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The Road to the Unitary Bose Gas

Benno S. Rem

Published Jan 1, 2013• 1 citation
OpenAlex

Abstract

Ultracold gases have become versatile systems to study quantum many-body effects. Their high degree of control and the tunability of the atomic interactions led to important advances in the understanding of strongly correlated matter. In the regime of strong interactions, unlike fermions, the study of bosons is hampered by three-particle recombination that leads to atom losses and keeps the system from reaching a real equilibrium state. In this thesis, we have performed the first quantitative comparison between theory and experiment on the three-particle loss coefficient L_3(a,T), for arbitrary scattering length a and temperature T. For unitary two-particle scattering (|a| → ∞), we show that the three-particle loss coefficient follows the law L_3(∞, T ) = λ_3/T^2, that we have tested using a trapped non-degenerate ^{7}Li gas maintained at constant temperature. The measured value of λ_3 = 2.5(3)_{stat}(6)_{cyst} × 10^{−20}(μK)^2cm^6s^{−1} is, within the error bars in good agreement with the theory prediction λ_3^{th} = 1.52 × 10^{−20}(μK)^2cm^6s^{−1}. We have extended our measurements to arbitrary values of the scattering length a. For a < 0, the theory predicts a smooth connection between the previously derived zero-temperature model for L_3(a, 0) and the unitarity limited loss coefficient L_3(∞, T ). We also show that a second Efimov resonance in 7Li should be observable near a = − 500 a0 for a temperature of 1 μK. Finally, we compare our theoretical prediction with measurements performed at Innsbruck with ^{133}Cs and at Cambridge with ^{39}K. The theory also shows remarkable quantitative agreement with these measurements.

