The computer industry has seen an immense development in the last decades. \nPersonal computers have become available for everybody living in industrialized \ncountries with rapidly increasing performance in terms of speed and storage capacities. \nHowever, the performance of nowadays' computers is fundamentally limited by the \nlaws of classical physics: a classical bit can only take on either of the two distinct \nvalues `0' or `1'. \nIn contrast, a quantum computer could, in principle, make direct use \nof quantum phenomena, such as state superpositions \n-- a quantum bit can be in both states `0' and `1' simultaneously --, \nto perform complex computational tasks much faster than any classical computer. \n \nThe idea of building computers that work according to the laws of quantum physics \nhas opened various fields of research, one of which is the search for the best \nphysical system to use as a quantum bit (qubit). One important criterion for determining \nthe optimal qubit system is the lifetime of state superpositions. \nTypically, once initialized, such superpositions are destroyed on remarkably short \ntimescales due to interactions with the environment -- a process which is referred to \nas decoherence --, posing the question which physical qubit candidate system might show a high-enough robustness against the \ninfluence of the `outside world' to allow for viable quantum computation. \n \nIn this thesis, we will consider three particular realizations of one specific and \nvery promising type of qubit candidate system: \nan electron (or hole) confined to a quantum dot -- a nanoscale structure \nwithin a (typically semiconducting) material --, where the spin states `down' \nand `up' of our electron (or hole) encode the logical states `0' and `1'. \nOur task will be to study the decay of spin-state superpositions in such quantum-dot \nsystems. The main objective of this thesis is to understand the most important physical \nprocesses that lead to spin decoherence and to show ways to suppress this undesirable effect. \nIt turns out that at low temperatures, the main source of decoherence \nis the coupling of the electron (hole) to the surrounding nuclear spins. \n \nThis thesis is divided into three logical parts, corresponding to the three qubit candidate \nsystems under consideration. First we will study electron-spin qubits in III-V semiconductor \nquantum dots, where the electron spin interacts with the nuclear spins of the semiconducting \nhost material \nvia the isotropic Fermi contact hyperfine interaction. Second we consider quantum-dot-confined \nheavy holes and the decoherence of their (pseudo-)spin states due to anisotropic interactions with the \nnuclear spins. Third and last, we study electron-spin qubits made from carbon-nanotube and \ngraphene quantum dots. Quantum dots made of carbon have the advantage of a low abundance \nof spin-carrying nuclear isotopes, therefore reducing decoherence effects significantly. \n \nFor each of the systems under consideration, we will carry out analytical calculations on \nthe nuclear-spin interactions and the spin dynamics of the qubit. Although one main goal of \nthis thesis is to show ways to extend spin decoherence times, we will also focus on physically more \nfundamental questions. Not only the timescale of the decay is relevant for \nthe system's applicability as a qubit, but also the form of the decay which can vary \nsignificantly from system to system. For example, the decay of spin-state superpositions \ncan follow an exponential, super-exponential or power-law decay, and can even pass through \nvarious stages. This is not only of academic interest, but also important for practical \npurposes, such as the implementation of quantum error-correction schemes in a potential \nquantum computer. \n
The computer industry has seen an immense development in the last decades. \nPersonal computers have become available for everybody living in industrialized \ncountries with rapidly increasing performance in terms of speed and storage capacities. \nHowever, the performance of nowadays' computers is fundamentally limited by the \nlaws of classical physics: a classical bit can only take on either of the two distinct \nvalues 0' or 1'. \nIn contrast, a quantum computer could, in principle, make direct use \nof quantum phenomena, such as state superpositions \n-- a quantum bit can be in both states 0' and 1' simultaneously --, \nto perform complex computational tasks much faster than any classical computer. \n \nThe idea of building computers that work according to the laws of quantum physics \nhas opened various fields of research, one of which is the search for the best \nphysical system to use as a quantum bit (qubit). One important criterion for determining \nthe optimal qubit system is the lifetime of state superpositions. \nTypically, once initialized, such superpositions are destroyed on remarkably short \ntimescales due to interactions with the environment -- a process which is referred to \nas decoherence --, posing the question which physical qubit candidate system might show a high-enough robustness against the \ninfluence of the outside world' to allow for viable quantum computation. \n \nIn this thesis, we will consider three particular realizations of one specific and \nvery promising type of qubit candidate system: \nan electron (or hole) confined to