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Automation System for Single Photon Generation and Detection

Kar Tim Chan

Published Jan 1, 2009• 0 citations
OpenAlex

Abstract

Single photon source can be produced by using spontaneous parametric down conversion or quantum emitter such as ions, molecules, atoms, quantum dots and colour centres. Main objective of current research is to automate single photon generation module and detection module based on nitrogen vacancy colour centre in diamond into one system. In single photon generation, diamond sample is held at a holder mounted on a 3D piezo translation stage. Laser source with wavelength 527nm is focused using a standard microscope objective to a spot size at the nitrogen vacancy centre to produce fluorescence. Since a single photon is generated by exciting an isolated nitrogen vacancy in a diamond crystal, it is critical that position of nitrogen vacancies in the crystal to be known. For this purpose, a scanning system was designed and constructed to determine the 3D position of nitrogen vacancy and identified their coordinates for later use. The system consists of a high precision 3D piezo translation stage and was controlled by a scanning programme built using LabVIEW. This programme will map the location of the vacancies in an intensity graph where axis X and Y show the scanning position while the bright colour spots determine the position of the vacancies. In single photon detection which is based on the Hanbury-Brown-Twiss setup, the fluorescence emitted from the nitrogen vacancy is split by a beamsplitter and directed to single photon detectors. A digital pulse is produced for each photocount detected. At the same time, output from the detectors is fed into a time to amplitude converter/single channel analyzer to produce coincidence counts. In order to read and record the number of photon counts and number of coincidences, a detection system was designed and built. This detection system interfaces a series of high performance single photon detectors to the same computer that controls the scanning system via a detection programme. Besides reading and recording data, the detection programme can also calculate the second order correlation function, g2(τ) from a subVI written in LabVIEW 8.2.

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An experimental study of diamond and the nitrogen vacancy centre as a source of single photons.

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For applications in Quantum Information and Quantum Key Distribution an on-demand source of single photons is desirable because absolute security is of utmost importance. Photons are quantum systems; hence encoding information onto them offers a secure alternative to classical cryptography as a measurement cannot be performed on photons without altering their properties. The Nitrogen Vacancy (NV) centre in diamond is a good source of such photons. It is photo-stable and its location in diamond offers robustness. It has zero phonon line at 637 nm and its relative short luminescence life-time of about 12 ns makes it suitable for generating single photons. This thesis covers two aspects: Firstly the characterization of defects in diamonds and subsequent selection of diamonds suitable for use in the single photon setup and secondly, the development of the experimental setup for single photon generation. This thesis sets out to describe the development of a laboratory based single photon source using the NV centre in diamond. For this purpose a suite of diamond samples were selected and subjected to various spectroscopic tests in order to characterize and classify the samples, especially the presence of the NV centres and their concentrations. The characterization of the defects was done through the use of the following spectroscopic techniques: UltravioletVisible-Near infrared spectroscopy, Infrared spectroscopy, Electron Spin Resonance and Photoluminescence. These techniques enabled us to understand the types and origins of crystal defects that were present in the diamond samples used in this study and to use this to select diamonds that are most suitable for use in generation of single photons. The experimental setup for single photon generation using the NV centre is based on a confocal microscope arrangement. Single NV centres were identified by measuring the second order autocorrelation function of the fluorescence light emitted by the sample when illuminated with a laser. This measurement was done using a Hanbury-Brown Twiss (HBT) interferometer.

•Jan 1, 2009•0 citations

Constructing an Autocorrelation System to Identify Single Nitrogen Vacancy Centers in Diamond

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•Jan 1, 2015•0 citations

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Photodynamics of the nitrogen-vacancy colour centre in diamond

Joanne Harrison

The nitrogen-vacancy (N-V⁻) colour centre in diamond has potential applications in quantum information processing and single photon generation. It is currently the only known defect in a solid detected at a single site level that has a non-zero spin in the electronic ground state. For the proposed applications it is desirable to have a good understanding of the electronic structure and photodynamics of the centre, however this is currently not the case. Various models have been proposed to explain the fluorescence characteristics observed in single site experiments. The challenge has been to also account for the properties of the centre well-known from observations of the fluorescence from large ensembles of N-V⁻ in diamond. Firstly, that a non-Boltzmann population distribution between the. ground state spin levels is induced by optical excitation. Secondly, that the fluorescence intensity exhibits a strong dependence on the spin orientation. The models proposed to date either cannot account for these properties, or do so only by invoking optical processes that are arbitrary or, in some cases, not physical. In this thesis an alternative model is presented. The derivation of the model, from group theoretical considerations, does not form part of this thesis. This thesis is concerned primarily with a series of independent measurements to determine the transition rates which govern the photodynamics of the centre. When these transition rates are known, there will be no free parameters in the model and the N-V⁻ emission can be simulated for an arbitrary optical field by solving the classical rate equations. To conclude the first part of this thesis, a two-pulse optical excitation is considered and the results of experiment are compared to the predictions of the model. The latter part of t his thesis is concerned with optically detecting single N-V⁻ centres. A confocal microscope system, to enable single site detection, was developed as part of this work. The photon statistics from a single N-V⁻ centre is compared to the statistics predicted by the model. The implications for the modelling of individual N-V⁻ photon statistics are discussed.