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Ultracold gases have become versatile systems to study quantum many-body effects. Their high degree of control and the tunability of the atomic interactions led to important advances in the understanding of strongly correlated matter. In the regime of strong interactions, unlike fermions, the study of bosons is hampered by three-particle recombination that leads to atom losses and keeps the system from reaching a real equilibrium state. In this thesis, we have performed the first quantitative comparison between theory and experiment on the three-particle loss coefficient L_3(a,T), for arbitrary scattering length a and temperature T. For unitary two-particle scattering (|a| → ∞), we show that the three-particle loss coefficient follows the law L_3(∞, T ) = λ_3/T^2, that we have tested using a trapped non-degenerate ^{7}Li gas maintained at constant temperature. The measured value of λ_3 = 2.5(3){stat}(6){cyst} × 10^{−20}(μK)^2cm^6s^{−1} is, within the error bars in good agreement with the theory prediction λ_3^{th} = 1.52 × 10^{−20}(μK)^2cm^6s^{−1}. We have extended our measurements to arbitrary values of the scattering length a. For a < 0, the theory predicts a smooth connection between the previously derived zero-temperature model for L_3(a, 0) and the unitarity limited loss coefficient L_3(∞, T ). We also show that a second Efimov resonance in 7Li should be observable near a = − 500 a0 for a temperature of 1 μK. Finally, we compare our theoretical prediction with measurements performed at Innsbruck with ^{133}Cs and at Cambridge with ^{39}K. The theory also shows remarkable quantitative agreement with these measurements.
We study the lifetime of a Bose gas at and around unitarity using a Feshbach resonance in lithium 7. At unitarity, we measure the temperature dependence of the three-body decay coefficient L3{L}_{3}L3​. Our data follow a ${L}_{3}={\ensuremath{\lambda}}_{3}/{T}^{2}$ law with ${\ensuremath{\lambda}}_{3}=2.5(3{)}_{\mathrm{stat}}(6{)}_{\mathrm{syst}}\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}20}\text{ }\text{ }(\ensuremath{\mu}\mathrm{K}{)}^{2}\text{ }{\mathrm{cm}}^{6}\text{ }{\mathrm{s}}^{\ensuremath{-}1}$ and are in good agreement with our analytical result based on zero-range theory. Varying the scattering length aaa at fixed temperature, we investigate the crossover between the finite-temperature unitary region and the previously studied regime where ∣a∣|a|∣a∣ is smaller than the thermal wavelength. We find that L3{L}_{3}L3​ is continuous across the resonance, and over the whole a<0a<0a<0 range our data quantitatively agree with our calculation.
The low-temperature unitary Bose gas is a fundamental paradigm in few-body and many-body physics, attracting wide theoretical and experimental interest. Here, we present experiments performed with unitary 133Cs and 7Li atoms in two different setups, which enable quantitative comparison of the three-body recombination rate in the low-temperature domain. We develop a theoretical model that describes the dynamic competition between two-body evaporation and three-body recombination in a harmonically trapped unitary atomic gas above the condensation temperature. We identify a universal "magic" trap depth where, within some parameter range, evaporative cooling is balanced by recombination heating and the gas temperature stays constant. Our model is developed for the usual three-dimensional evaporation regime as well as the two-dimensional evaporation case, and it fully supports our experimental findings. Combined 133Cs and 7Li experimental data allow investigations of loss dynamics over 2 orders of magnitude in temperature and 4 orders of magnitude in three-body loss rate. We confirm the 1/T2 temperature universality law. In particular, we measure, for the first time, the Efimov inelasticity parameter η*=0.098(7) for the 47.8-G d-wave Feshbach resonance in 133Cs. Our result supports the universal loss dynamics of trapped unitary Bose gases up to a single parameter η*.
This thesis describes studies of out-of-equilibrium dynamics in an interacting homogeneous Bose gas. We use the versatile platform of an ultracold gas of 39^{39}39K, prepared in an optical box trap. The experiment features both tuneable interaction strengths and a homogeneous atomic density. We examine first a weakly interacting near-equilibrium system, followed by far-from-equilibrium dynamics under moderate interactions, and finally combine strong interactions with highly non-equilibrium dynamics in studies of the unitary Bose gas. We start with a theoretical study of the effects of three-body recombination on the temperature of a weakly interacting, partially condensed gas. Contrary to the expectation of heating, we find that for appropriate values of the condensed fraction and gas parameter, the system temperature is expected to decrease. Not only do we predict lower temperatures, however, but also for the condensate fraction to grow. We then present experiments in which we engineer a far-from-equilibrium momentum distribution, and study the dynamics as the gas relaxes. As the distribution evolves, we observe bidirectional dynamic scaling, with a flow of particles to lower momenta while energy is transported to higher ones. These flows are characterised by spatiotemporal scaling exponents, which we find do not vary appreciably over a range of moderate interaction strengths. Finally, we look to the unitary Bose gas, quenching clouds into the strongly interacting regime. This regime offers insight into universal behaviour that depends only on the interparticle spacing, as well as being an avenue for the study of Efimov physics. However, few things come for free; strongly interacting Bose systems are plagued by high atom-loss and heating rates. We study atom-loss rates and the dynamics of correlations in our gases, isolate the coherent effects from the dissipative ones, and identify a quasi-equilibrium state that features a non-zero condensate fraction.
We study the properties of strongly interacting Bose gases at the density and temperature regime when the three-body recombination rate is substantially reduced. In this regime, one can have a Bose gas with all particles in scattering states (i.e., the "upper branch") with little loss even at unitarity over the duration of the experiment. We show that because of bosonic enhancement, pair formation is shifted to the atomic side of the original resonance (where scattering length a(s)<0), opposite to the fermionic case. In a trap, a repulsive Bose gas remains mechanically stable when brought across resonance to the atomic side until it reaches a critical scattering length a(s)*<0. For a(s)<a(s)*, the density consists of a core of upper branch bosons surrounded by an outer layer of equilibrium branch. The conditions of low three-body recombination require that the particle number N<1.024(T/ω)(5/2) in a harmonic trap with frequency ω.
This thesis deals with the Bose gas at large scattering lengths using quantum path-integral Monte Carlo simulations. In the first chapter, this type of simulation is presented through the example of the free Bose gas. The second chapter describes the Bose gas in the regime where interactions become too strong for mean-field theories to be accurate, using a quantum Monte Carlo simulation that quantitatively reproduces both experimental results and theoretical predictions.The second part of this thesis concerns the situation in which the interactions between bosons are resonant, called the unitary regime. In this situation, although two bosons cannot bind, three bosons may form a trimer state. This counter-intuitive effect, called the Efimov effect, is studied in the third chapter of this thesis, both through theoreticalarguments and a dedicated three-body quantum path-integral Monte Carlo simulation. In the fourth chapter, this simulation serves as the building block of a simulation of the unitary Bose gas, that reproduces high-temperature theoretical results and predicts the existence of a low-temperature quantum liquid phase, of the same physical origin as the Efimov effect.
We study the stability of a thermal (39)K Bose gas across a broad Feshbach resonance, focusing on the unitary regime, where the scattering length a exceeds the thermal wavelength λ. We measure the general scaling laws relating the particle-loss and heating rates to the temperature, scattering length, and atom number. Both at unitarity and for positive a<<λ we find agreement with three-body theory. However, for a<0 and away from unitarity, we observe significant four-body decay. At unitarity, the three-body loss coefficient, L(3) proportional λ(4), is 3 times lower than the universal theoretical upper bound. This reduction is a consequence of species-specific Efimov physics and makes (39)K particularly promising for studies of many-body physics in a unitary Bose gas.