a quantum dot -- a nanoscale structure \nwithin a (typically semiconducting) material --, where the spin states down' \nand up' of our electron (or hole) encode the logical states 0' and `1'. \nOur task will be to study the decay of spin-state superpositions in such quantum-dot \nsystems. The main objective of this thesis is to understand the most important physical \nprocesses that lead to spin decoherence and to show ways to suppress this undesirable effect. \nIt turns out that at low temperatures, the main source of decoherence \nis the coupling of the electron (hole) to the surrounding nuclear spins. \n \nThis thesis is divided into three logical parts, corresponding to the three qubit candidate \nsystems under consideration. First we will study electron-spin qubits in III-V semiconductor \nquantum dots, where the electron spin interacts with the nuclear spins of the semiconducting \nhost material \nvia the isotropic Fermi contact hyperfine interaction. Second we consider quantum-dot-confined \nheavy holes and the decoherence of their (pseudo-)spin states due to anisotropic interactions with the \nnuclear spins. Third and last, we study electron-spin qubits made from carbon-nanotube and \ngraphene quantum dots. Quantum dots made of carbon have the advantage of a low abundance \nof spin-carrying nuclear isotopes, therefore reducing decoherence effects significantly. \n \nFor each of the systems under consideration, we will carry out analytical calculations on \nthe nuclear-spin interactions and the spin dynamics of the qubit. Although one main goal of \nthis thesis is to show ways to extend spin decoherence times, we will also focus on physically more \nfundamental questions. Not only the timescale of the decay is relevant for \nthe system's applicability as a qubit, but also the form of the decay which can vary \nsignificantly from system to system. For example, the decay of spin-state superpositions \ncan follow an exponential, super-exponential or power-law decay, and can even pass through \nvarious stages. This is not only of academic interest, but also important for practical \npurposes, such as the implementation of quantum error-correction schemes in a potential \nquantum computer. \n
It was Richard Feynman who first proposed, in 1982, the far-reaching concept of \na ”quantum computer”—a device more powerful than classical computers. The idea \nof a quantum computer is to employ the fascinating and often counterintuitive \nlaws of quantum mechanics to process information. It is far from obvious that \nthe proposed concept of a quantum computer is more powerful than its classical \ncounterpart, it was only in 1994 when Peter Shor theoretically demonstrated the \nexistence of a quantum algorithm for factorizing integers into prime factors \nthat runs in polynomial time unlike its classical counterpart which works in \nsub-exponential time. The factorization of integers into prime factors is the \nbasis of asymmetric cryptography. These early theoretical results lunched an \nimmense interest of the scientific community. Already during ’90s, the first \nproposals for the physical implementation of quantum computation emerged. Ever \nsince, many experimental groups around the world pursued different physical \nimplementations of quantum bits (qubits). The first decade of the new century \nsaw a steady improvement in the control and decoherence time (the time over \nwhich the information carried by the qubit is lost) for various qubits by many \norders of magnitude. The natural next step in this context is to answer the \nquestion of how to scale the system up to include many qubits and thus build a \nquantum computer? One of the main parts of this thesis addresses exactly this \nquestion, namely the question of architecture and scalability of future quantum \ncomputer. \n \nAmong various different physical realizations of qubits, the idea of using \nelectron spins trapped in electrostatic semiconductor quantum dots as the \nbuilding blocks of a quantum computer (the so-called spin qubits), put forward \nby Daniel Loss and David DiVincenzo in 1997, triggered tremendous interest in \nscientific community. Nevertheless, the implementation of the original \nLoss-DiVincenzo proposal posed a considerable technical challenge. It used \nquantum tunneling between qubits to enable their communication with each other, \nand thus required that the qubits to be placed very close to each other. This \nrequirement not only leaves little \nspace for the placement of the vast amount of gates and wirings needed to define \nthe electrostatic quantum dots, but also makes it challenging to control the \nlocal magnetic field needed for single-qubit operations. For these reasons, no \nsystem with more than a couple of spin qubits has been \nsuccessfully implemented thus far. In the first part of this thesis, we leap \nover this long-standing problem with an entirely different strategy of using \nmetallic floating gates or ferromagnets to couple together qubits that are \nseparated over a long distance. Our scheme works for any type of \nspin qubits, including the qubits based on nitrogen-vacancy center (NV-center) \nin diamond and technologically very important silicon qubits. \n \nThe main topic of this thesis is related to quantum computer. Still, quite \nunexpectedly, some of the ideas we employed in order to tackle the problem