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Resonances, dissipation and decoherence in exotic and artificial atoms

Mikhail Genkin

Published Jan 1, 2010• 0 citations
OpenAlex

Abstract

There are several reasons why exotic and artificial atoms attract the interest of different scientific communities.In exotic atoms, matter and antimatter can coexist for surprisingly long times. Thus, they present a unique natural laboratory for high precision antimatter studies. In artificial atoms, electrons can be confined in an externally controlled way. This aspect is crucial, as it opens new possibilities for high precision measurements and also makes artificial atoms promising potential candidates for qubits, i.e. the essential bricks for quantum computation.The first part of the thesis presents theoretical studies of resonant states in antiprotonic atoms and spherical two-electron quantum dots, where well established techniques, frequently used for conventional atomic systems, can be applied after moderate modifications. In the framework of Markovian master equations, it is then demonstrated that systems containing resonant states can be approached as open systems in which the resonance width determines the environmental coupling. The second part of the thesis focuses on possible quantum computational aspects of two kinds of artificial atoms, quantum dots and Penning traps. Environmentally induced decoherence, the main obstacle for a practical realization of a quantum computer based on these devices, is studied within a simple phenomenological model. As a result, the dependence of the decoherence timescales on the temperature of the heat bath and environmental scattering rates is obtained.

