This thesis describes studies of out-of-equilibrium dynamics in an interacting homogeneous Bose gas. We use the versatile platform of an ultracold gas of $^{39}$K, prepared in an optical box trap. The experiment features both tuneable interaction strengths and a homogeneous atomic density. We examine first a weakly interacting near-equilibrium system, followed by far-from-equilibrium dynamics under moderate interactions, and finally combine strong interactions with highly non-equilibrium dynamics in studies of the unitary Bose gas. We start with a theoretical study of the effects of three-body recombination on the temperature of a weakly interacting, partially condensed gas. Contrary to the expectation of heating, we find that for appropriate values of the condensed fraction and gas parameter, the system temperature is expected to decrease. Not only do we predict lower temperatures, however, but also for the condensate fraction to grow. We then present experiments in which we engineer a far-from-equilibrium momentum distribution, and study the dynamics as the gas relaxes. As the distribution evolves, we observe bidirectional dynamic scaling, with a flow of particles to lower momenta while energy is transported to higher ones. These flows are characterised by spatiotemporal scaling exponents, which we find do not vary appreciably over a range of moderate interaction strengths. Finally, we look to the unitary Bose gas, quenching clouds into the strongly interacting regime. This regime offers insight into universal behaviour that depends only on the interparticle spacing, as well as being an avenue for the study of Efimov physics. However, few things come for free; strongly interacting Bose systems are plagued by high atom-loss and heating rates. We study atom-loss rates and the dynamics of correlations in our gases, isolate the coherent effects from the dissipative ones, and identify a quasi-equilibrium state that features a non-zero condensate fraction.
This thesis describes studies of out-of-equilibrium dynamics in an interacting homogeneous Bose gas. We use the versatile platform of an ultracold gas of 39K, prepared in an optical box trap. The experiment features both tuneable interaction strengths and a homogeneous atomic density. We examine first a weakly interacting near-equilibrium system, followed by far-from-equilibrium dynamics under moderate interactions, and finally combine strong interactions with highly non-equilibrium dynamics in studies of the unitary Bose gas. We start with a theoretical study of the effects of three-body recombination on the temperature of a weakly interacting, partially condensed gas. Contrary to the expectation of heating, we find that for appropriate values of the condensed fraction and gas parameter, the system temperature is expected to decrease. Not only do we predict lower temperatures, however, but also for the condensate fraction to grow. We then present experiments in which we engineer a far-from-equilibrium momentum distribution, and study the dynamics as the gas relaxes. As the distribution evolves, we observe bidirectional dynamic scaling, with a flow of particles to lower momenta while energy is transported to higher ones. These flows are characterised by spatiotemporal scaling exponents, which we find do not vary appreciably over a range of moderate interaction strengths. Finally, we look to the unitary Bose gas, quenching clouds into the strongly interacting regime. This regime offers insight into universal behaviour that depends only on the interparticle spacing, as well as being an avenue for the study of Efimov physics. However, few things come for free; strongly interacting Bose systems are plagued by high atom-loss and heating rates. We study atom-loss rates and the dynamics of correlations in our gases, isolate the coherent effects from the dissipative ones, and identify a quasi-equilibrium state that features a non-zero condensate fraction.
This thesis describes a collection of experiments that explore interacting ultracold Bose gases, both in and out of equilibrium. Our experiments are performed using a gas of 39K or 87Rb confined in the uniform potential of an optical box trap, a novel testbed for quantum many-body phenomena. Our work focuses on weakly interacting non-equilibrium systems, moderately interacting systems that are still in equilibrium, and the unitary Bose gas which is both strongly interacting and eludes equilibrium. We begin with studies of weakly-interacting gases far from equilibrium, which feature ties to nonlinear wave phenomena. Highlights of our experiments include the direct measurement of turbulent-cascade fluxes, which (alongside realizing a tuneable dissipation scale) allow us to demonstrate the zeroth law of turbulence, and the first observation of weak collapse, a general type of nonlinear wave collapse predicted over 40 years ago. We then turn to moderately strong interactions, confronting existing theories of interacting quantum fluids. One of our most important results is the first quantitative measurement of the quantum depletion of a Bose–Einstein condensate, confirming a 70-year-old theory first developed to describe liquid helium. The culmination of our work explores the unitary Bose gas, where interparticle interactions are as strong as allowed by the laws of quantum mechanics. This strongly-correlated state promises tantalizing possibilities, including emergent universal behavior set solely by the gas density and novel forms of superfluidity. However, the strong interactions also lead to a complex interplay between coherent and dissipative dynamics. By disentangling these two processes, we have caught a glimpse of the promises that the unitary Bose gas holds. In particular, we observe the emergence of universal behavior, and find that the gas features a well defined quasi-equilibrium state, with a non-zero condensed fraction.
