effects. The Josephson effect in a superconducting loop can also be exploited to exact more control over the nonlinearities of the meta-material.In this thesis, we present Josephson junction based metamaterials with in-situ tunability of second and third-order (Kerr) nonlinearities. We optimized the Josephson junction composites SNAILs, well-known in the superconducting circuits community, for the specific use case of building blocks for an impedance-matched nonlinear meta-material. In such devices, the strong third-order (Kerr) nonlinearity can be tuned from positive to negative values. To demonstrate the efficacy of this phenomenon, we have shown a use case of the meta-material as a TWPA with a new phase-matching mechanism: reversed Kerr phase matching, which utilizes the sign reversal of the Kerr nonlinearity to correct for the dispersion curvature of such devices arising due to its finite plasma. The meta-material operated as reversed Kerr TWPA exhibits up to 4 GHz wide combined amplification band with 8 GHz dynamic band tunability, -98 dBm saturation (1 dB compression point) around 20 dB gain, and amplifier added noise close to the standard quantum limit. The absence of any gaps in the transmission can provide a continuous amplification band with significantly lower gain ripples in contrast to the previously demonstrated TWPAs with dispersion engineering.We also present the generation of entanglement utilizing the metamaterials to demonstrate their versatility and further emphasize their potential in the general framework of nonlinear microwave quantum optics. Due to their large bandwidth, these devices have been identified as promising for generating two-mode squeezing and broadband entanglement. With a device optimized for the generation of broadband entanglement, we observed entanglement between two modes separated by up to 400 MHz. We measured logarithmic negativity between 0.27 and 0.51, and the collective quadrature squeezing below the vacuum limit between 1.5 and 2.1 dB. The presented proof-of-principle results can pave the way towards the implementation of Josephson junction based metamaterials in novel applications, including non-destructive single-photon detection, single-photon measurement and control in c-QED, photon-based quantum computing, precision sensing, the detection of dark matter, and quantum illumination.
Metamaterials are artificially designed materials to exhibit properties not available in natural materials by engineering the constituting elements at sub-wavelength scales, enabling unique interactions of matter with electromagnetic waves or coupling modes of electromagnetic waves. Examples of such novel optics phenomenons include negative index of refraction, cloaking, and super-resolution imaging. The study of superconducting metamaterials operating in the microwave frequency domain has recently generated significant interest in the framework of quantum technologies due to a wide range of direct applications, e.g., exploration of novel quantum optics phenomena, non-destructive quantum sensing, quantum-limited amplification, quantum information processing, and quantum illumination. In contrast to their normal metal and semiconducting counterparts, superconducting metamaterials offer some unique advantages. The most relevant of these for Josephson junction based metamaterials are low losses, flux quantization, and Josephson effects. The Josephson effect in a superconducting loop can also be exploited to exact more control over the nonlinearities of the meta-material.In this thesis, we present Josephson junction based metamaterials with in-situ tunability of second and third-order (Kerr) nonlinearities. We optimized the Josephson junction composites SNAILs, well-known in the superconducting circuits community, for the specific use case of building blocks for an impedance-matched nonlinear meta-material. In such devices, the strong third-order (Kerr) nonlinearity can be tuned from positive to negative values. To demonstrate the efficacy of this phenomenon, we have shown a use case of the meta-material as a TWPA with a new phase-matching mechanism: reversed Kerr phase matching, which utilizes the sign reversal of the Kerr nonlinearity to correct for the dispersion curvature of such devices arising due to its finite plasma. The meta-material operated as reversed Kerr TWPA exhibits up to 4 GHz wide combined amplification band with 8 GHz dynamic band tunability, -98 dBm saturation (1 dB compression point) around 20 dB gain, and amplifier added noise close to the standard quantum limit. The absence of any gaps in the transmission can provide a continuous amplification band with significantly lower gain ripples in contrast to the previously demonstrated TWPAs with dispersion engineering.We also present the generation of entanglement utilizing the metamaterials to demonstrate their versatility and further emphasize their potential in the general framework of nonlinear microwave quantum optics. Due to their large bandwidth, these devices have been identified as promising for generating two-mode squeezing and broadband entanglement. With a device optimized for the generation of broadband entanglement, we observed entanglement between two modes separated by up to 400 MHz. We measured logarithmic negativity between 0.27 and 0.51, and the collective quadrature squeezing below the vacuum limit between 1.5 and 2.1 dB. The presented proof-of-principle results can pave the way towards the implementation of Josephson junction based metamaterials in novel applications, including non-destructive single-photon detection, single-photon measurement and control in c-QED, photon-based quantum computing, precision sensing, the detection of dark matter, and quantum illumination.
