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arXiv:2105.05188 · Physical Review Research

Cavity-driven Rabi oscillations between Rydberg states of atoms trapped on a superconducting atom chip

Manuel Kaiser, Conny Glaser, Li Yuan Ley, Jens Grimmel, H. Hattermann, Daniel Bothner, D. Koelle, R. Kleiner, David Petrosyan, Andreas Günther, József Fortágh

Published Mar 18, 2022• 33 citations
arXivHTMLPDF

Abstract

Hybrid quantum systems involving cold atoms and microwave resonators can enable cavity-mediated infinite-range interactions between atomic spin systems and realize atomic quantum memories and transducers for microwave-to-optical conversion. To achieve strong coupling of atoms to on-chip microwave resonators, it was suggested to use atomic Rydberg states with strong electric-dipole transitions. Here we report on the experimental realization of coherent coupling of a Rydberg transition of ultracold atoms, trapped on an integrated superconducting atom chip, to the microwave field of an on-chip coplanar waveguide resonator. Close to the chip surface, stray electric fields lead to inhomogeneous Rydberg level shifts, which would hinder coherent interactions of atoms in a cloud with the Rydberg excitation lasers and the microwave cavity field. We, however, use optical excitation of a Rydberg state of atoms in a narrow layer with nearly constant electric field, which allows for resonant coupling of the atoms to the cavity microwave field on an appropriate Rydberg transition. We also achieve state-selective detection of the energetically close Rydberg states. We then observe and characterize cavity-driven Rabi oscillations between a pair of atomic Rydberg states. The residual damping of the oscillations is dominated by the spread of Rabi frequencies of atoms in different positions of the resonant cavity mode, as revealed by our model. Despite the technical challenges, our studies demonstrate the feasibility of coherent-state manipulation of Rydberg atoms interacting with superconducting circuits, paving the way for realization of capable hybrid quantum systems.