This thesis describes experiments focused on investigating out-of-equilibrium phenomena in the Bose-Hubbard Model and exploring novel cooling techniques for ultracold gases in optical lattices. In the first experiment, we study quenches across the Mott-insulator-to-superfluid quantum phase transition in the 3D Bose-Hubbard Model. The quench is accomplished by continuously tuning the ratio of the Hubbard energies. We observe that the degree of excitation is proportional to the fraction of atoms that cross the phase boundary, and that the amount of excitations and energy produced during the quench have a power-law dependence on the quench rate. These phenomena suggest an excitation process analogous to the mechanism for defect generation in non-equilibrium classical phase transitions. This experiment constitutes the first observation of the Kibble-Zurek mechanism in a quantum quench. We have reported our findings in Ref. [1]. In a second experiment, published in Ref. [2], we investigate dissipation as a method for cooling a strongly interacting gas. We introduce dissipation via a bosonic reservoir to a strongly interacting bosonic gas in the Mott-insulator regime of a 3D spin-dependent optical lattice. The lattice atoms are excited to a higher energy band using laser-induced Bragg transitions. A weakly interacting superfluid comprised of atoms in a state that does not experience the lattice potential acts as a dissipative bath that interacts with the lattice atoms through collisions. We measure the resulting bath-induced decay using the atomic quasimomentum distribution, and we compare the decay rate with predictions from a weakly interacting model with no free parameters. A competing intrinsic decay mechanism arising from collisions between lattice atoms is also investigated. The presence of intrinsic decay can not be accommodated within a non-interacting framework and signals that strong interactions may play a central role in the lattice-atom dynamics. The intrinsic decay process we observe may negatively impact the success of cooling via dissipation because a fraction of intrinsic decay events can deposit a large amount of energy into the lattice gas. In a third experiment, we develop and carry out the first demonstration of cooling an atomic quasimomentum distribution. Our scheme, applied in a proof-of-principle experiment to 3D Bose-Hubbard gas in the superfluid regime, involves quasimomentum-selective Raman transitions. This experiment is motivated by the search of new cooling techniques for lattice-trapped gases. Efficient cooling exceeding heating rates is achieved by iteratively removing high quasimomentum atoms from the lattice. Quasimomentum equilibration, which is necessary for cooling, is investigated by directly measuring rethermalization rates after bringing the quasimomentum distribution of the gas out of equilibrium. The measured relaxation rate is consistent at high lattice depths with a short-range, two-particle scattering model without free parameters, despite an apparent violation of the Mott-Ioffe-Regel bound. Our results may have implications for models of unusual transport phenomena in materials with strong interactions, such as heavy fermion materials and transition metal oxides. The cooling method we have developed is applicable to any species, including fermionic atoms. Our results are available in Ref. [3]
The quenched unitary Bose gas is a paradigmatic example of a strongly interacting out-of-equilibrium quantum system, whose dynamics become difficult to describe theoretically due to the growth of non-Gaussian quantum correlations. We develop a conserving many-body theory capable of capturing these effects, allowing us to model the postquench dynamics in the previously inaccessible time regime where the gas departs from the universal prethermal stage. Our results show that this departure is driven by the growth of strong lossless three-body correlations, rather than atomic losses, thus framing the heating of the gas in this regime as a fully coherent phenomenon. We uncover the specific few-body scattering processes that affect this heating and show that the expected connection between the two-body and three-body contacts and the tail of the momentum distribution is obscured following the prethermal stage, explaining the absence of this connection in experiments. Our general framework, which reframes the dynamics of unitary quantum systems in terms of explicit connections to microscopic physics, can be broadly applied to any quantum system containing strong few-body correlations. Published by the American Physical Society 2024