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There are several reasons why exotic and artificial atoms attract the interest of different scientific communities.In exotic atoms, matter and antimatter can coexist for surprisingly long times. Thus, they present a unique natural laboratory for high precision antimatter studies. In artificial atoms, electrons can be confined in an externally controlled way. This aspect is crucial, as it opens new possibilities for high precision measurements and also makes artificial atoms promising potential candidates for qubits, i.e. the essential bricks for quantum computation.The first part of the thesis presents theoretical studies of resonant states in antiprotonic atoms and spherical two-electron quantum dots, where well established techniques, frequently used for conventional atomic systems, can be applied after moderate modifications. In the framework of Markovian master equations, it is then demonstrated that systems containing resonant states can be approached as open systems in which the resonance width determines the environmental coupling. The second part of the thesis focuses on possible quantum computational aspects of two kinds of artificial atoms, quantum dots and Penning traps. Environmentally induced decoherence, the main obstacle for a practical realization of a quantum computer based on these devices, is studied within a simple phenomenological model. As a result, the dependence of the decoherence timescales on the temperature of the heat bath and environmental scattering rates is obtained.
The computer industry has seen an immense development in the last decades. \nPersonal computers have become available for everybody living in industrialized \ncountries with rapidly increasing performance in terms of speed and storage capacities. \nHowever, the performance of nowadays' computers is fundamentally limited by the \nlaws of classical physics: a classical bit can only take on either of the two distinct \nvalues `0' or `1'. \nIn contrast, a quantum computer could, in principle, make direct use \nof quantum phenomena, such as state superpositions \n-- a quantum bit can be in both states `0' and `1' simultaneously --, \nto perform complex computational tasks much faster than any classical computer. \n \nThe idea of building computers that work according to the laws of quantum physics \nhas opened various fields of research, one of which is the search for the best \nphysical system to use as a quantum bit (qubit). One important criterion for determining \nthe optimal qubit system is the lifetime of state superpositions. \nTypically, once initialized, such superpositions are destroyed on remarkably short \ntimescales due to interactions with the environment -- a process which is referred to \nas decoherence --, posing the question which physical qubit candidate system might show a high-enough robustness against the \ninfluence of the `outside world' to allow for viable quantum computation. \n \nIn this thesis, we will consider three particular realizations of one specific and \nvery promising type of qubit candidate system: \nan electron (or hole) confined to a quantum dot -- a nanoscale structure \nwithin a (typically semiconducting) material --, where the spin states `down' \nand `up' of our electron (or hole) encode the logical states `0' and `1'. \nOur task will be to study the decay of spin-state superpositions in such quantum-dot \nsystems. The main objective of this thesis is to understand the most important physical \nprocesses that lead to spin decoherence and to show ways to suppress this undesirable effect. \nIt turns out that at low temperatures, the main source of decoherence \nis the coupling of the electron (hole) to the surrounding nuclear spins. \n \nThis thesis is divided into three logical parts, corresponding to the three qubit candidate \nsystems under consideration. First we will study electron-spin qubits in III-V semiconductor \nquantum dots, where the electron spin interacts with the nuclear spins of the semiconducting \nhost material \nvia the isotropic Fermi contact hyperfine interaction. Second we consider quantum-dot-confined \nheavy holes and the decoherence of their (pseudo-)spin states due to anisotropic interactions with the \nnuclear spins. Third and last, we study electron-spin qubits made from carbon-nanotube and \ngraphene quantum dots. Quantum dots made of carbon have the advantage of a low abundance \nof spin-carrying nuclear isotopes, therefore reducing decoherence effects significantly. \n \nFor each of the systems under consideration, we will carry out analytical calculations on \nthe nuclear-spin interactions and the spin dynamics of the qubit. Although one main goal of \nthis thesis is to show ways to extend spin decoherence times, we will also focus on physically more \nfundamental questions. Not only the timescale of the decay is relevant for \nthe system's applicability as a qubit, but also the form of the decay which can vary \nsignificantly from system to system. For example, the decay of spin-state superpositions \ncan follow an exponential, super-exponential or power-law decay, and can even pass through \nvarious stages. This is not only of academic interest, but also important for practical \npurposes, such as the implementation of quantum error-correction schemes in a potential \nquantum computer. \n
This thesis is concerned with studying the fascinating quantum properties of real-world nanostructures embedded in a noisy condensed matter environment. The interaction with light is used for controlling and manipulating the quantum state of the systems considered here. In some instances, laser pulses also provide a way of actively probing and controlling environmental interactions. The first two research chapters assess two different ways of performing all-optical spin qubit gates in self-assembled quantum dots. The principal conclusion is that an `adiabatic' control technique holds the promise of achieving a high fidelity when all primary sources of decoherence are taken into account. In the next chapter, it is shown that an optically driven quantum dot exciton interacting with the phonons of the surrounding lattice acts as a heat pump. Further, a model is developed which predicts the temperature-dependent damping of Rabi oscillations caused by bulk phonons, finding an excellent agreement with experimental data. A different system is studied in the following chapter: two electron spin qubits with no direct interaction, yet both exchange-coupled to an optically active mediator spin. The results of this study show that these general assumptions are sufficient for generating controlled electron spin entanglement over a wide range of parameters, even in the presence of noise. Finally, the Radical Pair model of the avian compass is investigated in the light of recent experimental results, leading to the surprising prediction that the electron spin coherence time in this molecular system seems to approach the millisecond timescale.
