High-sensitivity quantum sensors are a promising tool for experimental searches for beyond-Standard-Model interactions. Here, we demonstrate an atomic comagnetometer operating under a resonantly-coupled hybrid spin-resonance (HSR) regime to probe P-odd, T-even interactions. The HSR regime enables robust nuclear-electron spin coupling, enhancing measurement bandwidth and stability without compromising the high sensitivity of spin-exchange relaxation-free magnetometers. To minimize vibration-related noise from velocity-modulated sources, we implement a multistage vibration isolation system, achieving a vibration-related noise reduction exceeding 700-fold. We establish new constraints on vector-boson-mediated parity-violating interactions, improving experimental sensitivity by three orders of magnitude compared to previous limits. The new constraints complement existing astrophysical and laboratory studies of potential extensions to the Standard Model.
High-sensitivity quantum sensors are a promising tool for experimental searches for beyond-Standard-Model interactions. Here, we demonstrate an atomic comagnetometer operating under a resonantly-coupled hybrid spin-resonance (HSR) regime to probe P-odd, T-even interactions. The HSR regime enables robust nuclear-electron spin coupling, enhancing measurement bandwidth and stability without compromising the high sensitivity of spin-exchange relaxation-free magnetometers. To minimize vibration-related noise from velocity-modulated sources, we implement a multistage vibration isolation system, achieving a vibration-related noise reduction exceeding 700-fold. We establish new constraints on vector-boson-mediated parity-violating interactions, improving experimental sensitivity by three orders of magnitude compared to previous limits. The new constraints complement existing astrophysical and laboratory studies of potential extensions to the Standard Model.
Achieving high energy resolution in spin systems is important for fundamental physics research and precision measurements, with alkali-noble-gas comagnetometers being among the best available sensors. We found a new relaxation mechanism in such devices, the gradient of the Fermi-contact-interaction field that dominates the relaxation of hyperpolarized nuclear spins. We report on precise control over spin distribution, demonstrating a tenfold increase of nuclear spin hyperpolarization and transverse coherence time with optimal hybrid optical pumping. Operating in the self-compensation regime, our $^{21}\mathrm{Ne}\text{\ensuremath{-}}\mathrm{Rb}\text{\ensuremath{-}}\mathrm{K}$ comagnetometer achieves an ultrahigh inertial rotation sensitivity of $3\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}8}\text{ }\text{ }\mathrm{rad}/\mathrm{s}/{\mathrm{Hz}}^{1/2}$ in the frequency range from 0.2 to 1.0 Hz, which is equivalent to the energy resolution of $3.1\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}23}\text{ }\text{ }{\mathrm{eV}/\mathrm{Hz}}^{1/2}$. We propose to use this comagnetometer to search for exotic spin-dependent interactions involving proton and neutron spins. The projected sensitivity surpasses the previous experimental and astrophysical limits by more than 4 orders of magnitude.
Atomic spin sensors are essential for beyond-the-standard-model exploration, biomagnetic measurement, and quantum navigation. While the traditional DC mode spin-exchange relaxation-free (SERF) comagnetometer achieves ultrahigh sensitivity, further improvements require suppressing technical noise and surpassing standard quantum limit. In this work, we develop a K-Rb- 21 Ne SERF atomic comagnetometer that dynamically polarizes the electron and nuclear spins, shielding signals from direct interference by pump light. We establish a three-phase evolutionary model for hybrid spin ensemble dynamics, yielding a complete analytical solution, and analyze the responses to various spin perturbations. Additionally, we achieve an average 39% suppression of the polarization noise and identify the key factors that limit sensitivity improvements. The dynamically polarized comagnetometer exhibits effective suppression of technical noise and holds the potential to overcome quantum noise limit while offering promising applications in exploring new physics and precise magnetic field measurements.
We present a magnetically levitated ferromagnetic vector force sensor that enables selective searches for spin-dependent exotic interactions mediated by beyond-Standard-Model bosons. A defining feature of spin-dependent exotic interactions is that they can generate forces with distinct directional signatures set by the relative spin configuration of the interacting bodies. We show that our sensor resolves these signatures by mapping forces along different axes onto distinct translational modes with different resonance frequencies, thereby separating interaction channels within the same coupling class. As a representative example, we study parity-violating axial-vector--vector interactions mediated by a spin-1 Z′ boson between a sensing and a driving levitated ferromagnet. Using a matched-filter likelihood analysis, we show that a setup based on an already demonstrated experiment can probe the pure electron--electron coupling gAegVe in the previously inaccessible force range λ≲1cm, corresponding to mediator masses MZ′≳10−5eV/c2. Our results establish levitated ferromagnets as a promising platform for millimeter-scale searches for spin-dependent fifth forces and for resolving the multiple effective potentials associated with a given coupling class.