of \nquantum computer scalability can be utilized in a completely different field of \nresearch, namely, in the field of magnetic field sensing. Qubit are not only a \nnecessary ingredient of quantum computer but they also provide a way to measure \nvery accurately magnetic fields. The magnetometer build upon the qubit based on \nNV-center, so-called NV-magnetometer, emerged in recent years as most sensitive \nmagnetic moment sensor. These magnetometers are able to detect about hundred \nnuclear spins within a minute of acquisition time. In the second part of this \nthesis, we propose an entirely novel experimental realization of \nNV-magnetometers which increases present NV-center sensitivities by four orders \nof magnitude at room temperature. This unprecedented amplification of \nsensitivity will render magnetometers capable of detecting individual nuclear \nspins. This amplification is achieved by introducing a ferromagnetic particle \nbetween the nuclear spin that needs to be detected and the NV-magnetometer. Our \nsetup, in contrast to existing schemes, is particularly advantageous because, \ndue to the large amplification of sensitivity, the nuclear spin need not lie \nwithin a few nanometers of the surface but rather can be detectable at a \ndistance of 30 nm. With these novelties, our scheme provides chemically \nsensitive spin detection under ambient conditions allowing nanoscale resolution \nof nuclear magnetic moments in biological systems—the holy grail of nuclear \nmagneticresonance. \n \nIn the last part of the thesis we focus our attention to a new direction in \nquantum computer implementation that deals with topological quantum computer \nintroduced by Alexei Kitaev in 1997; in this approach the idea is to use \nquasiparticles with ”fractional” statistics and to perform the single- and \ntwo-qubit gates by merely exchanging these quasiparticles. Additionally, \ninformation in this system is stored non-locally thus it mitigates the problem \nof decoherence caused by local noise from the environment. Majorana fermions are \none of the most well known examples of such excitations. We analyze transport \nsignatures of different topological states in one-dimensional systems, like \nMajorana fermions and fractionally charged states. We envision an Aharonov-Bohm \nsetup wherein conductance measurement provides a clear signature of presence of \nfractionally charged fermionic states, since oscillations with double period \nemerge in this case. Additionally, we propose a very simple setup that enables \nexistence of degenerate mid-gap states, so-called Tamm-Shockley states that are \ncharacterized by fractional charge and discuss possible ways of detecting these \nstates experimentally. \n
Since the development of microsized devices is moving forward at enormous speed, there is huge amount of new industrial opportunities. However such devices also require high precision and understanding of the operating of their constituent parts up to the quantum level. The device of the purely quantum nature being developed so far is quantum computer. However the physical realization of it is still not performed, as the requirements for it are very rigorous. \n \nIn the pioneering work by Loss and DiVincenzo it was suggested to use a spin of electron placed in a quantum dot as an information qubit. Following this work the study of electron or hole spin qubits developed. Both experimental and theoretical tools for studying them greatly advanced. \n \nIn the first part of the thesis we study the phonon-induced decoherence and relaxation of singlet-triplet qubits in the double quantum dots. First of all we consider AlGaAs/GaAs double quantum dots. The important result we present here is the strong dephasing that occurs at large detuning. This dephasing is due to two-phonon process that affects mainly singlet state of the qubit and consequently changes the splitting between singlet and triplet leading to dephasing. Remarkably at small detuning this dephasing process is suppressed and the decoherence time is by orders of magnitude longer than in case of large detuning and is mainly defined by one-phonon process. We also present the dependence of relaxation time and decoherence time on the strength of spin-orbit interaction and different directions of the system. Our results provide a deeper insight into the recently obtained experimental data. \n \nWe also studied Si/SiGe quantum dots as a potential candidate for a qubit. Apart from the absence of hyperfine interaction and bulk spin-orbit interaction in the isotopically purified 28Si, its electron-phonon interaction is different from GaAs that also leads to longer qubit lifetimes. We study S-T− qubit near the anticrossing of the basis states. This particular region is interesting due to possibilities in operating the qubit. We show that the type of singlet plays a crucial role, i.e. whether it is a singlet with each dot singly occupied or a singlet with only one dot doubly occupied. Depending on the type of singlet the qubit lifetimes change by several orders of magnitude. We also study the influence of a micromagnet, usually used in experiments to operate the qubit, on the relaxation time and decoherence time and present the regime where its effect is negligible. We suggest how to test experimentally our theory of one-phonon and two-phonon processes separately. We also show