Ultracold gases have become versatile systems to study quantum many-body effects. Their high degree of control and the tunability of the atomic interactions led to important advances in the understanding of strongly correlated matter. In the regime of strong interactions, unlike fermions, the study of bosons is hampered by three-particle recombination that leads to atom losses and keeps the system from reaching a real equilibrium state. In this thesis, we have performed the first quantitative comparison between theory and experiment on the three-particle loss coefficient L_3(a,T), for arbitrary scattering length a and temperature T. For unitary two-particle scattering (|a| → ∞), we show that the three-particle loss coefficient follows the law L_3(∞, T ) = λ_3/T^2, that we have tested using a trapped non-degenerate ^{7}Li gas maintained at constant temperature. The measured value of λ_3 = 2.5(3)_{stat}(6)_{cyst} × 10^{−20}(μK)^2cm^6s^{−1} is, within the error bars in good agreement with the theory prediction λ_3^{th} = 1.52 × 10^{−20}(μK)^2cm^6s^{−1}. We have extended our measurements to arbitrary values of the scattering length a. For a < 0, the theory predicts a smooth connection between the previously derived zero-temperature model for L_3(a, 0) and the unitarity limited loss coefficient L_3(∞, T ). We also show that a second Efimov resonance in 7Li should be observable near a = − 500 a0 for a temperature of 1 μK. Finally, we compare our theoretical prediction with measurements performed at Innsbruck with ^{133}Cs and at Cambridge with ^{39}K. The theory also shows remarkable quantitative agreement with these measurements.
We study non-equilibrium and strongly-correlated dynamics in two contexts. We begin by analysing quantum many-body systems out of equilibrium through the lens of cold atomic impurities in Bose gases. Such highly-imbalanced mixtures provide a controlled arena for the study of interactions, dissipation, decoherence and transport in a many-body quantum environment. Specifically we investigate the oscillatory dynamics of a trapped and initially highly-localised impurity interacting with a weakly-interacting trapped quasi low-dimensional Bose gas. This relates to and goes beyond a recent experiment by the Inguscio group in Florence. We witness a delicate interplay between the self-trapping of the impurity and the inhomogeneity of the Bose gas, and describe the dissipation of the energy of the impurity through phononic excitations of the Bose gas. We then study the transport of a driven, periodically-trapped impurity through a quasi one-dimensional Bose gas. We show that placing the weakly-interacting Bose gas in a separate periodic potential leads to a phononic excitation spectrum that closely mimics those in solid state systems. As a result we show that the impurity-Bose gas system exhibits phonon-induced resonances in the impurity current that were predicted to occur in solids decades ago but never clearly observed. Following this, allowing the bosons to interact strongly, we predict the effect of different strongly-correlated phases of the Bose gas on the motion of the impurity. We show that, by observing the impurity, properties of the excitation spectrum of the Bose gas, e.g., gap and bandwidth, may be inferred along with the filling of the bosonic lattice. In other words the impurity acts as a probe of its environment. To describe the dynamics of such a strongly-correlated system we use the powerful and near-exact time-evolving block decimation (TEBD) method, which we describe in detail. The second part of this thesis then analyses, for the first time, the performance of this method when applied to simulate non-equilibrium classical stochastic processes. We study its efficacy for a well-understood model of transport, the totally-asymmetric exclusion process, and find it to be accurate. Next, motivated by the inefficiency of sampling-based numerical methods for high variance observables we adapt and apply TEBD to simulate a path-dependent observable whose variance increases exponentially with system size. Specifically we calculate the expected value of the exponential of the work done by a varying magnetic field on a one-dimensional Ising model undergoing Glauber dynamics. We confirm using Jarzynski's equality that the TEBD method remains accurate and efficient. Therefore TEBD and related methods complement and challenge the usual Monte Carlo-based simulators of non-equilibrium stochastic processes.