Atomic spin sensors are essential for beyond-the-standard-model exploration, biomagnetic measurement, and quantum navigation. While the traditional DC mode spin-exchange relaxation-free (SERF) comagnetometer achieves ultrahigh sensitivity, further improvements require suppressing technical noise and surpassing standard quantum limit. In this work, we develop a K-Rb-21Ne SERF atomic comagnetometer that dynamically polarizes the electron and nuclear spins, shielding signals from direct interference by pump light. We establish a three-phase evolutionary model for hybrid spin ensemble dynamics, yielding a complete analytical solution, and analyze the responses to various spin perturbations. Additionally, we achieve an averaged 38.5 % suppression of the polarization noise and identify the key factors that limit sensitivity improvements. The dynamically polarized comagnetometer exhibits effective suppression of technical noise and holds the potential to overcome quantum noise limit, while offering promising applications in exploring new physics and precise magnetic field measurements.
Quantum sensing utilizes the quantum resources of well-controlled quantum systems to measure small signals with high sensitivity, and has great potential in both fundamental science and concrete applications. Interacting quantum systems have attracted increasing interest in the field of precise measurements, owing to their potential to generate quantum-correlated states and exhibit rich many-body dynamics. These features provide a novel avenue for exploiting quantum resources in sensing applications. Although previous studies have shown that using such systems can improve sensitivity, they mainly focused on measuring individual physical quantities. In experiment, the challenge of using interacting quantum systems to achieve high-precision measurements of multiple physical parameters simultaneously has not been explored to a large extent. In this study, we demonstrate a first realisation of interaction-based multiparameter sensing by using strongly interacting nuclear spins under ultra-low magnetic field conditions. We find that, as the interaction strength among nuclear spins becomes significantly larger than their Larmor frequencies, a different regime emerges where the strongly interacting spins can be simultaneously sensitive to all components of a multidimensional field, such as a three-dimensional magnetic field. Moreover, we observe that the strong interactions between nuclear spins can increase their quantum coherence times to as long as several seconds, thereby improving measurement precision. Our sensor successfully achieves precision measurement of three-dimensional vector magnetic fields with a field sensitivity reaching the order of 10–11 T and an angular resolution as high as 0.2 rad. Importantly, this approach eliminates the need for external reference fields, thereby avoiding calibration errors and technical noise commonly encountered in traditional magnetometry. Experimentally optimized protocol further enhances the sensitivity of the interacting spin-based sensor by up to five orders of magnitude compared with non-interacting or classical schemes. These results demonstrate the enormous potential of interacting spin systems as a powerful platform for high-precision multi-parameter quantum sensing. The techniques developed here pave the way for a new generation of quantum sensors that use intrinsic spin interactions to exceed the traditional sensitivity limits, presenting a promising route toward ultra-sensitive, calibration-free magnetometry in complex environments.
Precision measurements utilizing atomic spins are widely used in fundamental physics research, inertial sensing, biomagnetism, and the generation of standard quantities. These precision measurements based on quantum sensors have long been disturbed by micro-vibration. In this work, we study the influence of micro-vibration on spin ensembles and perform the experiment on atomic comagnetometer for the first time, which is a powerful tool for search for dark matter and new force, as well as inertial navigation. The model of the effects of micro-vibration on the atomic comagnetometer is established, which considers the transfer characteristics of micro-vibration and the response characteristics of the atomic spin ensembles to the vibration. Moreover, we develop a vibration isolation system, which is a combination of air-floating passive vibration isolators and active feedback systems, to suppress the influence of micro-vibration. Based on the established model and the vibration isolator, we achieve an ultrahigh sensitive comagnetometer, which is among the most sensitive comagnetometer. This work is of wide interest in precision measurement based on quantum sensors and could pave the way for the design of combined vibration isolation systems for such experiments to further improve the sensitivity.