24pRG-13 Novel Method for Solving the Quantum Nonlinear Dynamics of Photons : Use of a Classical Input

Darrick E. Chang, Vladan Vuletić, Mikhail D. Lukin

Kazuki Koshino

In order to investigate the nonlinear dynamics of photons, one must in principle solve a quantum many-particle problem, which usually requires intensive computation. In this study, we show that the spatial wave function of photons after nonlinear interaction can be obtained with less computation by assuming a classical input pulse and calculating a correlation function in the output field. This method is particularly useful when nonlinear optical media have many mechanical degrees of freedom, where quantum many-particle problems become extremely difficult.

Kazuki Koshino

Optical nonlinear effects between several photons are usually negligibly small. Such nonlinear optical effects have been attracting much attention from the viewpoint of all-optical quantum computation. In order to analyze the nonlinear dynamics of photons quantitatively, it is essential to quantize both the photon field and the material system, and also to take account of the multimode nature of the photon field rigorously.

Vincenzo Macr `i, Anton Frisk Kockum, Roberto Stassi +3 more

I. R. Senitzky

Sofia Arranz Regidor, Matthew Kozma, Stephen Hughes

We present a quantum dynamical study of pulsed few-photon scattering from a single artificial atom, consisting of a two-level system (TLS) or qubit, in a waveguide QED system, directly comparing and contrasting two different quantum theoretical simulation methods: (i) an input-output scattering approach that uses frequency-dependent scattering matrices, and (ii) a matrix product states (MPS) approach, which uses quantum noise operators in time bins and a tensor network technique to solve the time-dependent waveguide function for the entire system. Beginning with pulsed excitation using one-photon and two-photon Fock state pulses, we first show how to compute time-dependent observables with the scattering matrix approach, in terms of frequency integrals that encode the pulse spectrum, including how to extract the population dynamics of the excited quantum emitter, as well as the linear and nonlinear contributions. We present solutions for both symmetric and chiral TLS coupling. We then show how to compute the qubit and field observables in a more direct way using MPS, and obtain the characteristic bird-like shape for the two-photon correlation function at two times, which has been observed in recent experiments. We compare and contrast both of these methods, for one and two-photon excitation pulses, and show excellent agreement. We also present a study of the linear and nonlinear contributions, which can easily be calculated using scattering theory, and show the important role of pulse duration. Finally, we demonstrate the clear advantages of MPS by easily going to higher N-photon excitations, and show selected example population dynamics of up to eight-photon Fock-state pulses, manifesting in clear nonlinear population oscillations during the pulse interaction, similar to classical Rabi oscillations, but with quantum input fields that have a vanishing electric field expectation value.