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Radio Frequency Spectroscopy Of a Quasi-Two-Dimensional Fermi Gas

Yingyi Zhang

Published Jan 1, 2013• 1 citation
OpenAlex

Abstract

This dissertation presents the first experiments on radio frequency (rf) spectroscopy of a quasi-two dimensional strongly interacting ultracold atomic Fermi gas. A 50-50 mixture of spin-up and spin-down atoms is confined in a series of pancake-shaped traps produced using an optical standing-wave. To make the system quasi-two dimensional, I adjust the Fermi energy in the weakly confined direction to be comparable to the harmonic oscillator energy level spacing in the tightly confined direction. For a perfectly two dimensional system, at low enough temperature, spin-up and spin-down atoms should form dimers in the ground state of the tightly confined direction. However, in our quasi-two dimensional system I find that the simple dimer theory does not agree with the measured radio-frequency spectra. Instead, the data can be explained by polaron to polaron transitions, which is a many-body effect. Here, a polaron is a spin-down impurity surrounded by a cloud of particle-hole pairs in a spin-up Fermi sea. With this unique strongly interacting quasi-two dimensional system, I am able to study the interplay between confinement induced two-body pairing and many-body physics in confined mesoscopic systems of several hundred atoms, which has not been previously explored and offers new challenges for predictions.