•Jan 1, 2006•0 citations
Single photon source can be produced by using spontaneous parametric down conversion or quantum emitter such as ions, molecules, atoms, quantum dots and colour centres. Main objective of current research is to automate single photon generation module and detection module based on nitrogen vacancy colour centre in diamond into one system. In single photon generation, diamond sample is held at a holder mounted on a 3D piezo translation stage. Laser source with wavelength 527nm is focused using a standard microscope objective to a spot size at the nitrogen vacancy centre to produce fluorescence. Since a single photon is generated by exciting an isolated nitrogen vacancy in a diamond crystal, it is critical that position of nitrogen vacancies in the crystal to be known. For this purpose, a scanning system was designed and constructed to determine the 3D position of nitrogen vacancy and identified their coordinates for later use. The system consists of a high precision 3D piezo translation stage and was controlled by a scanning programme built using LabVIEW. This programme will map the location of the vacancies in an intensity graph where axis X and Y show the scanning position while the bright colour spots determine the position of the vacancies. In single photon detection which is based on the Hanbury-Brown-Twiss setup, the fluorescence emitted from the nitrogen vacancy is split by a beamsplitter and directed to single photon detectors. A digital pulse is produced for each photocount detected. At the same time, output from the detectors is fed into a time to amplitude converter/single channel analyzer to produce coincidence counts. In order to read and record the number of photon counts and number of coincidences, a detection system was designed and built. This detection system interfaces a series of high performance single photon detectors to the same computer that controls the scanning system via a detection programme. Besides reading and recording data, the detection programme can also calculate the second order correlation function, g2(τ) from a subVI written in LabVIEW 8.2.
For applications in Quantum Information and Quantum Key Distribution an on-demand source of single photons is desirable because absolute security is of utmost importance. Photons are quantum systems; hence encoding information onto them offers a secure alternative to classical cryptography as a measurement cannot be performed on photons without altering their properties. The Nitrogen Vacancy (NV) centre in diamond is a good source of such photons. It is photo-stable and its location in diamond offers robustness. It has zero phonon line at 637 nm and its relative short luminescence life-time of about 12 ns makes it suitable for generating single photons. This thesis covers two aspects: Firstly the characterization of defects in diamonds and subsequent selection of diamonds suitable for use in the single photon setup and secondly, the development of the experimental setup for single photon generation. This thesis sets out to describe the development of a laboratory based single photon source using the NV centre in diamond. For this purpose a suite of diamond samples were selected and subjected to various spectroscopic tests in order to characterize and classify the samples, especially the presence of the NV centres and their concentrations. The characterization of the defects was done through the use of the following spectroscopic techniques: UltravioletVisible-Near infrared spectroscopy, Infrared spectroscopy, Electron Spin Resonance and Photoluminescence. These techniques enabled us to understand the types and origins of crystal defects that were present in the diamond samples used in this study and to use this to select diamonds that are most suitable for use in generation of single photons. The experimental setup for single photon generation using the NV centre is based on a confocal microscope arrangement. Single NV centres were identified by measuring the second order autocorrelation function of the fluorescence light emitted by the sample when illuminated with a laser. This measurement was done using a Hanbury-Brown Twiss (HBT) interferometer.
The nitrogen-vacancy (NV) center is a defect in the structure of diamond, roughly the size of a single atom, that possesses properties that make it applicable to quantum information processing, high-resolution magnetic resonance imaging, and probing biological systems. When an NV center is excited by green light of wavelength 523 nm, it emits red light of in the range from 600-800 nm tens of nanoseconds later. A confocal microscope can be used to excite and collect emitted photons from NV centers. By detecting the intensity of the emitted red photons, we can determine the quantum state of a single NV center, which is needed to build various quantum computing, sensing and imaging devices. The autocorrelation method is used to detect antibunching in the emission of red photons and ascertain that the observed photons are being emitted from a single NV center. We have built an autocorrelation device that measures, with sub-nanosecond accuracy, the statistical distribution of the arrival times of the red photons emitted from a diamond sample at a photon counter. The device can measure fixed time values with a time resolution of 120 ps FWHM. For uncorrelated sources measured for 120 seconds at the TAC full range of 100 ns, the average counts in each histogram bin were about 0.01% of the predicted value. The autocorrelation device that we have built costs about 10 times less than commercial units used by other NV researchers.