how the relaxation and decoherence time depend on different system parameters for S-T0 qubits. \n \nThe second part of the thesis is devoted to the other important constituent part of microsized devices, namely nanowires. We are interested in the dynamic of polarization of localized spins in the nanowires, as it can affect such important device characteristics as e.g. conductance. \n \nWe studied Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction-induced polarization in the nanowire in case when the voltage is applied to it. It was already proposed theoretically that in the ground state the localized spins in 1D systems align in a helix due to RKKY interaction. This polarization is still present until some critical temperature. The presence of such polarization acts as a spin filter for electrons, that most likely affects the conductance of the nanowire. Therefore we studied how this helical polarization changes when the voltage is applied. The key result is the appearance of the uniform polarization perpendicular to the helix plane, that occurs due to backscattering of electrons that is accompanied by flip-flop process with localized spins. When this uniform polarization is formed, the helix starts to rotate as a whole around the direction of the uniform polarization. We present the dependence of polarization of the localized spins on temperature and voltage. Remarkably the uniform polarization grows both with voltage and temperature in the given range of parameters. \n \nWe also considered the electron-induced relaxation of the nuclear spins. As the electron spins and nuclear spins interact via hyperfine interaction, the nuclear relaxation time reflects some properties of electron bath. Namely, we see a strong dependence of nuclear relaxation time on spin-orbit interaction strength. We present here the dependence of the nuclear relaxation time on the external magnetic field and chemical potential of the wire, that can be experimentally varied via gate. The dependences for the strong spin-orbit interaction and for the weak one are substantially different. Moreover, they have distinct peaks, that allow to get the value of spin-orbit interaction amplitude with the high precision.
Quantum information processing in semiconductor quantum dots using single and multi-spin qubitsThe idea of a quantum computer, a device capable of processing information using quantum bits (qubit) instead of classical bits that outperforms classical computer in terms of computation speed, is still science ction. However, recent advances in quantum information processing showed that this ction may come true faster than anticipated. A promising platform for the physical realization of a qubit are spin qubits where the information is encoded in the quantum mechanical spin of an electron con ned in a semiconductor quantum dot. There are a variety of di erent implementations how the logical qubit is physically encoded, the use of a single electron spin or the use of the spins of multi electrons. This thesis focuses on the implementation of the spin- 1/2 qubit using the spin of a single electron in a single quantum dot, the exchangeonly (EO) qubit using three electron spins distributed in three quantum dots, and the novel quadrupolar exchange-only (QUEX) qubit using four electron spins distributed in three quantum dots. In this thesis we investigate several theoretical aspects of the physical implementation of the aforementioned qubit encodings. Since all three qubit encodings are allelectric controlled these implementations su er decoherence, the loss of information, from electric uctuations of the environment commonly called charge noise. Typically, the use of more quantum dots increases the decoherence due to charge noise while it decreases the decoherence due to magnetic noise. The rst main aspect investigated in this thesis is the protection of the quantum information encoded in the di erent qubit implementations against charge noise. Special attention is paid to the multi-electron spin implementations where high-symmetry points of operation are discovered which are less sensitive to the charge noise. Protection against charge noise is even better by increasing the number of electrons while keeping the number of quantum dots making the QUEX qubit superior to the EO qubit. So far the main direction in this thesis is the reduction of the qubit sensitivity to electric uctuations. However, coherent electromagnetic elds in form of microwaves v can be used to interconnect qubits. In this thesis also a high-performance coupling between two spin-1/2 is investigated. The use of a resonator, subsequently, allows for a coupling of qubits over macroscopic distances as well as to extract valuable information about the physical system. Because of the larger susceptibility of multi-spin qubits to the electric eld of the resonator, this thesis focuses on the coupling between an EO or a QUEX qubit and a microwave resonator. Points of operations are discovered for both qubit implementations which o er a strong coupling towards a microwave resonator while maintaining their protection against charge noise. Subsequently, a series of measurements are proposed to extract information about the microscopic structure of the quantum dots. Finally, a promising high-performance protocol for coupling two qubits remotely via the resonator is investigated in detail.