Josephson meta-materials have recently emerged as very promising platform for superconducting quantum science and technologies. Their distinguishing potential resides in ability to engineer them at sub-wavelength scales, which allows complete control over wave dispersion and nonlinear interaction. In this article we report a versatile Josephson transmission line with strong third order nonlinearity which can be tuned from positive to negative values, and suppressed second order non linearity. As an initial implementation of this multipurpose meta-material, we operate it to demonstrate reversed Kerr phase-matching mechanism in traveling wave parametric amplification. Compared to previous state of the art phase matching approaches, this reversed Kerr phase matching avoids the presence of gaps in transmission, can reduce gain ripples, and allows in situ tunability of the amplification band over an unprecedented wide range. Besides such notable advancements in the amplification performance with direct applications to superconducting quantum computing and generation of broadband squeezing, the in-situ tunability with sign reversal of the nonlinearity in traveling wave structures, with no counterpart in optics to the best of our knowledge, opens exciting experimental possibilities in the general framework of microwave quantum optics, single-photon detection and quantum limited amplification.
Bringing signals from quantum to classical, from few-photon to many-photon levels for further processing, is a common challenge in rising quantum technologies. These include quantum computing, quantum communication, quantum sensing, radio astronomy, and dark matter searches, typically operating at microwave frequencies and millikelvin temperatures. Superconducting parametric amplifiers, as the first piece in the readout chain, have become a cornerstone of these technologies, since they offer unrivaled noise performance near the quantum-mechanical limit and high gain to surpass the noise of subsequent amplifiers. A notable implementation is the Josephson traveling-wave parametric amplifier (TWPA), which stands out due to its bandwidth of several Gigahertz and high saturation power, often larger than -100 dBm. These key properties come at the cost of complexity in design and fabrication: TWPA metamaterials often contain several thousands of Josephson junctions. Designing high-gain TWPAs involves three major challenges: ensuring impedance-matching, phase-matching of parametric amplification, and suppressing unwanted processes, all achievable through sub-wavelength dispersion engineering. This thesis covers the circuit design and analysis, implementation, and experimental characterization of a dispersion-engineered TWPA based on radio-frequency superconducting interference devices (rf-SQUIDs). It focuses on a detailed investigation of dispersion-engineering techniques and their effects on amplifier performance, particularly through the use of time-domain circuit simulations to analyze the multimode dynamics of the circuit. The experimentally realized device features 18 dB of gain, an instantaneous bandwidth spanning from 2.2 to 6.7 GHz, a system noise of 2.5 quanta, and a saturation power of (−86.5 ± 4.0) dBm. With these characteristics, it is suitable for frequency-multiplexed readout of detector arrays or qubits. Its high saturation power, about 10 dB higher than other reported Josephson-junction-based TWPAs, allows increasing the number of qubits per readout line, or decreasing the intermodulation between frequency-multiplexed qubits, both crucial for scaling up quantum computation.