This thesis is concerned with studying the fascinating quantum properties of real-world nanostructures embedded in a noisy condensed matter environment. The interaction with light is used for controlling and manipulating the quantum state of the systems considered here. In some instances, laser pulses also provide a way of actively probing and controlling environmental interactions. The first two research chapters assess two different ways of performing all-optical spin qubit gates in self-assembled quantum dots. The principal conclusion is that an `adiabatic' control technique holds the promise of achieving a high fidelity when all primary sources of decoherence are taken into account. In the next chapter, it is shown that an optically driven quantum dot exciton interacting with the phonons of the surrounding lattice acts as a heat pump. Further, a model is developed which predicts the temperature-dependent damping of Rabi oscillations caused by bulk phonons, finding an excellent agreement with experimental data. A different system is studied in the following chapter: two electron spin qubits with no direct interaction, yet both exchange-coupled to an optically active mediator spin. The results of this study show that these general assumptions are sufficient for generating controlled electron spin entanglement over a wide range of parameters, even in the presence of noise. Finally, the Radical Pair model of the avian compass is investigated in the light of recent experimental results, leading to the surprising prediction that the electron spin coherence time in this molecular system seems to approach the millisecond timescale.
The ability to manipulate individual quantum systems in a precise way has led to a new era of quantum technologies, including quantum computation and quantum simulation. In this thesis we present several new implementations of these quantum technologies. We first aim at addressing current experimental challenges for quantum dot based quantum computing. We propose a systematic way to study the dynamics of nuclear spin, which is responsible for the short electron spin coherence time. Our calculation is based on diffusion model and is consistent with experiments. We also invent a novel protocol to realize high-fidelity ultrafast universal quantum gate in recently-developed quantum dot molecule system. Experimental realization of our protocol requires only a simple time engineering of optical pulses. We then propose a new quantum state transfer scheme for Nitrogen-Vacancy center based quantum computer, which is applicable at room temperature. Our method accomplishes high fidelity robust quantum state transfer through uncontrolled thermal nitrogen spin chain between two remote NV registers. Our next study helps building a hybrid quantum computer by entangling disparate systems using photonic links. The photons emitted from two types of system need to be matched in both frequency and pulse shape. We propose a simple method to match the emitted pulse shape from two qubit systems with different transition linewidths. We then focus on quantum simulation with trapped ions. We show the possibility of observing a novel type of temperature driven structural phase transition in trapped ion chain, which originates from anharmonic interaction between different vibrational modes. Afterward, an experimental protocol to simulate a conceptually new state of matter, called time crystal, is proposed based on ions trapped in a ring trap. Finally, we propose two new applications based on the recently developed trapped ion quantum simulator of spin models: (1) simulation of Haldane-Shastry model, which opens the way of experimental study to a remarkable theoretical model involving spin liquid ground state and fractional excitations (2) observation of prethermalization and dynamical phase transition, which are poorly understood non-equilibrium phenomena in closed quantum many-body system.
In this Thesis, we study open quantum spin systems from di↵erent perspectives.The first part is motivated by technological challenges of quantum computation.An important building block for quantum computation and quantum communication networks is an interface between material qubits for storage and data processing and travelling photonic qubits for communication.We propose the realisation of a quantum interface between a travelling-wave light field and the nuclear spins in a quantum dot strongly coupled to a cavity.Our scheme is robust against cavity decay as it uses the decay of the cavity to achieve the coupling between nuclear spins and the travelling-wave light fields.A prerequiste for such a quantum interface is a highly polarized ensemble of nuclear spins.High polarization of the nuclear spin ensemble is moreover highly desirable as it protects the potential electron spin qubit from decoherence.Here we present the theoretical description of an experiment in which highly asymmetric dynamic nuclear spin pumping is observed in a single self-assembled InGaAs quantum dot.The second part of this Thesis is devoted to fundamental studies of dissipative spin systems.We study general one-dimensional spin chains under dissipation and propose a scheme to realize a quantum spin system using ultracold atoms in an optical lattice in which both coherent interaction and dissipation can be engineered and controlled.This system enables the study of non-equilibrium and steady state physics of open and driven spin systems.We find, that the steady state expectation values of di↵erent spin models exhibit discontinuous behaviour at degeneracy points of the Hamiltonian in the limit of weak dissipation.This e↵ect can be used to dissipatively probe the spectrum of the Hamiltonian.We moreover study spin models under the aspect of state preparation and show that dissipation drives certain spin models into highly entangled state.Finally,
This thesis is concerned with various aspects of ion traps and their use as a quantum simulation and computation device. In its first part we investigate various sources of noise and decoherence in ion traps. As quantum information is very fragile, a detailed knowledge of noise and decoherence sources in a quantum computation device is essential. In the special case of an ion trap quantum computer we investigate the effects of intensity and phase noise in the laser, which is used to perform the gate operations. We then look at other sources of noise which are present without a laser being switched on. These are fluctuations in the trapping frequency caused by noise in the electric potentials applied to the trap and fluctuating electrical fields which will cause heating of the centre-of-mass vibrational state of the ions in the trap. For the case of fluctuating electrical fields we estimate the effect on a quantum gate operation. We then propose a scheme for performing quantum gates without having the ions cooled down to their motional ground state. The second part deals with various aspects of the use of ion traps as a device for quantum computation. We start with the use of ionic qubits as a measurement device for the centre-of-mass vibrational mode and investigate in detail the effect these measurements will have on the vibrational mode. If one wants to use quantum computation devices as systems to simulate quantum mechanics, it is of interest to know how to simulate say a k-level system with N qubits. We investigate the easiest case of this wider problem and look at how to simulate a three-level system (a so called trit) with two qubits in an ion trap quantum computer. We show how to get and measure a SU (3) geometric phase with this toy model. Finally we investigate how to simulate collective angular momentum models with a string of qubits in an ion trap. We assume that the ionic qubits are coupled to a thermal reservoir and derive a master equation for this case. We investigate the semiclassical limit of this master equation and, in the case for two qubits in the trap, determine the entanglement of the steady state. We also outline a way to find the steady state for the master equation using coherence vectors.