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Laser-cooling of Neutral Mercury and Laser-spectroscopy of the 1S0-3P0 optical clock transition

Michael Petersen

Published Feb 6, 2009• 1 citation
OpenAlex

Abstract

Thesis on the subject of lasercooling and trapping of neutral mercury for the purpose of making a lattice clock.

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Mercury is the heaviest stable atom that could be laser cooled, and have a large nuclear charge number. So it has a distinct advantage in quantum precision measurement such as fine-structure constant α and permanent electric dipole moment. Due to its insensitivity of black body radiation, atomic mercury is a good candidate of optical clock. Here we report our recent development of laser cooling of neutral mercury atom. By cooling the mercury source to about -70°C, an ultra-high vacuum system was realized to produce ultracold mercury atoms. The commercial frequency quadrupled semiconductor laser is locked on the cooling transition (1S0-3P1 transition, wavelength of 253.7 nm) by sub-Doppler frequency modulation spectroscopy. By the modification with feed-forward method, the UV laser becomes faster tunable and more stable. A folded beam configuration was used to realize the magneto-optical trap (MOT) because of the shortage of cooling laser power, and the ultracold mercury atoms were observed by fluorescence detection. All of six rich abundant isotopes have been observed, and the atom number is about 1.5×106 with density of 3.5×109 /cm3 for 202Hg. With optical shutter and the programmable system to control the time sequence, the temperature of ultracold atoms can be measured by time of flight method. To enhance the laser power, a 1014.8 nm fiber laser amplifier was developed, which can work at room temperature. After two stages of frequency doubling, about 75 mW of 253.7 nm UV laser were generated, and the saturated absorption spectroscopy of mercury atom was also observed. More power of UV laser could help to trap more atoms in the future. These works laid a good foundation to realize the mercury lattice clock.

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Observation of the 1S0–3P0 optical clock transition in cold 199Hg atoms

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We report on the observation of the highly forbidden 1S0–3P0 optical clock transition in laser-cooled 199Hg atoms. More than 95% depletion of cold 199Hg atoms is detected in the magneto-optical trap. Using the free-of-field detection method, the AC Stark shift from the cooling laser is removed from the in-field spectroscopy. At low-power clock laser pumping, the linewidth of the clock spectroscopy is approximately 450 kHz (full width at half-maximum), which corresponds to a Doppler broadening at the atom temperature of 60 μK. We determine the 1S0–3P0 transition frequency to be 1,128,575,290.819(14) MHz by referencing with a hydrogen maser and measuring with a fiber optical frequency comb. Moreover, a weak Doppler-free signal is observed.

Chinese Optics Letters•Jan 1, 2018•5 citations
The optical lattice clock develops fast in recent years, and its stability and accuracy has already surpassed the microwave fountain clock and the optical clock based on ion trap. The mercury (Hg) lattice clock has the possibility to make a breakthrough in the limitation of blackbody radiation shift for strontium (Sr) and ytterbium (Yb) lattice clock, and reach the uncertainty in E-18 level at room temperature. For the purposes of laser cooling of mercury atoms and interrogating of the clock transition from1S0state to3P0state, a high-power cooling laser at 253.7 nm and an ultra-stable Hz-level linewidth laser at 265.6 nm are required, respectively. Here, we report our development of these laser sources for a neutral Hg lattice clock.
Mercury is the heaviest stable atom that could be laser cooled, and have a large nuclear charge number. So it has a distinct advantage in quantum precision measurement such as fine-structure constant α and permanent electric dipole moment. Due to its insensitivity of black body radiation, atomic mercury is a good candidate of optical clock. Here we report our recent development of laser cooling of neutral mercury atom. By cooling the mercury source to about -70°C, an ultra-high vacuum system was realized to produce ultracold mercury atoms. The commercial frequency quadrupled semiconductor laser is locked on the cooling transition (1S0-3P1 transition, wavelength of 253.7 nm) by sub-Doppler frequency modulation spectroscopy. By the modification with feed-forward method, the UV laser becomes faster tunable and more stable. A folded beam configuration was used to realize the magneto-optical trap (MOT) because of the shortage of cooling laser power, and the ultracold mercury atoms were observed by fluorescence detection. All of six rich abundant isotopes have been observed, and the atom number is about 1.5×106 with density of 3.5×109 /cm3 for 202Hg. With optical shutter and the programmable system to control the time sequence, the temperature of ultracold atoms can be measured by time of flight method. To enhance the laser power, a 1014.8 nm fiber laser amplifier was developed, which can work at room temperature. After two stages of frequency doubling, about 75 mW of 253.7 nm UV laser were generated, and the saturated absorption spectroscopy of mercury atom was also observed. More power of UV laser could help to trap more atoms in the future. These works laid a good foundation to realize the mercury lattice clock.
We report on the observation of the highly forbidden 1S0–3P0 optical clock transition in laser-cooled 199Hg atoms. More than 95% depletion of cold 199Hg atoms is detected in the magneto-optical trap. Using the free-of-field detection method, the AC Stark shift from the cooling laser is removed from the in-field spectroscopy. At low-power clock laser pumping, the linewidth of the clock spectroscopy is approximately 450 kHz (full width at half-maximum), which corresponds to a Doppler broadening at the atom temperature of 60 μK. We determine the 1S0–3P0 transition frequency to be 1,128,575,290.819(14) MHz by referencing with a hydrogen maser and measuring with a fiber optical frequency comb. Moreover, a weak Doppler-free signal is observed.