Single photons are fundamental elements for quantum information technologies such as quantum cryptography, quantum information storage and optical quantum computing. Colour centres in diamond have proven to be stable single-photon sources and thus essential components for reliable and integrated quantum information technology. A key requirement for such applications is a large photon flux and a high efficiency. Paying tribute to various attempts to maximize the single-photon flux, we show that collection efficiencies of photons from colour centres can be increased with a rather simple experimental setup. To do so, we spin-coated nanodiamonds containing single nitrogen-vacancy (N-V) colour centres on the flat surface of a ZrO 2 solid immersion lens. We found stable single-photon count rates of up to 853 kcts s − 1 at saturation under continuous wave excitation while having access to more than 100 defect centres with count rates from 400 to 500 kcts s − 1 . For a blinking defect centre, we found count rates up to 2.4 Mcts s − 1 for time intervals of several tens of seconds. It seems to be a general feature that very high rates are accompanied by blinking behaviour. The overall collection efficiency of our setup of up to 4.2% is the highest yet reported for N-V defect centres in diamond. Under pulsed excitation of a stable emitter of 10 MHz, 2.2% of all pulses caused a click on the detector adding to 221 kcts s − 1 thus, opening the way towards diamond-based on-demand single-photon sources for quantum applications.
Abstract The work reports the manipulation of nitrogen-vacancy centres in chemical vapor deposition grown single crystal diamonds by incorporation of nitrogen, boron and oxygen during the growth process. Single photon emission measurements were performed on diamond samples by using continuous wave and pulsed laser of wavelength 532 nm. The second order auto-correlation measurement 0.3 < g 2 ( 0 ) < 0.6 on nitrogen incorporated diamond sample shows the anti-bunching behavior of photons emerging from the population of one- and two-color centres. However, the correlation measurement 0.6 < g 2 ( 0 ) < 0.8 on oxygen and boron incorporated diamond samples show the anti-bunching behaviour of photons due to population of two- and three-color centres present in the samples. The result opens the possibilities of in situ development of nitrogen-vacancy centres in diamond during the growth process for next generation quantum computing devices.
A simple and convenient design enables real-time three-dimensional position tracking of nitrogen-vacancy (NV) centers in diamond. The system consists entirely of commercially available components (a single-photon counter, a high-speed digital-to-analog converter, a phase-sensitive detector-based feedback device, and a piezo stage), eliminating the need for custom programming or rigorous optimization processes. With a large input range of counters and trackers combined with high sensitivity of single-photon counting, high-speed position tracking (upper bound recovery time of 0.9 s upon 250 nm of step-like positional shift) not only of bright ensembles, but also of low-photon-collection-efficiency single to few NV centers (down to 103 s−1) is possible. The tracking requires position modulation of only 10 nm, which allows simultaneous position tracking and pulsed measurements in the long term. Therefore, this tracking system enables measuring a single-spin magnetic resonance and Rabi oscillations at a very high resolution even without photon collection optimization. The system is widely applicable to various fields related to NV center quantum manipulation research such as NV optical trapping, NV tracking in fluid dynamics, and biological sensing using NV centers inside a biological cell.
The nitrogen-vacancy (N-V⁻) colour centre in diamond has potential applications in quantum information processing and single photon generation. It is currently the only known defect in a solid detected at a single site level that has a non-zero spin in the electronic ground state. For the proposed applications it is desirable to have a good understanding of the electronic structure and photodynamics of the centre, however this is currently not the case. Various models have been proposed to explain the fluorescence characteristics observed in single site experiments. The challenge has been to also account for the properties of the centre well-known from observations of the fluorescence from large ensembles of N-V⁻ in diamond. Firstly, that a non-Boltzmann population distribution between the. ground state spin levels is induced by optical excitation. Secondly, that the fluorescence intensity exhibits a strong dependence on the spin orientation. The models proposed to date either cannot account for these properties, or do so only by invoking optical processes that are arbitrary or, in some cases, not physical. In this thesis an alternative model is presented. The derivation of the model, from group theoretical considerations, does not form part of this thesis. This thesis is concerned primarily with a series of independent measurements to determine the transition rates which govern the photodynamics of the centre. When these transition rates are known, there will be no free parameters in the model and the N-V⁻ emission can be simulated for an arbitrary optical field by solving the classical rate equations. To conclude the first part of this thesis, a two-pulse optical excitation is considered and the results of experiment are compared to the predictions of the model. The latter part of t his thesis is concerned with optically detecting single N-V⁻ centres. A confocal microscope system, to enable single site detection, was developed as part of this work. The photon statistics from a single N-V⁻ centre is compared to the statistics predicted by the model. The implications for the modelling of individual N-V⁻ photon statistics are discussed.