DOI
10.1103/physrevresearch.4.013207

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Hybrid quantum systems involving cold atoms and microwave resonators can enable cavity-mediated infinite-range interactions between atomic spin systems and realize atomic quantum memories and transducers for microwave-to-optical conversion. To achieve strong coupling of atoms to on-chip microwave resonators, it was suggested to use atomic Rydberg states with strong electric-dipole transitions. Here we report on the experimental realization of coherent coupling of a Rydberg transition of ultracold atoms, trapped on an integrated superconducting atom chip, to the microwave field of an on-chip coplanar waveguide resonator. Close to the chip surface, stray electric fields lead to inhomogeneous Rydberg level shifts, which would hinder coherent interactions of atoms in a cloud with the Rydberg excitation lasers and the microwave cavity field. We, however, use optical excitation of a Rydberg state of atoms in a narrow layer with nearly constant electric field, which allows for resonant coupling of the atoms to the cavity microwave field on an appropriate Rydberg transition. We also achieve state-selective detection of the energetically close Rydberg states. We then observe and characterize cavity-driven Rabi oscillations between a pair of atomic Rydberg states. The residual damping of the oscillations is dominated by the spread of Rabi frequencies of atoms in different positions of the resonant cavity mode, as revealed by our model. Despite the technical challenges, our studies demonstrate the feasibility of coherent-state manipulation of Rydberg atoms interacting with superconducting circuits, paving the way for realization of capable hybrid quantum systems.
Ultracold atoms in their ground states are well-isolated quantum systems offering long coherence times. Hence, ensembles of trapped atoms coupling with on-chip microwave resonators are considered as promising systems for the realization of quantum memories. Here, we demonstrate the coupling of magnetically trapped ultracold 87Rb ground state atoms to a coherently driven superconducting coplanar waveguide resonator. When driving the cavity in resonance with the atomic transition, we observed Rabi oscillations between hyperfine states. This showed the capability in coherent controlling of the atomic states through the cavity field. When driving the cavity on-resonance with the atomic transition, the AC stark shift is observed. This showed the microwave field strength in the cavity seen by atoms. Strong interaction strength of Rydberg atoms in the microwave transition regime has been proposed as an interface during quantum memory writing. Here, we also describe the implementation of a Rydberg system into our experimental setup.
Ensembles of trapped atoms interacting with on-chip microwave resonators are considered as promising systems for the realization of quantum memories, novel quantum gates, and interfaces between the microwave and optical regime. Here, we demonstrate coupling of magnetically trapped ultracold Rb ground-state atoms to a coherently driven superconducting coplanar resonator on an integrated atom chip. When the cavity is driven off-resonance from the atomic transition, the microwave field strength in the cavity can be measured through observation of the AC shift of the atomic hyperfine transition frequency. When driving the cavity in resonance with the atoms, we observe Rabi oscillations between hyperfine states, demonstrating coherent control of the atomic states through the cavity field. These observations enable the preparation of coherent atomic superposition states, which are required for the implementation of an atomic quantum memory.
Abstract Ensembles of trapped atoms interacting with on-chip microwave resonators are considered as promising systems for the realization of quantum memories, novel quantum gates, and interfaces between the microwave and optical regime. Here, we demonstrate coupling of magnetically trapped ultracold Rb ground-state atoms to a coherently driven superconducting coplanar resonator on an integrated atom chip. When the cavity is driven off-resonance from the atomic transition, the microwave field strength in the cavity can be measured through observation of the AC shift of the atomic hyperfine transition frequency. When driving the cavity in resonance with the atoms, we observe Rabi oscillations between hyperfine states, demonstrating coherent control of the atomic states through the cavity field. These observations enable the preparation of coherent atomic superposition states, which are required for the implementation of an atomic quantum memory.
Helium atoms in the 1 s 50 s S 1 3 Rydberg level have been resonantly coupled to the 2 π × 11.722 GHz second harmonic mode of a chip-based superconducting coplanar wave-guide microwave resonator. To achieve this, the single-photon electric-dipole-allowed 1 s 50 s S 1 3 → 1 s 50 p P J 3 transition was tuned into resonance with the resonator mode through the ac Stark shift induced by a second strong 2 π × 3.350 GHz microwave dressing field. The effects of this dressing field, and residual uncanceled dc electric fields at the location of the atoms close to the superconducting chip surface were interpreted with support from Floquet calculations of the energy level structure of the Rydberg states. To observe appreciable population transfer in the 1 µ s atom-resonator interaction time using this transition, which had an electric dipole moment of 1500 e a 0 , pulsed microwave fields were injected into the resonator. From the photon occupation number in the resonator mode under these conditions, the single-photon Rabi frequency associated with the coupling of the atoms to the resonator was estimated to be ∼ 2 π × 100 Hz . These results represent an important step toward operation of this Rydberg-atom–superconducting-circuit interface in the single-photon strong-coupling regime.
Abstract We describe a scheme to coherently convert a microwave photon of a superconducting co-planar waveguide resonator to an optical photon emitted into a well-defined temporal and spatial mode. The conversion is realized by a cold atomic ensemble trapped close the surface of the superconducting atom chip, near the antinode of the microwave cavity. The microwave photon couples to a strong Rydberg transition of the atoms that are also driven by a pair of laser fields with appropriate frequencies and wavevectors for an efficient wave-mixing process. With only several thousand atoms in an ensemble of moderate density, the microwave photon can be completely converted into an optical photon emitted with high probability into the phase matched direction and, e.g. fed into a fiber waveguide. This scheme operates in a free-space configuration, without requiring strong coupling of the atoms to a resonant optical cavity.
Rydberg helium atoms traveling in pulsed supersonic beams have been coupled to microwave fields in a superconducting coplanar waveguide (CPW) resonator. The atoms were initially prepared in the 1s55s ^{3}S_{1} Rydberg level by two-color two-photon laser excitation from the metastable 1s2s ^{3}S_{1} level. Two-photon microwave transitions between the 1s55s ^{3}S_{1} and 1s56s ^{3}S_{1} levels were then driven by the 19.556 GHz third-harmonic microwave field in a quarter-wave CPW resonator. This superconducting microwave resonator was fabricated from niobium nitride on a silicon substrate and operated at temperatures between 3.65 and 4.30 K. The populations of the Rydberg levels in the experiments were determined by state-selective pulsed electric field ionization. The coherence of the atom-resonator coupling was studied by time-domain measurements of Rabi oscillations.