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This dissertation presents the first experiments on radio frequency (rf) spectroscopy of a quasi-two dimensional strongly interacting ultracold atomic Fermi gas. A 50-50 mixture of spin-up and spin-down atoms is confined in a series of pancake-shaped traps produced using an optical standing-wave. To make the system quasi-two dimensional, I adjust the Fermi energy in the weakly confined direction to be comparable to the harmonic oscillator energy level spacing in the tightly confined direction. For a perfectly two dimensional system, at low enough temperature, spin-up and spin-down atoms should form dimers in the ground state of the tightly confined direction. However, in our quasi-two dimensional system I find that the simple dimer theory does not agree with the measured radio-frequency spectra. Instead, the data can be explained by polaron to polaron transitions, which is a many-body effect. Here, a polaron is a spin-down impurity surrounded by a cloud of particle-hole pairs in a spin-up Fermi sea. With this unique strongly interacting quasi-two dimensional system, I am able to study the interplay between confinement induced two-body pairing and many-body physics in confined mesoscopic systems of several hundred atoms, which has not been previously explored and offers new challenges for predictions.
This thesis studies radio-frequency spectroscopy of superfluid alkali Fermi gases. Radio-frequency and laser fields provide a coherent and well understood tool for manipulating atomic gases. However, new phenomena are expected and have already been seen experimentally when the alkali atoms become strongly interacting. Here we use a simple perturbative treatment of the atom-rf-field coupling for studying the spectroscopy of a strongly interacting gas. At ultracold temperatures fermionic atoms become paired in analogy to electrons in superconductors. The resulting binding energy, or the pairing gap, can be observed as a shift in the radio-frequency spectrum. With strong interactions, the fermions begin pairing already above the critical superfluid transition temperature. The radio-frequency spectroscopy grants a way to study these fluctuation effects quantitatively. The inhomogeneous trapping potential of the atom cloud also adds its own flavour, resulting in distinct mesoscopic effects in the radio-frequency spectra. Our theoretical models are in very good agreement with the experimental results. First order perturbation theory provides qualitatively correct lineshapes, and our generalised perturbative approach gives quantitatively correct magnitudes for the transfer rates. The inhomogeneity plays an important part also in more exotic systems in which the simple BCS-type pairing of atoms is prevented by polarising the gas. Superfluidity and phase separation in such spin-imbalanced gases has been experimentally observed. We have suggested the use of radio-frequency spectroscopy for observing exotic polarised superfluid states, present at the edges of the atom cloud.
Low-dimensional ultracold gases are created in the laboratory by confining three-dimensional (3D) gases inside highly anisotropic trapping potentials. Such trap geometries not only provide access to simulating 1D and 2D physics, but also can be used to study how the character of excitations cross over to three dimensions at higher energy. In this work we study the signature in radio-frequency (rf) spectroscopy for both the 1D-to-3D and the 2D-to-3D crossovers, in spin-polarized Fermi gases. We solve the two-body scattering TTT matrix in the presence of strong harmonic confinement and use it to evaluate both the high-frequency rf transfer rate and the two-body bound-state energies. These general expressions are then compared both to the low-dimensional limit and to the 3D limit. We find that in order to understand the dimensional crossover for spin-polarized Fermi gases with ppp-wave interactions, one needs to take into account an emergent sss-wave interaction.
This thesis reports on experiments conducted in a single layer, quasi two-dimensional, two-component ultracold Fermi gas in the strongly interacting regime. Ultracold gases can be used to simulate key aspects of more complicated systems like for example cuprates which show high-Tc superconductivity. \nThe momentum distribution of a sample of bosonic dimers in a quasi-2D square lattice geometry was measured to obtain the coherence properties. For shallow lattices, sharp peaks in the momentum distribution, indicating coherence, were observed at zero momentum as well as at positive and negative lattice momenta along each axis. For deeper \nlattices, heating impeded the ability to prepare a Mott-insulator. \nA spatially resolved radio-frequency spectroscopy was employed for a quasi-2D Fermi gas in the normal phase throughout the BEC-BCS crossover. The interaction induced \nenergy shifts were measured in the strongly interacting region where they can be on the order of the Fermi energy and thus the local resolution is crucial. Furthermore, the onset of pairing in the strongly interacting region was measured as a function of temperature and it was shown that the fraction of free atoms decreases faster than expected from thermal non-interacting theory. At last, the pairing gap was measured using an imbalanced sample. On the BEC side it was found to be in very good agreement with two-body physics as expected. In the strongly interacting regime, however, a deviation from two-body physics indicates that here many-body effects play a role and thus further studies are required.
This thesis reports on experiments with few-fermion systems in quasi one dimensional confining potentials with tunable interaction. \nUsing ultracold atoms we prepare these systems in a well defined quantum state with fidelities of 90% for up to 8 particles. The interparticle interaction in the 1D environment can be effectively described by a 1D contact interaction where the coupling strength can be tuned with a confinement induced resonance (CIR). \nWe investigate a system of two repulsively interacting distinguishable fermions and compare it to a system of two identical noninteracting fermions. For diverging coupling strength we show the fermionization of two distinguishable fermions, i.e. we observe the energy and the square modulus of the wavefunction of both system to be identical. We also perform radio frequency spectroscopy to measure the energy of a single minority particle interacting repulsively with a defined number of majority particles of different spin. We study the crossover from a few-particle system to a many-particle system by adding majority particles one by one. \nWe observe that already four majority particles are enough to describe the properties of the minority by that of a polaron-like particle, i.e. by a single impurity dressed by a 1D Fermi sea. \nInvestigating attractively interacting systems we observe that for increasing interaction strength the pair correlations in the system increases. This correlation leads to a strong odd-even effect of the single particle dissociation energy similar to the one observed for nuclei.
This thesis presents experiments investigating the phase diagram of ultracold atomic Fermi gases using radio-frequency spectroscopy. The tunability of many experimental parameters including the temperature, the interparticle interaction strength and the relative population of different Fermions allows to access very different physical regimes. Radio-frequency spectroscopy has been developed into an ideal tool to probe correlations between particles in these different phases. In particular, radio-frequency spectroscopy of highly population imbalanced atomic Fermi systems gives access to the impurity problem: A single Fermion, or Boson, immersed in a sea of Fermions constitutes a polaron, which can be described by Landau's Fermi liquid theory. A critical interaction strength can be identified separating the regime of a fermionic polaron and a bosonic polaron. Radio-frequency spectroscopy of the polarized superfluid phase allows an accurate measure of the superfluid gap [Delta] and allows to identify the importance of Hartree Mean-field energies. Furthermore, it is shown how these different physical regimes are connected.