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Optics Communications

Coherent manipulation of Rydberg atoms in a triple-microwave driven V+ Ξ configuration

Shuo Mei, Yan Yang, 宋洪亭, Hanyang Leng, Xiaomin Bei, Lei Wang, Jinpeng Yuan, Lirong Wang, Liantuan Xiao, Suotang Jia

Published Oct 17, 2025• 1 citation
Publisher
DOI
10.1016/j.optcom.2025.132569

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Hybrid quantum systems involving cold atoms and microwave resonators can enable cavity-mediated infinite-range interactions between atomic spin systems and realize atomic quantum memories and transducers for microwave-to-optical conversion. To achieve strong coupling of atoms to on-chip microwave resonators, it was suggested to use atomic Rydberg states with strong electric-dipole transitions. Here we report on the experimental realization of coherent coupling of a Rydberg transition of ultracold atoms, trapped on an integrated superconducting atom chip, to the microwave field of an on-chip coplanar waveguide resonator. Close to the chip surface, stray electric fields lead to inhomogeneous Rydberg level shifts, which would hinder coherent interactions of atoms in a cloud with the Rydberg excitation lasers and the microwave cavity field. We, however, use optical excitation of a Rydberg state of atoms in a narrow layer with nearly constant electric field, which allows for resonant coupling of the atoms to the cavity microwave field on an appropriate Rydberg transition. We also achieve state-selective detection of the energetically close Rydberg states. We then observe and characterize cavity-driven Rabi oscillations between a pair of atomic Rydberg states. The residual damping of the oscillations is dominated by the spread of Rabi frequencies of atoms in different positions of the resonant cavity mode, as revealed by our model. Despite the technical challenges, our studies demonstrate the feasibility of coherent-state manipulation of Rydberg atoms interacting with superconducting circuits, paving the way for realization of capable hybrid quantum systems.
The interactions between Rydberg atoms and microwave fields provide a robust platform for exploring non-equilibrium dynamics, exotic phases, and critical phenomena. In this work, we observe a phase transition from bistability to multistability in strongly interacting Rydberg atoms. By tuning the microwave field intensity, we drive the system through a transition from Z 2 - to Z 3 -symmetry breaking. This process features a hidden critical point where multistable states are intrinsically difficult to measure. By manipulating the initial state of the system, we successfully uncover a hidden multistable state and its dynamical trajectory, allowing us to track the hidden critical point. Furthermore, we observe multiple spectral phase transitions, indicating higher-order multistability induced by split Rydberg sublevels. These findings advance the manipulation of multistability in microwave-driven Rydberg systems and open new avenues for applications in non-equilibrium collective atomic physics.