At the dawn of the twentieth century, the underpinnings of centuries-old classical physics were beginning to be unravelled by the advent of quantum mechanics. As well as fundamentally shifting the way we understand the very nature of reality, this quantum revolution has subsequently shaped and created entire fields, paving the way for previously unimaginable technology. The quintessential instance of such technology is the quantum computer, whose building blocks - quantum bits, or qubits - are premised on the uniquely quantum principles of superposition and entanglement. It is predicted that quantum computers will be capable of efficiently solving certain classically intractable problems. To build a quantum computer, it is necessary to find a system which exhibits these uniquely quantum phenomena. The success of silicon-based integrated circuits for classical computing made semiconductors an obvious architecture in which to focus experimental quantum computing efforts. The two-dimensional electron gas which forms at the interface of GaAs/AlGaAs heterostructures constitutes an ideal platform for isolating and controlling single electrons, encoding quantum information in their spin and charge states. This thesis broadly addresses three key challenges to quantum computing with GaAs qubits: scalability, particularly in the context of readout, unwanted interactions between fragile quantum states and their environment, and the facilitation of controllable, strong interactions between separated qubits as a means of generating entanglement. These significant, unavoidable challenges must be addressed in order for a future solid-state quantum computer to be viable.
The goal of this thesis is to investigate theoretically the generation and behaviour of multipartite entanglement for solid-state nanosystems, in particular electron spin quantum bits (so-called 'qubits') in quantum dots. A quantum dot is a tiny potential well where a single electron can be trapped. A quantum bit can be implemented in this system by applying a magnetic field, and thereby lifting the degeneracy of the spin states of the electron. These spins can then be used as single qubits, and engineering many of these quantum dots next to each other gives as a register of qubits. In this scheme, the so-called Loss-DiVincenzo quantum computer, the single spins can be rotated e.g. by applying a time dependent magnetic field, and two spins can interact through controlling the potential barrier between them. A qubit cannot only be in a superposition of the two computational states 0 and 1 at the same time, but an even stranger characteristic arises for multiple qubits: this phenomenon is called entanglement and refers to a strong correlation between two or more qubits, which can not be achieved within the framework of classical physics, and exponentially enlarges the possible states for a N-qubit system as compared to a classical N-bit system. In this thesis we devise algorithms how to generate multipartite entangled states in electron spin qubits in quantum dots. We compare which classes of entangled states can be generated efficiently in this system. Once the states are created, they decay due to a process called decoherence. We compare how entangled states can be generated and detected in a realistic experiment, and which classes of states are the most suitable. Furthermore, we compare which classes conserve the entanglement, and quantify the robustness of various classes of entangled states. In the last chapter, we devise a scheme of how to execute a simple quantum algorithm, the Deutsch-Jozsa algorithm, in a system containing another type of solid-state qubit, the so-called flux qubit.
A quantum computer would exploit the phenomena of quantum superposition and entanglement in its functioning and with them offer pathways to solving problems that are too hard or complex to even the best classical computers built today. The implementation of a large-scale working quantum computer could bring about a change in our society rivaling the one started by the digital computer. However, the field is still in its infancy and there are many theoretical and practical issues needing to be solved before large-scale quantum computing can become reality. In digital computers, data is stored in bits. The quantum equivalent is called a qubit (quantum bit) and it is basically a quantum mechanical two-level system that can be in a superposition of its two basis states. There are many different proposals for implementing qubits, but one of the most promising ones is to encode the qubit using electron spins trapped in semiconductor quantum dots. Singlet-triplet qubits are spin qubits where the two-electron spin eigenstates are used as the qubit's basis. The required one and two-qubit operations have already been demonstrated experimentally by several research groups around the world in this qubit architecture. The most severe factor limiting the implementation of larger systems of qubits is decoherence. The qubits are not isolated systems, they interact with their environment, which can lead to the loss of quantum information. Few-electron systems can be simulated accurately using first principle methods that become too taxing when the particle number increases. The topic of this thesis is the simulation of quantum dot singlet-triplet qubit systems using accurate exact diagonalization based methods. The emphasis is on the realistic description of qubit operations, both single-qubit ones and those involving the interaction between neighboring qubits. The decoherence effects are also discussed alongside with certain proposals to alleviate their effects.