A requirement for quantum information experiments using superconducting quantum circuits is the readout of extremely weak microwave signals. Quantum limited amplifiers are essential for such task and this is precisely why they occupy an always-growing importance in such experiments, particularly for superconducting quantum bits readout.In this thesis, we present two quantum limited amplifiers architectures: the first one is based on a resonator while the second one leverages a traveling-wave construction. These amplifiers both take advantage of tunable Josephson junctions (squid). It is the ideal component for quantum limited parametric amplification: it is both nonlinear and dissipationless (given its superconducting nature). This thesis demonstrates the operation of these Josephson quantum limited amplifiers and how they go beyond the state-of-the-art thanks to original design choices.An important limitation of resonant Josephson parametric amplifiers is their poor dynamic range. We identified the Kerr nonlinearity as the main cause, and we successfully managed to tailor it using Josephson junction arrays. We also developed a model in good agreement with the experimental data, therefore validating our initial assumption that the Kerr nonlinearity and saturation are linked. However, most of the resonant Josephson parametric amplifiers suffer from a fundamental issue, arising from their architecture. It is the conservation of the gain bandwidth product, therefore limiting their bandwidth. Traveling-wave architectures are well suited to overcome this limitation. However, two new issues must be dealt with: impedance matching and phase matching. To tackle the former, we developed an original and simple fabrication process in order to obtain a 50ohm matched 2000 squid array. As for the phase, we matched it by periodically modulating the impedance of the squid transmission line in order to open a photonic band gap. Therefore, we locally distort the dispersion relation. This step does not add any complexity to the initial fabrication process. Moreover, we developed a model in good agreement with experimental data while considering the nonlinear behavior of the photonic gap in a Josephson metamaterial. In addition to demonstrating high performance amplifiers poised for numerous quantum technological applications, this thesis opens the door to more fundamental quantum optics experiments taking advantage of these highly nonlinear transmission lines.With the resonant amplifiers, we measured a 1dB compression point around -117dBm and 45MHz bandwidth (at 20 db gain). With the traveling-wave amplifiers, we measured 18dB gain on a 2.25GHz bandwidth, a 1dB compression point reaching -103dBm and near quantum-limited noise performances.
Superconducting traveling-wave parametric amplifiers (TWPA) have emerged as highly versatile devices, offering broadband amplification with quantum-limited noise performance. They hold significant potential for addressing the readout bottleneck in prototype quantum computers, enabling scalability. Key challenges with this technology include achieving sufficient gain with minimal gain ripple while maintaining low noise performance. Efficient phase matching between a weak signal and a strong pump over the entire length of the TWPA is critical to overcoming these challenges. We present an experimental demonstration of the inverse Kerr phase matching technique in a TWPA, first proposed in Ref. Phys. Rev. Appl. 4, 024014. This method addresses several limitations of conventional dispersion engineering approaches of phase matching in the four-wave mixing parametric process in TWPAs. Most notably the existence of an unusable region of gain near the pump frequency which typically corresponds to the region of most optimal phase matching and maximum gain. The inverse Kerr phase matching approach, allows for greater frequency separation between the region of optimal gain and pump, \textit{in situ} tunability of the pump, minimal gain ripple, and a compact footprint which reduces losses. A TWPA employing the inverse Kerr phase matching technique experimentally demonstrated 20 dB of gain over a 3 GHz instantaneous bandwidth, with a tunable bandwidth of 8 GHz, minimal gain ripple, and near quantum-limited noise performance, with 1.5 photons of added noise.
The optical Kerr effect, in which a medium's refractive index is affected by the intensity of the transmitted light, is exploited not only in conventional optics, but also in superconducting circuits. This article reports a Josephson-junction-based metamaterial with a widely tunable Kerr constant that can even change sign. Controlled by an external magnetic field, this material can speed up or slow down the phase velocity of light per the intensity of the propagating electromagnetic wave. Such an engineered medium could be used for phase matching in traveling-wave parametric amplifiers, or in superconducting hardware for encoding or reading out quantum information.
Josephson traveling-wave parametric amplifiers (JTWPAs) are promising platforms for realizing broadband quantum-limited amplification of microwave signals. However, substantial gain in such systems is attainable only when strict constraints on phase matching of the signal, idler, and pump waves are satisfied---this is rendered particularly challenging in the presence of nonlinear effects, such as self- and cross-phase modulation, which scale with the intensity of propagating signals. In this work, we present a simple JTWPA based on ``left-handed'' (negative-index) nonlinear Josephson metamaterial, which has phase matching native to its design, precluding the need for any complicated circuit or dispersion engineering. The resultant efficiency of the four-wave-mixing process can implement gains in excess of 20 dB over few-gigahertz bandwidths with much shorter lines than previous implementations. Furthermore, the intrinsic phase matching considerably simplifies the JTWPA design and operation compared to the previous implementations based on ``right-handed'' (positive-index) Josephson metamaterials, making the proposed architecture particularly appealing for integration with large superconducting architectures. The left-handed Josephson transmission line introduced here constitutes an alternative modality in distributed Josephson circuits, and forms a crucial piece of the unified framework that can be used to inform the optimal design and operation of broadband microwave amplifiers.