The study of out-of-equilibrium dynamics in ultra-cold gases is a new and exciting field, driven largely by the recent experimental advances in controlling and imaging cold clouds. The experimental and theoretical work thus far has been somewhat exploratory and largely numerical in nature, as the very paradigms for thinking about these systems are not well established. In this thesis I consider several different scenarios of ultra-cold bosonic and fermionic gases driven out of equilibrium and study their properties. In Chapter 1, I provide an overview of the phenomenology of ultra-cold gases, highlighting the timescales governing these systems and how the experimentalist can tune them. I discuss how cold gases can be cooled and trapped and discuss the basic physics behind optical lattices. I also discuss experimental probes of these gases, in particular the new high resolution imaging techniques developed recently at Chicago, Munich and Harvard. In Chapter 2, I discuss an early experiment (circa. 2008) which observed long lived spin dynamics in a thermal spin-1/2 Fermi gas. This experiment is an nice illustration of interesting physics resulting from the separation of timescales between spin and collisional dynamics. In my opinion, it is an excellent example of why cold gases are naturally suited to studying non-equilibrium dynamics. I simulate the experiment numerically using a collisionless Boltzmann equation and explain the observed spin dynamics both qualitatively and quantitively. In Chapter 3, I continue the discussion of spin waves in thermal gases by extending previous works on spin-1/2 gases to spin-1 Bose gases. In contrast to Chapter 2, the bulk of the work in this Chapter is analytic in nature. In particular, I find a spin wave instability in the thermal spin-1 Bose gas, which is the high temperature analog of the polar to ferromagnetic transition in a spin-1 Bose Einstein condensate. In Chapter 3, I turn my attention to bosonic systems and briefly review the the Bogoliubov mean-field theory. I calculate the momentum distribution and density-density correlation function of an interacting Bose gas within the Bogoliubov framework. Then I consider bosons in an optical lattice, and introduce the Bose Hubbard model. I calculate the mean-field phase diagram of the Bose Hubbard model and then consider fluctuations about the mean field, and derive the excitation spectrum of the lattice gas in the superfluid and insulating regimes. In Chapter 4, I ask what we learn by studying the dynamics of correlation functions following a sudden change in the interactions in a superfluid. Using the Bogoliubov theory developed in Chapter 3, I will show how the underlying excitation spectrum influences the long and short time behavior of the correlation functions. By considering a lattice dispersion, I study the analogous problem in a weak optical lattice and discuss how the lattice dispersion leads to additional features in the correlation functions. I will also discuss the timescale governing the revival of the condensate fraction in a quantum depleted gas. In Chapter 5, I derive equations of motion governing the dynamics of one and two body correlation functions in the single-band Bose Hubbard model, applicable to bosons in deep lattices. I then consider a simple quench from a Mott insulating initial state to a weakly interacting final state and produce analytic expressions describing the dynamics of correlations following such a quench. I discuss the timescale for the development of long range order following such a quench. I study the problem of chapter 4 using an equations of motion approach. This approach complements the Bogoliubov approach of Chapter 4. First, I derive exact expressions for a quench to a non-interacting state. I then consider how interactions redistribute quasi-momentum to first order in perturbation theory in different dimensions. In Chapter 6, I calculate the relevant timescales for local and global dynamics in trapped lattice Bose gases, a work done in collaboration with Dr. Kaden R. A Hazzard. Using a time-dependent Gutzwiller mean-field theory, I show that the timescale for local equilibration in these systems is fast in experimental terms. I then show that due to the spatial inhomogeneities inherent to cold gases, achieving global equilibrium can be quite complicated, sometimes taking longer than the lifetime of the experiment, an issue of practical importance to current day experiments. I continue this discussion in Chapter 7 which is a collaborative work with experimentalists David McKay and Prof. Brian DeMarco from the University of Toronto and the University of Illinois, Urbana Champaign. Using experimental and numerical methods, we show that the rapid timescales for local dynamics in interacting systems invalidates a frequently used cold atom technique for mapping out the momentum distribution of atoms in an optical lattice.